Stable Nanodiamond Dispersion via pH and Conductivity Control

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Solution Overview

Problem

Existing methods for producing nanodiamond dispersions result in unstable colloids with large particle diameters and low concentrations, prone to aggregation over time, especially at high concentrations.

Innovation Solution

A method involving the purification of detonation nanodiamond aggregates by adjusting the pH to 8-10.5 and electric conductivity to 300 µS/cm or less, followed by deaggregation using a bead mill or ultrasonic treatment, to produce a stable single-nano-sized nanodiamond dispersion with a concentration of 4 weight percent or more.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Quantity of substance

If nanodiamond particles are produced by detonation technique and dispersed in water, then high concentration dispersion can be achieved, but the particles undergo aggregation over time and particle diameter increases

Engineering Contradiction:
ImproveconcentrationVSAvoiddispersion stability
Core Design Contradiction:
Quantity of substanceVSStability of the object's composition

Solution Approach 1:

The patent applies preliminary action by adjusting the pH to 8-10.5 and electric conductivity to 300 µS/cm or less before dispersion. This pre-treatment of the nanodiamond aggregates creates optimal conditions for stable high-concentration dispersion, preventing aggregation before it occurs. The pH adjustment and conductivity control are performed in advance to ensure long-term stability.

Inventive Principle:
Principle #10Preliminary action

Solution Approach 2:

The patent changes key parameters including pH (adjusted to 8-10.5), electric conductivity (reduced to 300 µS/cm or less), and uses deaggregation treatment. These parameter changes transform the nanodiamond aggregates into a stable dispersion state that maintains both high concentration and long-term stability without aggregation.

Inventive Principle:
Principle #35Parameter changes

2Manufacturing precision

If bead mill or ultrasonic homogenizer is used to pulverize nanodiamond aggregates, then particle size is reduced to single-nano-sized, but the concentration becomes low

Engineering Contradiction:
Improveparticle sizeVSAvoidconcentration
Core Design Contradiction:
Manufacturing precisionVSQuantity of substance

Solution Approach 1:

The patent applies partial action by using deaggregation treatment (bead mill or ultrasonic homogenizer) selectively on the nanodiamond aggregates under controlled conditions. Rather than excessive pulverization that would dilute the dispersion, the treatment is applied just enough to achieve single-nano-sized particles while maintaining high concentration through the optimized pH and conductivity parameters.

Inventive Principle:
Principle #16Partial or excessive action

3Duration of action of stationary object

If nanodiamond dispersion is left stand at room temperature for long time, then aggregation gradually occurs and particle diameter increases, but maintaining stability requires additional control measures

Engineering Contradiction:
Improvestorage timeVSAvoidparticle size stability
Core Design Contradiction:
Duration of action of stationary objectVSStability of the object's composition

Solution Approach 1:

The patent applies preliminary action by adjusting the pH to 8-10.5 and electric conductivity to 300 µS/cm or less before storage. This pre-treatment creates a stable environment that prevents aggregation during long-term storage at room temperature, allowing the dispersion to maintain its properties over extended periods without additional control measures.

Inventive Principle:
Principle #10Preliminary action

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The method achieves excellent dispersion stability even at high concentrations, preventing aggregation and maintaining particle size stability over time, resulting in a highly stable single-nano-sized nanodiamond dispersion.

Implementation Method 1

pulverized using a disperser such as a bead mill or an ultrasonic homogenizer

Methodology Applied
Scientific EffectUltrasonic cavitation: Cavitation

Implementation Method 2

The agglutinate structure was broken up using a bead mill

Methodology Applied
Scientific EffectMechanical force: Mechanical Force

Data Source

PatentEP3216758B1Suspension of nanodiamond aggregates and single-nano-sized nanodiamond dispersion
Publication Date: 2021.10.13 DAICEL CORP

AI summary

A suspension of nanodiamond aggregates according to the present invention is a suspension of detonation nanodiamond aggregates. The suspension has such a pH and an electric conductivity as to meet one of conditions (1) and (2) as follows. (1) The suspension has a pH of 4 to 7 and an electric conductivity of 50 µS/cm or less per weight percent of the solids concentration of the suspension; and (2) the suspension has a pH of 8 to 10.5 and has an electric conductivity of 300 µS/cm or less per weight percent of the solids concentration of the suspension.