Monolithic Solid-Phase Channels for Chemical Stability in Metal Separation

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Solution Overview

Problem

Existing metal separation and purification methods, particularly in platinum group metal (PGM) refining, face issues such as chemical degradation of solid phase extractants, instability due to varying eluent concentrations, long elution cycles, broad elution bands, and high dilution of products, which hinder industrial scalability and economic viability.

Innovation Solution

Employing a monolithic solid phase body with functionalized channels for solid phase extraction and optimized liquid-liquid extraction processes, utilizing a monolithic solid phase body with channels to stabilize the extractant under aggressive conditions, enable gradient chromatography, and enhance separation efficiency by controlling flow and pressure.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If traditional solid phase extraction techniques are used with powdered/granular/beaded solid phase extractant media, then metal separation can be achieved, but the extractant stability deteriorates under aggressive chemical conditions

Engineering Contradiction:
Improveextractant stabilityVSAvoidchemical degradation
Core Design Contradiction:
ReliabilityVSObject-affected harmful factors

Solution Approach 1:

The patent employs a monolithic porous solid phase extractant with a continuous porous structure that provides mechanical stability while maintaining high surface area for metal extraction. The porous monolithic structure resists chemical degradation and physical breakdown under aggressive elution conditions, solving the stability problem of traditional particulate extractants.

Inventive Principle:
Principle #31Porous materials

Solution Approach 2:

The patent uses composite monolithic structures combining organic polymer matrices with inorganic support materials or functional groups. This composite approach enhances chemical resistance and structural integrity while maintaining extraction efficiency, addressing the degradation issues of single-material extractants.

Inventive Principle:
Principle #40Composite materials

2Productivity

If concentrated halide eluents are used for metal elution, then metal extraction efficiency is improved, but the solid phase extractant media becomes destabilized due to expansion or contraction

Engineering Contradiction:
Improvemetal extraction efficiencyVSAvoidextractant media stability
Core Design Contradiction:
ProductivityVSStability of the object's composition

Solution Approach 1:

The patent implements gradient elution techniques where eluent concentration is progressively changed from low to high concentrations. This controlled parameter change allows efficient metal extraction while minimizing sudden structural shocks to the monolithic extractant, preventing expansion/contraction destabilization.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent uses dynamic flow rate and concentration gradients during the extraction process. By adjusting these parameters progressively rather than applying maximum conditions immediately, the monolithic structure experiences reduced mechanical stress and maintains stability during high-efficiency extraction.

Inventive Principle:
Principle #15Dynamics

3Manufacturing precision

If traditional packed column chromatography is used, then metal separation can be achieved, but the elution cycle time becomes excessively long

Engineering Contradiction:
Improvemetal separation purityVSAvoidelution cycle time
Core Design Contradiction:
Manufacturing precisionVSLoss of time

Solution Approach 1:

The patent divides the extraction process into multiple parallel columns operating in sequence or parallel fashion. This segmentation allows one column to be eluting while another is being loaded or regenerated, significantly reducing overall cycle time while maintaining separation purity through the same monolithic extractant technology.

Inventive Principle:
Principle #1Segmentation

Solution Approach 2:

The patent implements continuous extraction processes where feed solution continuously flows through the monolithic extractant columns. The monolithic structure's high flow capacity and low backpressure enable continuous operation without the long idle times required by traditional packed columns, maintaining high separation efficiency throughout continuous operation.

Inventive Principle:
Principle #20Continuity of useful action

4Manufacturing precision

If traditional chromatographic separation is used, then metal species can be separated, but broad elution bands result in high dilution of product solutions

Engineering Contradiction:
Improvemetal species separationVSAvoidproduct concentration
Core Design Contradiction:
Manufacturing precisionVSQuantity of substance

Solution Approach 1:

The monolithic porous structure provides uniform flow paths and high surface area to volume ratio, creating sharp elution bands. The controlled porosity ensures consistent metal species interaction with the extractant, preventing band broadening and maintaining high product concentration during elution.

Inventive Principle:
Principle #31Porous materials

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The method improves stability, reduces cycle times, enhances separation and purification efficiency, decreases metal losses, and lowers operating costs, making the process more economically viable for industrial applications.

Implementation Method 1

the surface of the monolithic solid body within the channels is functionalized to selectively adsorb one or more target metal containing species

Methodology Applied
Scientific EffectAdsorption: Adsorption

Implementation Method 2

The metal containing species adsorbed onto the solid phase extractant can subsequently be desorbed from the solid phase extractant, e.g. by washing with a suitable eluent

Methodology Applied
Scientific EffectDesorption: Desorption

Data Source

PatentEP4182051B1Methods for the separation and/or purification of metals
Publication Date: 2025.10.29 JOHNSON MATTHEY PLC
  • EP4182051B1 patent drawingFigure 1~2
  • EP4182051B1 patent drawingFigure 3~4
  • EP4182051B1 patent drawingFigure 5A~5C

AI summary

A method for separating at least two metals from each other in a metal refining process, the method comprising: injecting a feed solution comprising the metals into a column or flow pipe comprising a monolithic solid body having a plurality of channels; and flowing the feed solution through the plurality of channels in the monolithic solid body to separate the metals.