Modified Ribotoxin Epitopes Reduce Immunogenicity

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Solution Overview

Problem

Wild-type ribotoxins like α-sarcin, clavin, gigantin, and restrictocin are highly immunogenic, leading to unwanted immune responses when used therapeutically or prophylactically, limiting their efficacy due to their strong binding to human MHC class II molecules and eliciting significant T cell responses.

Innovation Solution

Modified ribotoxin epitopes with specific mutations at critical amino acid positions, such as D9, Q10, P13, T15, N16, Y18, K139, E140, or Q142, reduce binding to human MHC class II and elicit a reduced T cell response, as measured by in vitro assays, thereby minimizing immunogenicity.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If wild-type ribotoxins are used therapeutically, then they can inhibit protein synthesis and kill target cells, but they elicit strong T cell responses and bind to human MHC class II molecules, causing unwanted immune responses

Engineering Contradiction:
Improvetherapeutic efficacyVSAvoidimmunogenicity
Core Design Contradiction:
ReliabilityVSObject-affected harmful factors

Solution Approach 1:

The patent applies parameter changes by introducing specific amino acid substitutions at positions 10, 16, and 139 of the ribotoxin sequence. These parameter changes at critical epitope regions reduce the toxin's binding affinity to human MHC class II molecules while preserving its ribonuclease activity and ability to inhibit protein synthesis in target cells

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent applies local quality by making targeted modifications only at specific amino acid positions (10, 16, and 139) that correspond to T cell epitopes, rather than altering the entire molecule. This localized approach reduces immunogenicity at the epitope level while maintaining the overall structure and catalytic function of the ribotoxin

Inventive Principle:
Principle #3Local quality

2Strength

If wild-type ribotoxins are used, then they maintain full ribonuclease activity, but they exhibit high binding to human MHC class II molecules, limiting therapeutic application

Engineering Contradiction:
Improveribonuclease activityVSAvoidtherapeutic applicability
Core Design Contradiction:
StrengthVSAdaptability or versatility

Solution Approach 1:

The patent introduces specific amino acid substitutions at positions 10, 16, and 139 that change the molecular parameters of the epitope regions. These changes reduce MHC class II binding affinity while preserving the catalytic triad (His50, Glu96, His137) and overall fold necessary for ribonuclease activity

Inventive Principle:
Principle #35Parameter changes

3Object-affected harmful factors

If ribotoxins are modified to reduce immunogenicity, then T cell response is reduced, but there may be loss of ribonuclease activity

Engineering Contradiction:
ImproveT cell responseVSAvoidprotein synthesis inhibition
Core Design Contradiction:
Object-affected harmful factorsVSStrength

Solution Approach 1:

The patent applies local quality by restricting modifications to specific amino acid positions (10, 16, and 139) that are outside the catalytic triad and active site. The substitutions at these localized epitope positions reduce T cell recognition while the core catalytic residues (His50, Glu96, His137) and structural elements remain unchanged, preserving ribonuclease activity

Inventive Principle:
Principle #3Local quality

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The modified ribotoxin epitopes exhibit reduced immunogenicity and T cell stimulation, potentially enhancing their therapeutic or prophylactic applications by minimizing adverse immune reactions.

Implementation Method 1

Without intending to be bound by any theory or mechanism, it is believed that the modified ribotoxin epitopes disclosed in this application possess reduced binding to human MHC class II and/or elicit a reduced T cell response as compared to the corresponding wild type ribotoxin epitopes

Methodology Applied
Scientific EffectMHC class II binding:

Data Source

PatentEP2971038B1Ribotoxin molecules derived from sarcin and other related fungal ribotoxins
Publication Date: 2019.12.04 RES CORP TECH INC
  • EP2971038B1 patent drawingFigure 1
  • EP2971038B1 patent drawingFigure 2
  • EP2971038B1 patent drawingFigure 3A~3B

AI summary

The present application relates to modified T cell epitopes derived from fungal ribotoxins, including a-sarcin, clavin, gigantin, mitogillin, and restrictocin, as well as modified ribotoxin molecules comprising one or more of the modified epitopes. The modified ribotoxin molecules inhibit protein synthesis, like the wild type ribotoxins, but exhibit reduced immunogenicity as compared to the corresponding wild type ribotoxin. Another aspect relates to a fusion protein which comprises a modified ribotoxin fused or conjugated or otherwise linked to a targeting molecule that is effective for binding a target of interest. Another aspect relates to the use of the modified ribotoxin or fusion protein for treating or managing a disease or condition.