Multi-Chamber Oxidation Reactor Steam Control

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Solution Overview

Problem

Current methods for wet oxidation of spent caustic liquor face challenges in achieving optimal sulfur component oxidation with minimum residence time and are not controllable over a wide operating range, especially with varying steam amounts, leading to high peak temperatures that cause corrosive attacks on reactor materials.

Innovation Solution

A multi-chamber oxidation reactor design where spent caustic and oxygen are fed into a larger first chamber, with steam regulation using control devices to distribute steam partially or fully across multiple chambers, reducing sulfide concentrations and allowing for precise temperature control to minimize corrosive attack and optimize conversion.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Productivity

If steam is added to heat the spent liquor in the oxidation reactor, then the oxidation reaction is enhanced, but peak temperatures increase causing corrosive attacks on reactor materials

Engineering Contradiction:
Improveoxidation reaction efficiencyVSAvoidcorrosive attack on reactor materials
Core Design Contradiction:
ProductivityVSObject-affected harmful factors

Solution Approach 1:

The oxidation reactor is divided into multiple chambers (first chamber, second chamber, and additional chambers) that receive steam in different quantities. This segmentation allows distributed heating throughout the reactor volume, preventing concentration of thermal stress and corrosion in a single location while maintaining overall oxidation efficiency.

Inventive Principle:
Principle #1Segmentation

Solution Approach 2:

Different chambers are equipped with different numbers of steam inlets, creating local variations in steam distribution. The first chamber receives a first quantity of steam while subsequent chambers receive progressively less steam, optimizing local heating conditions to balance oxidation efficiency with corrosion prevention in each zone.

Inventive Principle:
Principle #3Local quality

2Productivity

If the reactor operates at high pressure and temperature to reduce residence time, then conversion efficiency improves, but the corrosive attack on reactor materials intensifies

Engineering Contradiction:
Improveconversion efficiencyVSAvoidcorrosive attack on reactor materials
Core Design Contradiction:
ProductivityVSObject-affected harmful factors

Solution Approach 1:

By dividing the reactor into multiple chambers with different steam injection rates, the system achieves high conversion efficiency through controlled heating while distributing the thermal load to prevent localized corrosive attacks. The segmented structure allows optimized temperature profiles that balance reaction kinetics with material durability.

Inventive Principle:
Principle #1Segmentation

Solution Approach 2:

The invention changes the steam injection parameters across different chambers, using varying quantities of steam to create optimized temperature and pressure profiles in each zone. This parameter variation allows the system to operate at high conversion efficiency while controlling peak temperatures that would otherwise intensify corrosive attack on the reactor materials.

Inventive Principle:
Principle #35Parameter changes

3Productivity

If steam is injected in large quantities to ensure adequate heating, then the oxidation reaction is enhanced, but the operating range becomes narrower and control difficulty increases

Engineering Contradiction:
Improveoxidation reaction rateVSAvoidoperating range
Core Design Contradiction:
ProductivityVSAdaptability or versatility

Solution Approach 1:

The reactor is segmented into multiple chambers with independent steam injection control. This allows the system to operate over a wide range of total steam quantities by adjusting the distribution pattern across chambers. Each chamber can be independently optimized for different operating conditions, maintaining adaptability while ensuring adequate heating for oxidation reactions.

Inventive Principle:
Principle #1Segmentation

Solution Approach 2:

The steam injection system is designed to be dynamically adjustable, with the ability to vary steam quantities and distribution patterns across different chambers based on operating conditions. This dynamic control enables the system to adapt to different feed rates, sulfur concentrations, and desired residence times, widening the operational range while maintaining reaction effectiveness.

Inventive Principle:
Principle #15Dynamics

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This approach allows for efficient oxidation of sulfur components with reduced residence time and wider operating range, minimizing corrosive damage to reactor materials by controlling steam quantity and temperature, thereby enhancing the overall conversion process.

Implementation Method 1

Steam is fed into the oxidation reactor

Methodology Applied
Scientific EffectHeating: Heating

Implementation Method 2

The lye and oxygen or the lye and an oxygen-containing gas mixture, for example air, are supplied to the first chamber

Methodology Applied
Scientific EffectOxidation: Oxidation

Data Source

PatentEP3784373B1Method and oxidation reactor for treating a spent liquor containing sulphides
Publication Date: 2022.06.22 LINDE AG
  • EP3784373B1 patent drawingFigure 1
  • EP3784373B1 patent drawingFigure 2~3B

AI summary

The invention relates to a method for treating a sulphide-containing waste lye from a caustic treatment, in which method the waste lye and oxygen or an oxygen-containing gas mixture are fed to an oxidation reactor (10) and subjected therein to wet oxidation, wherein steam is fed into the oxidation reactor (10). According to the invention, an oxidation reactor (10) is used comprising a number of chambers (11-19), of which a first chamber (11) has a larger volume than a second chamber (12), wherein the waste lye and the oxygen or the oxygen-containing gas mixture is fed to the first chamber (11), fluid flowing out of the first chamber (11) is transferred to the second chamber (12), a steam quantity and/or steam temperature of the steam fed into the oxidation reactor (10) is controlled using a control device (TIC), and at least part of the steam fed into the oxidation reactor (10) is fed into the first chamber (11) and into the second chamber (12). The invention also relates to a corresponding system (100) and a corresponding oxidation reactor (10).