M-SiOx Anode Material Phase Balance for Silicon Volume Stability

Resolve Bottlenecks,
Find Innovative Solutions
Generate Solutions

Solution Overview

Problem

Lithium secondary batteries with silicon-based particles face limitations in initial efficiency and lifespan due to excessive volume changes during charging and discharging, which are not effectively controlled by existing coatings or polymer composites, leading to reduced capacity retention and increased resistance.

Innovation Solution

A negative electrode active material comprising silicon-based particles represented by M-SiOx (where M is Li, Mg, Ca, or Ti) with a crystalline and amorphous phase ratio of 20 wt % to 70 wt %, prepared through vacuum-heating and solid-phase condensation, minimizing internal structural changes and optimizing lithium absorption.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Stability of the object's composition

If a SiO2 layer or carbon coating layer is formed on the silicon-based particle surface, then volume control is improved, but efficiency is reduced due to excessive coating

Engineering Contradiction:
Improvevolume controlVSAvoidefficiency
Core Design Contradiction:
Stability of the object's compositionVSProductivity

Solution Approach 1:

The invention changes the chemical composition parameter by introducing aluminum oxide (Al2O3) into the coating layer formulation. This creates a composite coating with optimized properties that controls volume expansion while maintaining efficiency, resolving the trade-off between volume stability and performance

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The invention uses a composite coating layer comprising SiO2, carbon, and Al2O3. This composite structure combines the volume control benefits of SiO2, the conductivity benefits of carbon, and the structural stability benefits of Al2O3, achieving both volume control and efficiency simultaneously

Inventive Principle:
Principle #40Composite materials

2Stability of the object's composition

If a polymer composite is added on the carbon coating layer, then volume change control is improved, but resistance increases due to decreased conductivity

Engineering Contradiction:
Improvevolume change controlVSAvoidconductivity
Core Design Contradiction:
Stability of the object's compositionVSReliability

Solution Approach 1:

The invention creates a multi-component composite coating layer combining SiO2, carbon, and Al2O3 in specific proportions. The carbon component maintains conductivity while SiO2 and Al2O3 provide volume control, achieving both requirements simultaneously rather than sequentially as in prior art

Inventive Principle:
Principle #40Composite materials

Solution Approach 2:

The invention optimizes the local composition of the coating layer by distributing different materials (SiO2, carbon, Al2O3) in specific ratios throughout the coating structure. This localized optimization ensures that conductivity and volume control properties are balanced at every point in the coating layer

Inventive Principle:
Principle #3Local quality

3Stability of the object's composition

If the silicon-based particle is excessively coated, then volume control is improved, but lithium ion absorption is hindered and capacity is reduced

Engineering Contradiction:
Improvevolume controlVSAvoidlithium ion absorption capacity
Core Design Contradiction:
Stability of the object's compositionVSQuantity of substance

Solution Approach 1:

The invention optimizes the thickness and composition parameters of the coating layer by incorporating Al2O3 and controlling the ratios of SiO2, carbon, and Al2O3. This creates a coating that is thin enough to allow lithium ion penetration but thick enough to control volume expansion, resolving the contradiction between protection and accessibility

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The solution enhances initial efficiency and lifespan characteristics by controlling volume changes and reducing irreversible reactions, resulting in improved discharge capacity and cycle stability.

Implementation Method 1

the M-SiOx includes a crystalline phase and an amorphous phase, and includes the amorphous phase at 20 wt % to 70 wt % based upon a total weight of the M-SiOx

Methodology Applied
Scientific EffectPhase transition: Phase Change

Implementation Method 2

vacuum-heating a powder mixture of Si and SiO2 to form SiOx

Methodology Applied
Scientific EffectVacuum heating: Heating

Implementation Method 3

mixing the SiOx vapor and the M vapor and solid-phase condensing the mixture of the SiOx vapor and the M vapor

Methodology Applied
Scientific EffectSolid-phase condensation: Condensation

Implementation Method 4

a negative electrode active material in which lithium ions exiting the positive electrode are intercalated and deintercalated

Methodology Applied
Scientific EffectIntercalation: Absorption (physical)

Data Source

PatentUS12009515B2Negative electrode active material for lithium secondary battery and preparation method thereof
Publication Date: 2024.06.11 LG ENERGY SOLUTION LTD

AI summary

A negative electrode active material for a lithium secondary battery, which includes a silicon-based particle represented by M-SiOx, wherein M is Li, Mg, Ca, Al, or Ti, and 0≤x<2, wherein the M-SiOx includes an amorphous phase at 20 wt % to 70 wt % based upon a total weight of the M-SiOx, thereby exhibiting excellent initial efficiency and lifespan characteristics, and a preparation method thereof.