Modular Electrolysis-Methanation Reactor for Thermal Coupling

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Solution Overview

Problem

Current energy storage solutions like hydraulic and compressed air storage face geographical limitations and inefficiencies, while hydrogen storage requires significant infrastructure. Additionally, methanation processes are costly due to the need for distinct reactors with different geometries, leading to high investment costs and poor thermal coupling between electrolysis/co-electrolysis and methanation reactions.

Innovation Solution

A modular design for reactors that integrates common components for high-temperature electrolysis/co-electrolysis and methanation, featuring a stack of flat sheets with specific perforations for fluid communication and thermal management, allowing for reduced investment costs and improved thermal coupling between reactions.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If distinct reactors with different geometries are used for electrolysis and methanation, then each reaction can be optimized independently, but investment costs increase and thermal coupling between reactions deteriorates

Engineering Contradiction:
Improvereaction optimizationVSAvoidreactor configuration
Core Design Contradiction:
ReliabilityVSDevice complexity

Solution Approach 1:

The patent combines the electrolysis reactor and methanation reactor into a single integrated reactor system. The electrolysis cell and methanation catalyst are positioned in the same reactor vessel, allowing both reactions to occur in one device. This merging eliminates the need for separate reactors with different geometries, reducing investment costs while enabling thermal coupling between the endothermic electrolysis and exothermic methanation reactions.

Inventive Principle:
Principle #5Merging (Combining)

Solution Approach 2:

The integrated reactor serves multiple functions: it performs both high-temperature electrolysis to produce hydrogen and simultaneous methanation to convert CO2 and H2 into methane. The reactor design accommodates different reaction zones within the same vessel, with the electrolysis cell in one region and the methanation catalyst in another, allowing one device to fulfill multiple process requirements.

Inventive Principle:
Principle #6Universality (Multi-functionality)

2Device complexity

If integrated reactor design is used, then investment costs decrease and thermal coupling improves, but manufacturing complexity increases

Engineering Contradiction:
Improvereactor configurationVSAvoidmanufacturing process
Core Design Contradiction:
Device complexityVSEase of manufacture

Solution Approach 1:

The integrated reactor is constructed using a modular stack of flat sheets, each sheet being a simple, flat component that is easy to manufacture. The sheets are stacked and assembled to form the complete reactor structure, with each sheet containing standardized perforations for fluid communication. This segmentation into simple, repeatable modules makes the manufacturing process more straightforward despite the complex overall functionality.

Inventive Principle:
Principle #1Segmentation

Solution Approach 2:

The patent uses standardized sheet thicknesses (0.1 to 1mm) and standardized perforation patterns that can be manufactured using consistent manufacturing parameters. By maintaining consistent geometric parameters across all sheets and using standard assembly procedures, the manufacturing complexity is reduced despite the integrated design's functional sophistication.

Inventive Principle:
Principle #35Parameter changes

3Manufacturing precision

If flat sheets with standardized perforations are used, then manufacturing precision is improved, but fluid distribution complexity increases

Engineering Contradiction:
Improvesheet geometryVSAvoidfluid distribution
Core Design Contradiction:
Manufacturing precisionVSDevice complexity

Solution Approach 1:

The flat sheets with standardized perforations serve multiple fluid distribution functions simultaneously. The same sheet structure distributes reactants to both the electrolysis cell and the methanation catalyst, collects products from both reactions, and enables thermal coupling. The standardized perforation patterns are designed to handle the complex fluid distribution requirements through their geometric arrangement rather than through complex mechanical components.

Inventive Principle:
Principle #6Universality (Multi-functionality)

Solution Approach 2:

Different regions of the flat sheets have different perforation patterns optimized for their local function. Sheets in contact with the electrolysis cell have perforations optimized for electrolyte and gas distribution, while sheets in contact with the methanation catalyst have perforations optimized for reactant distribution and product collection. This local optimization of perforation patterns allows complex fluid distribution through simple geometric variations.

Inventive Principle:
Principle #3Local quality

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This design reduces the overall size of the reactors, facilitates integration, and enhances thermal management, leading to lower production costs and more efficient energy storage through the production of synthetic natural gas, which can be used in existing infrastructure and has a potentially zero or negative carbon footprint.

Implementation Method 1

a electrolyte membrane, placed between the anodic and cathodic compartments, which is pierced with at least one light for allowing a fluidic communication between said compartments

Methodology Applied
Scientific EffectIon transport through electrolyte membrane: Ion Exchange

Implementation Method 2

converting by heterogeneous catalysis into the desired combustible gas, the synthesis gas previously obtained

Methodology Applied
Scientific EffectHeterogeneous catalysis: Catalysis

Implementation Method 3

electrolysis of water at high temperature (EHT, or EVHT for electrolysis of water vapor at high temperature)

Methodology Applied
Scientific EffectHigh-temperature electrolysis: Electrolysis

Implementation Method 4

co-electrolysis of water and carbon dioxide CO2 at high temperature

Methodology Applied
Scientific EffectCo-electrolysis: Electrolysis

Data Source

PatentEP3233270B1Elementary module for a reactor performing water electrolysis (HTE) or h2o/co2 co-electrolysis or an sofc fuel cell and for a catalytic methanation or reforming reactor
Publication Date: 2023.10.11 COMMISSARIAT A LENERGIE ATOMIQUE ET AUX ENERGIES ALTERNATIVES
  • EP3233270B1 patent drawingFigure 1~2
  • EP3233270B1 patent drawingFigure 3~5
  • EP3233270B1 patent drawingFigure 6A~6B

AI summary

The invention relates to the production, by means of common components, of both HTE reactors or SOFC fuel cells, and of catalytic reactors-heat exchangers such as methanation reactors that are intended to be kept cool and are supplied with H2 or with an H2+CO mixture from an SOEC electrolyser, or reforming reactors that are intended to be kept hot and that are used to supply an SOFC fuel cell, and more generally all types of catalytic reactors that require thermal management of the reaction (cooling or heating).