Multiplexed Transdermal Glucose Sensor Array

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Solution Overview

Problem

Existing non-invasive glucose monitoring devices face challenges such as variable dilution factors due to large skin areas, requiring frequent calibration and operating close to their limits of detection, especially during hypoglycemia, which limits their effectiveness and commercial success.

Innovation Solution

A multiplexed transdermal extraction and detection system using a miniaturized iontophoretic sampling device with an array of sensor pixels that target preferential pathways in the skin, allowing for semi-continuous or continuous monitoring of glucose levels without the need for finger-stick calibration, by employing graphene-based electrodes and platinum nanoparticles for enhanced detection sensitivity.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Measurement precision

If a large skin area is used for transdermal extraction, then the detection limit is improved, but the dilution factor becomes variable and calibration is required

Engineering Contradiction:
Improvedetection limitVSAvoiddilution factor variability
Core Design Contradiction:
Measurement precisionVSReliability

Solution Approach 1:

The patent divides the sensing area into multiple independently addressable sensor pixels arranged in an array. Each pixel can be individually activated to sample from a specific location, enabling selective sampling while maintaining overall detection sensitivity. This segmentation allows the system to achieve both improved detection limits through multiple pixels and reduced dilution factor variability by selecting specific sampling locations.

Inventive Principle:
Principle #1Segmentation

2Quantity of substance

If a large skin area is used for transdermal extraction, then more substance is extracted, but the device requires frequent calibration

Engineering Contradiction:
Improveextracted substance amountVSAvoidcalibration frequency
Core Design Contradiction:
Quantity of substanceVSEase of operation

Solution Approach 1:

By segmenting the sensing area into multiple pixels, the system can extract substance through multiple parallel pathways simultaneously, increasing the total quantity extracted. The multiplexed readout capability allows data from multiple pixels to be combined, enhancing the overall signal while maintaining consistent extraction characteristics that reduce calibration needs.

Inventive Principle:
Principle #1Segmentation

Solution Approach 2:

The patent employs graphene-based electrodes and platinum nanoparticles to enhance detection sensitivity, allowing the system to detect lower concentrations of analytes. This parameter change in detection sensitivity means that frequent calibration is no longer necessary even when extracting larger quantities of substance through multiple pixels.

Inventive Principle:
Principle #35Parameter changes

3Ease of operation

If miniaturized sensor pixels are used to target preferential pathways, then calibration-free monitoring is achieved, but the detection sensitivity may be reduced

Engineering Contradiction:
Improvecalibration requirementVSAvoiddetection sensitivity
Core Design Contradiction:
Ease of operationVSMeasurement precision

Solution Approach 1:

The patent creates an array of miniaturized sensor pixels that can be individually addressed. While each pixel is small, the collective array provides sufficient detection sensitivity by combining signals from multiple pixels. The ability to selectively activate specific pixels allows the system to maintain calibration-free operation while achieving the required detection sensitivity through signal aggregation.

Inventive Principle:
Principle #1Segmentation

Solution Approach 2:

The use of graphene-based electrodes combined with platinum nanoparticles creates a composite material structure that significantly enhances detection sensitivity. This composite approach allows miniaturized pixels to achieve sensitivity levels comparable to or exceeding larger traditional sensors, thereby maintaining both the calibration-free advantage and the required measurement precision.

Inventive Principle:
Principle #40Composite materials

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

Enables clinically relevant, non-invasive glucose monitoring with reduced variability in dilution factors, improved sensitivity, and the ability to detect glucose levels across a wide range without calibration, enhancing the accuracy and reliability of glucose monitoring.

Implementation Method 1

transdermal extraction and detection of substances, such as glucose via reverse iontophoresis

Methodology Applied
Scientific EffectReverse iontophoresis: Iontophoresis

Implementation Method 2

selective sampling of interstitial and biological fluids

Methodology Applied
Scientific EffectIontophoresis: Iontophoresis

Implementation Method 3

electrochemically detected

Methodology Applied
Scientific EffectElectrochemical detection: Redox Reactions

Data Source

PatentEP3448258B1Multiplexed transdermal extraction and detection system for non-invasive monitoring of substances and method of use
Publication Date: 2024.06.26 UNIVERSITY OF BATH
  • EP3448258B1 patent drawingFigure 1
  • EP3448258B1 patent drawingFigure 2a~3
  • EP3448258B1 patent drawingFigure 4

AI summary

Multiplexed transdermal extraction and detection devices and systems for non-invasive monitoring of substances, such as glucose, are disclosed, as are methods of using these devices for substance monitoring in subjects.