Modified Boron Nitride Nanotubes for Aqueous Solubility

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Solution Overview

Problem

Boron nitride nanotubes (BNNTs) face challenges due to bundling, which limits their utilization in applications despite their advantageous properties, and existing covalent functionalization methods often result in poor solubility in aqueous solutions.

Innovation Solution

The method involves treating BNNTs with a halogen in an aqueous solution to introduce pendant hydroxyl (OH) and amino (NH2) functional groups covalently bonded to the surface of the BNNTs, allowing for solubility in both aqueous and organic solutions.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Manufacturing precision

If BNNTs are purified to remove impurities, then purity is improved, but the nanotubes bundle together due to van der Waals forces, becoming inert and insoluble

Engineering Contradiction:
ImprovepurityVSAvoidsolubility
Core Design Contradiction:
Manufacturing precisionVSEase of operation

Solution Approach 1:

The patent applies parameter changes by introducing chemical functional groups (hydroxyl and amino groups) onto the BNNT surface through halogen treatment. This chemical modification changes the surface parameters of BNNTs, transforming them from hydrophobic and bundling-prone to hydrophilic and soluble, thereby resolving the contradiction between maintaining purity and achieving solubility

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent creates a composite structure by combining BNNTs with functional groups (hydroxyl and amino groups) through covalent bonding. This composite material approach allows the BNNTs to retain their core properties while gaining new solubility characteristics, enabling them to be dispersed in both aqueous and organic solutions without bundling

Inventive Principle:
Principle #40Composite materials

2Ease of operation

If covalent functionalization is used to modify BNNTs, then solubility may be improved, but existing methods often result in poor solubility in aqueous solutions

Engineering Contradiction:
ImprovesolubilityVSAvoidaqueous solubility
Core Design Contradiction:
Ease of operationVSReliability

Solution Approach 1:

The patent applies local quality by selectively introducing specific functional groups (hydroxyl and amino groups) at specific locations on the BNNT surface through halogen treatment. This localized functionalization ensures that the modification occurs at the surface level without compromising the overall structure, achieving reliable aqueous solubility while maintaining the nanotube's core properties

Inventive Principle:
Principle #3Local quality

Solution Approach 2:

The patent changes the chemical parameters of the BNNT surface by introducing polar functional groups (hydroxyl and amino groups) that are compatible with aqueous environments. This parameter change transforms the surface chemistry from hydrophobic to hydrophilic, ensuring reliable solubility in aqueous solutions while maintaining structural integrity

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This approach effectively solubilizes BNNTs, enabling their use in various applications such as surface coatings and composite materials, while maintaining the nanotubes' unique properties.

Implementation Method 1

introduce pendant hydroxyl (OH) and amino (NH2) functional groups covalently bonded to the surface of the BNNTs

Methodology Applied
Scientific EffectCovalent bonding: Chemical Bonding

Implementation Method 2

treating BNNTs with a halogen in an aqueous solution to introduce pendant hydroxyl (OH) and amino (NH2) functional groups

Methodology Applied
Scientific EffectHalogen reaction: Chemical Transport Reactions

Implementation Method 3

The modified BNNTs are soluble in aqueous solutions and in organic solutions

Methodology Applied
Scientific EffectHydrogen bonding: Hydrogenation

Implementation Method 4

allowing for solubility in both aqueous and organic solutions

Methodology Applied
Scientific EffectSolvation: Solvation

Data Source

PatentEP3700981B9Modified boron nitride nanotubes and solutions thereof
Publication Date: 2025.05.21 NAT RES COUNCIL OF CANADA
  • EP3700981B9 patent drawingFigure 1
  • EP3700981B9 patent drawingFigure 2
  • EP3700981B9 patent drawingFigure 3

AI summary

A modified boron nitride nanotube (BNNT) comprising pendant hydroxyl (OH) and amino (NH2) functional groups covalently bonded to a surface of the BNNT. Aqueous and organic solutions of these modified BNNTs are disclosed, along with methods of producing the same. The modified BNNTs and their solutions can be used to coat substrates and to make nanocomposites.