Nanoparticle-Coated Proppants for Crush Resistance

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Solution Overview

Problem

Conventional proppants, such as sand and ceramic particles, lack sufficient crush resistance and durability in downhole environments, leading to fracture closure and reduced oil and gas production due to degradation in wet conditions and high temperatures.

Innovation Solution

Development of nanoparticle-coated proppants with a coating comprising unfunctionalized organic resin, strengthening agents like carbon nanotubes and silica, and functionalized nanoparticles that provide hydrophobic and oleophobic properties, enhancing mechanical strength and resistance to chemical degradation.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Strength

If sand particles are used as proppants, then they provide sufficient quantity and low cost, but they lack crush resistance due to polycrystalline nature

Engineering Contradiction:
Improvecrush resistanceVSAvoiddurability in downhole conditions
Core Design Contradiction:
StrengthVSReliability

Solution Approach 1:

The patent applies composite materials by coating sand proppants with a multi-component coating system consisting of organic resin matrix combined with inorganic strengthening agents (alumina, silica, titania nanoparticles) and hydrophobic additives. This composite coating structure provides both mechanical strength to prevent crushing and chemical resistance to withstand downhole wet and hot conditions, resolving the contradiction between using inexpensive sand and achieving sufficient durability.

Inventive Principle:
Principle #40Composite materials

2Strength

If ceramic proppants are used, then crush resistance is improved, but they break down in wet conditions and high temperatures

Engineering Contradiction:
Improvecrush resistanceVSAvoidchemical stability in wet conditions
Core Design Contradiction:
StrengthVSStability of the object's composition

Solution Approach 1:

The patent changes the chemical parameters of the coating by incorporating hydrophobic additives (fluorinated compounds, silicones, waxes) that fundamentally alter the coating's interaction with water. This parameter change provides chemical stability and water resistance to the coating system, preventing ceramic proppant breakdown in wet downhole conditions while maintaining the crush resistance benefits of ceramic materials.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The coating uses a composite formulation combining organic resin with inorganic nanoparticles and hydrophobic additives, creating a multi-functional protective layer that provides both mechanical strength and chemical stability, preventing ceramic proppant degradation in harsh downhole environments.

Inventive Principle:
Principle #40Composite materials

3Strength

If proppant coating is applied to increase surface area, then crush stress distribution improves, but coating degradation occurs in wet conditions

Engineering Contradiction:
Improvecrush resistanceVSAvoidcoating durability
Core Design Contradiction:
StrengthVSReliability

Solution Approach 1:

The coating system employs a composite structure with organic resin matrix, inorganic strengthening nanoparticles (alumina, silica, titania), and hydrophobic additives. This composite formulation provides both the mechanical strength needed for crush resistance and the chemical stability required for durability in wet and hot downhole conditions.

Inventive Principle:
Principle #40Composite materials

Solution Approach 2:

The inclusion of hydrophobic additives (fluorinated compounds, silicones, waxes) fundamentally changes the coating's chemical parameters, providing water resistance and chemical stability that prevent coating degradation in wet downhole conditions while maintaining the protective function of the coating.

Inventive Principle:
Principle #35Parameter changes

4Ease of manufacture

If conventional proppants are used, then manufacturing is simple and cost-effective, but fines migration occurs due to particle crushing

Engineering Contradiction:
Improvemanufacturing simplicityVSAvoidfines migration
Core Design Contradiction:
Ease of manufactureVSObject-generated harmful factors

Solution Approach 1:

The patent applies a composite coating material system on conventional sand proppants that significantly enhances particle strength and prevents crushing. This eliminates fines generation and migration while maintaining the manufacturing simplicity and cost-effectiveness of using sand as the base proppant material, as the coating is applied through established coating processes.

Inventive Principle:
Principle #40Composite materials

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The nanoparticle-coated proppants improve crush resistance, prevent fines migration, and maintain hydraulic conductivity, leading to increased hydrocarbon production and reduced condensate banking by resisting chemical and thermal degradation.

Implementation Method 1

The functionalized nanoparticles in the proppant coating impart hydrophobicity, oleophobicity, or omniphobicity to the proppants

Methodology Applied
Scientific EffectHydrophobic effect: Hydrophobe

Implementation Method 2

The functionalized nanoparticles in the proppant coating impart hydrophobicity, oleophobicity, or omniphobicity to the proppants

Methodology Applied
Scientific EffectOleophobic effect: Hydrophobe

Implementation Method 3

The dispersion of strengthening agents enhances the mechanical strength of the coating materials

Methodology Applied
Scientific EffectComposite materials strengthening: Composite Materials

Implementation Method 4

The proppant coating increases the surface area of the particle; therefore, the crush stress is distributed over a larger area of the coated proppant particle

Methodology Applied
Scientific EffectStress distribution:

Data Source

PatentEP4017935B1Nanoparticle coated proppants and methods of making and use thereof
Publication Date: 2023.08.30 SAUDI ARABIAN OIL CO
  • EP4017935B1 patent drawingFigure 1
  • EP4017935B1 patent drawingFigure 2A~2B
  • EP4017935B1 patent drawingFigure 3

AI summary

Methods for producing proppant with nanoparticle proppant coating are provided. The methods include coating the proppant particles with a strengthening agent, functionalized nanoparticles, and unfunctionalized organic resin to produce proppant with nanoparticle proppant coating. Additionally, a proppant comprising a proppant particle and a nanoparticle proppant coating is provided. The nanoparticle proppant coating includes a strengthening agent, functionalized nanoparticles, and unfunctionalized organic resin. The nanoparticle proppant coating coats the proppant particle. Additionally, a method for increasing a rate of hydrocarbon production from a subsurface formation through the use of the proppant is provided.