Nanocellulose Production via Oxidation and Sonication

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Solution Overview

Problem

Current methods for producing nanocellulose, such as acid hydrolysis and mechanical defibrillation, face limitations including low yield, high energy consumption, and increased costs due to the use of harsh chemicals like sulfuric acid and TEMPO, which also result in damaged microfibril structures and environmental concerns.

Innovation Solution

A method involving oxidation and sonication of natural fibers using a chemical oxidant like NaClO or H2O2, in conjunction with a swelling agent, to produce nanocellulose with improved yield, mechanical properties, and reduced environmental impact, while utilizing cheaper oxidants and minimizing waste.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If acid hydrolysis is used to produce nanocellulose, then a stable suspension with high negative charge is obtained, but the yield is low and scaling up is limited

Engineering Contradiction:
Improvestability of nanocellulose suspensionVSAvoidyield of nanocellulose
Core Design Contradiction:
ReliabilityVSProductivity

Solution Approach 1:

The patent changes the chemical parameters by replacing sulfuric acid with oxidizing agents (NaClO, H2O2) and adjusting pH conditions using swelling agents (NaOH, Na2CO3, KOH). This parameter change enables high yield production while maintaining suspension stability through controlled oxidation rather than acid hydrolysis

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent uses cheap, readily available oxidizing agents like sodium hypochlorite and hydrogen peroxide instead of expensive specialized reagents. These conventional chemicals can be easily obtained and disposed of, making the process economically viable for large-scale production

Inventive Principle:
Principle #27Cheap short-living objects (Disposable)

2Strength

If mechanical defibrillation is used, then longer and entangled nanoscale cellulose elements are obtained, but energy consumption increases and microfibril structure is damaged

Engineering Contradiction:
Improvenetwork strength of nanocelluloseVSAvoidenergy consumption for disintegration
Core Design Contradiction:
StrengthVSUse of energy by moving object

Solution Approach 1:

The patent replaces the mechanical defibrillation system with a chemical oxidation system. Instead of using mechanical homogenizers that consume high energy and damage microfibrils, the invention uses controlled chemical oxidation with NaClO or H2O2 to achieve fibrillation, thereby reducing energy consumption while preserving the microfibril structure

Inventive Principle:
Principle #28Mechanics substitution (Replace mechanical system)

Solution Approach 2:

The patent employs strong oxidizing agents (NaClO, H2O2) to accelerate the oxidation process, enabling efficient breakdown of cellulose into nanofibrils without requiring excessive mechanical energy input. The oxidation reaction itself provides the driving force for fibrillation

Inventive Principle:
Principle #38Strong oxidants (Accelerated oxidation)

3Productivity

If TEMPO pretreatment is used, then energy consumption is reduced and high yield is achieved, but the cost increases and waste treatment becomes an issue

Engineering Contradiction:
Improveyield of nanocelluloseVSAvoidcost of fabrication
Core Design Contradiction:
ProductivityVSEase of manufacture

Solution Approach 1:

The patent replaces the expensive TEMPO catalyst with cheap, conventional oxidizing agents like sodium hypochlorite and hydrogen peroxide that are readily available and inexpensive. This substitution maintains high yield while dramatically reducing the cost of fabrication and simplifying waste treatment

Inventive Principle:
Principle #27Cheap short-living objects (Disposable)

Solution Approach 2:

The patent achieves similar results to TEMPO pretreatment using alternative chemical systems (NaClO, H2O2) that copy the oxidative function without requiring the expensive TEMPO catalyst. The alternative systems provide comparable nanocellulose yield and quality at a fraction of the cost

Inventive Principle:
Principle #26Copying

4Productivity

If high concentration of sulfuric acid is used, then nanocellulose production is achieved, but the acid/solid ratio becomes too high for industrial scaling

Engineering Contradiction:
Improveproduction of nanocelluloseVSAvoidacid/solid ratio
Core Design Contradiction:
ProductivityVSQuantity of substance

Solution Approach 1:

The patent replaces the requirement for high concentration sulfuric acid with cheap, dilute oxidizing agents like sodium hypochlorite and hydrogen peroxide. These substances can be used at much lower concentrations and ratios, making the process suitable for industrial scaling while maintaining production effectiveness

Inventive Principle:
Principle #27Cheap short-living objects (Disposable)

Solution Approach 2:

The patent fundamentally changes the chemical parameters from acid-based hydrolysis to oxidation-based fibrillation. This parameter change eliminates the need for high acid/solid ratios, allowing the process to be scaled up industrially without the logistical and safety issues associated with handling concentrated acids

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This method achieves a high yield of nanocellulose with enhanced mechanical performance, increased tensile strength, and stability, reducing production costs and environmental footprint, and can be used to improve recycled paper products.

Implementation Method 1

A method involving oxidation and sonication of natural fibers using a chemical oxidant like NaClO or H2O2

Methodology Applied
Scientific EffectOxidation: Oxidation

Implementation Method 2

A method involving oxidation and sonication of natural fibers

Methodology Applied
Scientific EffectCavitation: Cavitation

Data Source

PatentEP3204171B1Method of producing nanocellulose
Publication Date: 2020.04.29 BRUNEL UNIVERSITY
  • EP3204171B1 patent drawingFigure 1~2
  • EP3204171B1 patent drawingFigure 3~4
  • EP3204171B1 patent drawingFigure 5~6

AI summary

A method of producing nanocellulose includes defibrillating cellulosic raw material by oxidation with an oxidant such as NaClOor H2O2 and sonication in the presence of a swelling agent. The nanocellusose produced by the method can be used in a method of recycling cellulosic material such as paper, card, cardboard or wood to produce recycled paper.