Multistage Nanofiltration Concentrate Processing to Reduce Monovalent Ions

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Solution Overview

Problem

Existing nanofiltration systems face challenges in achieving complete separation of monovalent ions from brine, resulting in high monovalent ion content in the final concentrate, necessitating improved methods to lower this content and enhance separation efficiency.

Innovation Solution

A nanofiltration system with at least three stages and concentrate staging, incorporating a recirculation pump, pH adjustment, and temperature control units to manage pH between 2 to 7 and temperature between 20°C to 60°C, along with optional deionized water dilution, to optimize the separation process.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Manufacturing precision

If nanofiltration membrane is used to separate monovalent ions from brine, then divalent and multi-valent ions are retained effectively, but monovalent ion content in the final concentrate remains relatively high

Engineering Contradiction:
Improveseparation efficiencyVSAvoidmonovalent ion content in concentrate
Core Design Contradiction:
Manufacturing precisionVSQuantity of substance

Solution Approach 1:

The system divides the nanofiltration process into multiple stages (at least three stages) with concentrate staging between them. Each stage processes the concentrate from the previous stage, progressively reducing monovalent ion content through sequential separation steps rather than attempting complete separation in a single stage.

Inventive Principle:
Principle #1Segmentation

Solution Approach 2:

The system adjusts operating parameters including pH control (using acid or base to adjust feed pH) and temperature control (heating or cooling the feed) to optimize membrane performance. These parameter changes enhance the membrane's ability to reject monovalent ions while maintaining divalent ion retention.

Inventive Principle:
Principle #35Parameter changes

2Productivity

If multiple-stage nanofiltration system with concentrate staging is implemented, then recovery rate is improved, but monovalent ion content in final concentrate increases

Engineering Contradiction:
Improverecovery rateVSAvoidmonovalent ion content in concentrate
Core Design Contradiction:
ProductivityVSQuantity of substance

Solution Approach 1:

The concentrate stream is segmented and processed through multiple sequential stages rather than being discharged after a single stage. This segmentation allows progressive concentration of divalent ions while continuously removing monovalent ions at each stage, achieving both high recovery and low monovalent content.

Inventive Principle:
Principle #1Segmentation

Solution Approach 2:

The system maintains continuous processing of the concentrate stream through all stages without interruption. The concentrate from each stage is immediately fed to the next stage, ensuring continuous separation action that progressively reduces monovalent ion content while maximizing water recovery.

Inventive Principle:
Principle #20Continuity of useful action

3Manufacturing precision

If pH adjustment is applied to optimize separation, then monovalent ion rejection is improved, but system complexity increases

Engineering Contradiction:
Improveion separation efficiencyVSAvoidsystem complexity
Core Design Contradiction:
Manufacturing precisionVSDevice complexity

Solution Approach 1:

Chemical intermediaries (acids or bases) are introduced to adjust the pH of the feed stream. This pH adjustment serves as an intermediary step that modifies the ionic environment to enhance membrane selectivity, improving monovalent ion rejection without requiring fundamental changes to the membrane or system architecture.

Inventive Principle:
Principle #24Intermediary (Mediator)

4Manufacturing precision

If temperature control is implemented to enhance separation, then membrane performance is improved, but energy consumption increases

Engineering Contradiction:
Improveseparation performanceVSAvoidenergy consumption
Core Design Contradiction:
Manufacturing precisionVSUse of energy by moving object

Solution Approach 1:

Temperature is adjusted as a controllable parameter to optimize membrane performance. By heating or cooling the feed stream to specific temperature ranges, the membrane's selective properties are enhanced, improving separation efficiency. The temperature control allows the system to operate at optimal conditions without requiring excessive energy input.

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The method effectively reduces the monovalent ion content in the final concentrate, improving the separation efficiency of monovalent ions from divalent or multivalent ions, achieving a lower concentration of monovalent ions in the final concentrate compared to the brine input.

Implementation Method 1

Nanofiltration (NF) is a membrane separation technology between osmosis and ultrafiltration. The cutoff relative molecular weight of a nanofiltration membrane may be between 200 and 2000 and the membrane pore size may be around 1-2 nm.

Methodology Applied
Scientific EffectNanofiltration: Semipermeable Membrane

Implementation Method 2

A nanofiltration membrane can effectively retain bivalent and multi-valent ions and organics with a relative molecular weight greater than 200, while most of monovalent inorganic salts can pass through.

Methodology Applied
Scientific EffectIon rejection: Electrostatic Induction

Implementation Method 3

recirculating a first portion of the concentrate produced by the last stage to the last stage

Methodology Applied
Scientific EffectRecirculation: Pump

Implementation Method 4

controlling the feed liquid in a pH range of 2 to 7

Methodology Applied
Scientific EffectpH control:

Implementation Method 5

controlling the feed liquid in a temperature range of 20 °C to 60 °C

Methodology Applied
Scientific EffectTemperature control:

Implementation Method 6

deionized water is fed through an inlet of a stage of a membrane system to dilute the feed stream to the stage

Methodology Applied
Scientific EffectDilution:

Data Source

PatentEP3606646B1Method for reducing monovalent ions in concentrate of nanofiltration system and the nanofiltration system
Publication Date: 2025.09.17 BL TECHNOLOGY INC
  • EP3606646B1 patent drawingFigure 1
  • EP3606646B1 patent drawingFigure 2
  • EP3606646B1 patent drawingFigure 3

AI summary

This specification describes a method for lowering the content of monovalent ions in a final concentrate of a nanofiltration system relative to a brine and a corresponding nanofiltration system. The nanofiltration system comprises at least three stages of nanofiltration, wherein the concentrate from each segment flows into the next segment. A feed stream is sent into one stage to generate a concentrate stream, and a first portion of the concentrate stream is recirculated to the one stage. The pH of the feed stream is controlled in a range of 2-7. The temperature of the feed stream is in a range of 20-60°C. The feed stream includes the recirculated concentrate stream and at least part of a concentrate generated from an upstream stage. The method and the system described herein can reduce the concentration of monovalent ions in the final concentrate during a nanofiltration separation process.