Multiferroic Nanodevice for Electric-Field Magnon-NV Spin Tuning

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Solution Overview

Problem

Existing methods for controlling the interaction between magnons and quantum spin defects (QSDs) face challenges in localizing magnetic fields at the nanoscale with minimal heating, which affects quantum coherence, and direct electric field coupling to QSDs has limitations in sensitivity and operational temperature.

Innovation Solution

A hybrid nanodevice system combining ferroelectric-ferromagnetic multiferroics with QSDs is engineered to enable electric-field control of magnon-QSD interaction, utilizing ferroelectric polarization to tune magnetic anisotropy and microwave fields, enhancing defect spin-based sensing and coherent manipulation.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Ease of operation

If a control magnetic field is applied to tune magnon-QSD interaction, then the interaction can be controlled, but it is challenging to localize the magnetic field at the nanoscale

Engineering Contradiction:
Improvecontrol of magnon-QSD interactionVSAvoidlocalization of magnetic field at nanoscale
Core Design Contradiction:
Ease of operationVSLength of moving object

Solution Approach 1:

The patent introduces an electric field as an intermediary to indirectly control the magnon-QSD interaction. Instead of directly applying a magnetic field, an electric field is applied to the ferroelectric substrate, which modulates the magnetic anisotropy of the ferromagnetic layer, thereby tuning the magnon resonance frequency and controlling the interaction with QSDs. This intermediary approach enables nanoscale localization without the challenges of direct magnetic field confinement.

Inventive Principle:
Principle #24Intermediary (Mediator)

Solution Approach 2:

The patent replaces the magnetic field control mechanism with an electric field control mechanism. By substituting the magnetic control approach (which suffers from localization difficulties) with an electric field approach through the multiferroic heterostructure, the system achieves precise nanoscale control of magnon-QSD interaction through voltage application to the ferroelectric substrate.

Inventive Principle:
Principle #28Mechanics substitution (Replace mechanical system)

2Ease of operation

If electric current is used to control magnon-QSD interaction via spin-orbit torque, then the interaction can be tuned, but Joule heating is generated which negatively affects quantum coherence

Engineering Contradiction:
Improvetuning of magnon-QSD interactionVSAvoidJoule heating affecting quantum coherence
Core Design Contradiction:
Ease of operationVSTemperature

Solution Approach 1:

The patent replaces the current-based spin-orbit torque control mechanism with an electric field-based control mechanism. Instead of passing current through the ferromagnetic layer (which generates Joule heating), an electric field is applied to the ferroelectric substrate to modulate the magnetic anisotropy. This substitution eliminates resistive heating while maintaining the ability to tune the magnon-QSD interaction, thereby preserving quantum coherence.

Inventive Principle:
Principle #28Mechanics substitution (Replace mechanical system)

Solution Approach 2:

The patent changes the control parameter from electric current to electric field voltage. By applying voltage to the ferroelectric substrate, the magnetic anisotropy energy is modulated, which tunes the magnon resonance frequency and controls the interaction with QSDs. This parameter change from current to voltage eliminates the Joule heating problem while achieving the desired tuning functionality.

Inventive Principle:
Principle #35Parameter changes

3Temperature

If direct electric field coupling is used to control QSDs, then heating is minimized, but sensitivity and operational temperature are limited

Engineering Contradiction:
Improveminimal heating preserving quantum coherenceVSAvoidelectric field sensitivity and operational temperature
Core Design Contradiction:
TemperatureVSMeasurement precision

Solution Approach 1:

The patent employs a multiferroic heterostructure composite consisting of a ferroelectric substrate and a ferromagnetic layer. This composite material system combines the advantages of both ferroelectric and ferromagnetic properties, enabling electric field control of magnetism. The ferroelectric component provides minimal heating and high sensitivity to electric fields, while the ferromagnetic component enables magnon resonance and spintronic functionality, together overcoming the limitations of direct electric field coupling to QSDs.

Inventive Principle:
Principle #40Composite materials

Solution Approach 2:

The patent changes the operational parameters by introducing a ferroelectric substrate that can be tuned via applied voltage. This allows dynamic control of the magnetic anisotropy and magnon resonance frequency, enhancing the sensitivity and extending the operational temperature range of the device while maintaining minimal heating through electric field control.

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The system achieves up to 400% tuning of NV-spin relaxation rates and improves electric field sensitivity by several orders of magnitude, enabling efficient electric-field-tunable quantum spintronic devices and single spin probes.

Implementation Method 1

In response to an applied voltage, the ferroelectric substrate can change an electric polarization of the ferroelectric substrate

Methodology Applied
Scientific EffectFerroelectric effect: Piezoelectric Effect

Implementation Method 2

induce a strain in the ferromagnetic material

Methodology Applied
Scientific EffectPiezoelectric effect: Piezoelectric Effect

Implementation Method 3

a magnon excitation spectrum of the ferromagnetic material is configured such that it changes with respect to an electron spin resonance (ESR) frequency of the NV ensemble

Methodology Applied
Scientific EffectMagnon resonance: Resonance

Implementation Method 4

The coupling mediated by the dipolar field components that are transverse to the NV-spin quantization axis can form the basis for quantum devices and sensors based on magnon-QSD hybrids

Methodology Applied
Scientific EffectZeeman effect: Zeeman Effect

Data Source

PatentUS12474418B2Nanodevice, method of making the same, and method of using the same
Publication Date: 2025.11.18 PURDUE RES FOUND
  • US12474418B2 patent drawing
  • US12474418B2 patent drawing
  • US12474418B2 patent drawing

AI summary

A nanodevice provides for electric-field control of magnon-QSD interactions. The nanodevice includes a ferroelectric substrate, a ferromagnetic material disposed over the ferroelectric substrate, and a nanodiamond including an ensemble of nitrogen-vacancy (NV) spins, each NV magnetically interfacing with the ferromagnetic material. An electric field is measured by applying a voltage across the ferroelectric substrate and the ferromagnetic material, changing a magnon excitation spectrum of the ferromagnetic material with respect to an electron spin resonance frequency of the ensemble of NV spins, and measuring a relaxation rate of the ensemble of NV spins.