Modified Nanoparticles for Scratch-Resistant Coatings

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Solution Overview

Problem

Existing film-forming compositions face challenges in achieving scratch resistance without using expensive silicone or fluor-based surface active chemicals, which can interfere with other additives and cause storage stability issues, and often result in reduced clarity and increased viscosity.

Innovation Solution

A film-forming composition comprising a resin and modified nanoparticles with an average diameter between 1 and 400 nanometers, adsorbed with a segmented copolymer having an adsorbing segment and a hydrophobic surface active segment that migrates to the surface, providing enhanced scratch resistance without the need for expensive additives.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Strength

If expensive silane coupling agents are used to chemically modify nanoparticles, then surface migration and scratch resistance are improved, but cost increases and storage stability deteriorates due to oligomer formation

Engineering Contradiction:
Improvescratch resistanceVSAvoidstorage stability
Core Design Contradiction:
StrengthVSReliability

Solution Approach 1:

The patent replaces expensive silane coupling agents with inexpensive block copolymers that do not form stable oligomers. The block copolymers provide the necessary surface activity and scratch resistance without the storage stability problems of silane-based modifications, effectively using cheaper alternatives that avoid the harmful side effects.

Inventive Principle:
Principle #27Cheap short-living objects (Disposable)

Solution Approach 2:

The patent changes the chemical nature of the surface modifying agent from silane-based to block copolymer-based. This parameter change eliminates the oligomerization reaction that causes storage instability while maintaining the surface migration capability through the hydrophobic block of the copolymer.

Inventive Principle:
Principle #35Parameter changes

2Strength

If surface active chemicals are added to enhance nanoparticle migration, then scratch resistance improves, but clarity decreases and viscosity increases

Engineering Contradiction:
Improvescratch resistanceVSAvoidclarity
Core Design Contradiction:
StrengthVSIllumination intensity

Solution Approach 1:

The patent combines the dispersant and surface active agent functions into a single block copolymer molecule. The hydrophilic block provides steric stabilization and dispersion, while the hydrophobic block provides surface activity and migration, eliminating the need for separate additives that would compromise clarity and increase viscosity.

Inventive Principle:
Principle #5Merging (Combining)

Solution Approach 2:

The block copolymer performs multiple functions simultaneously: it acts as a dispersant to prevent agglomeration, a surface active agent to enable migration, and a stabilizer to maintain clarity. This multi-functionality eliminates the need for multiple separate additives that would degrade optical properties.

Inventive Principle:
Principle #6Universality (Multi-functionality)

3Strength

If multiple additives are used to disperse and migrate nanoparticles, then scratch resistance improves, but device complexity increases and ease of operation decreases

Engineering Contradiction:
Improvescratch resistanceVSAvoidformulation complexity
Core Design Contradiction:
StrengthVSDevice complexity

Solution Approach 1:

The patent merges the functions of dispersant and surface active agent into a single block copolymer component. This eliminates the need for multiple separate additives and simplifies the formulation process, making it easier to handle and apply while maintaining effective nanoparticle dispersion and migration.

Inventive Principle:
Principle #5Merging (Combining)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The modified nanoparticles effectively enhance scratch resistance and stability of the film-forming composition, maintaining clarity and preventing agglomeration, while being cost-effective and simple to use, suitable for clear coatings on various surfaces including metals and plastics.

Implementation Method 1

modified nanoparticles comprising nanoparticles having an average diameter between 1 and 400 nanometres and adsorbed thereon a segmented copolymer

Methodology Applied
Scientific EffectAdsorption: Adsorption

Implementation Method 2

the hydrophobic segment is more hydrophobic than the resin providing surface migration of the nanoparticles

Methodology Applied
Scientific EffectSurface migration: Surfactant

Data Source

PatentEP2106424B1Film forming composition comprising modified nanoparticles and modified nanoparticles for use in film forming compositions
Publication Date: 2016.11.09 ALLNEX NETHERLANDS BV

AI summary

The present invention relates to afilm forming composition comprisinga resin andmodified nanoparticles comprising nanoparticles and adsorbed thereon a segmented copolymer, preferably a segmented blockcopolymer, comprising an adsorbing segment and a hydrophobic surface active segment, wherein the adsorbing segment has one or more functional groups that adsorb on the nanoparticles and wherein the hydrophobic segment is more hydrophobic than the resin providing surface migration of the nanoparticles. The invention also relates to novelmodified particles and the use of the specified segmented copolymer of specified modified particels in afilm forming composition for imparting thereto improvedsurface properties such as scratch resistance.