One-Pot Nanoparticle Polymer Synthesis for Rubber

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Solution Overview

Problem

Existing methods for synthesizing nanoparticles and liquid polymers for rubber compositions involve separate synthesis and processing, which are inefficient due to the high viscosity of liquid polymers and require significant inventory space, making it difficult to integrate them effectively into rubber compositions.

Innovation Solution

A one-pot synthesis method where nanoparticles and liquid polymers are synthesized together in a single reaction vessel, allowing for easier processing and dispersion within rubber compositions, reducing inventory space requirements.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Manufacturing precision

If nanoparticles and liquid polymer are synthesized separately, then each component can be produced with controlled properties, but the processing difficulty increases due to high viscosity of liquid polymer and significant inventory space is required

Engineering Contradiction:
Improvecontrolled properties of nanoparticles and liquid polymerVSAvoidprocessing difficulty
Core Design Contradiction:
Manufacturing precisionVSEase of manufacture

Solution Approach 1:

The patent combines the synthesis of nanoparticles and liquid polymer into a single polymerization reaction system. The liquid polymer serves as both the continuous phase and the matrix for nanoparticle formation, eliminating the need for separate synthesis, drying, and blending steps. This merging of processes directly addresses the processing difficulty while maintaining property control through sequential monomer addition and reaction condition optimization.

Inventive Principle:
Principle #5Merging (Combining)

2Manufacturing precision

If liquid polymer is synthesized separately, then its polymerization can be controlled, but the drying process becomes extremely difficult due to high viscosity

Engineering Contradiction:
Improvepolymerization controlVSAvoiddrying difficulty
Core Design Contradiction:
Manufacturing precisionVSEase of manufacture

Solution Approach 1:

The patent merges the liquid polymer synthesis with nanoparticle formation in a single reaction system. The liquid polymer remains in the reaction medium throughout the process, eliminating the need for separate drying. The nanoparticle formation occurs within the liquid polymer matrix, and the final product is obtained directly after a single filtration step, bypassing the drying difficulty entirely.

Inventive Principle:
Principle #5Merging (Combining)

3Manufacturing precision

If nanoparticles and liquid polymer are stored separately, then each component can be optimized independently, but valuable inventory space is consumed

Engineering Contradiction:
Improveindependent optimizationVSAvoidinventory space
Core Design Contradiction:
Manufacturing precisionVSVolume of stationary object

Solution Approach 1:

The patent produces nanoparticles and liquid polymer as a single integrated product system in one reaction vessel. The resulting composition contains both components in the desired ratios, already mixed and ready for use. This eliminates the need for separate storage of nanoparticles and liquid polymer, significantly reducing inventory space while maintaining the ability to optimize properties through controlled reaction parameters and monomer feed rates.

Inventive Principle:
Principle #5Merging (Combining)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The one-pot synthesis method results in a blend that is easier to process and dry, saving space and improving the integration of nanoparticles and liquid polymers into rubber compositions, enhancing properties like traction and durability of tire treads while reducing the need for processing oils.

Implementation Method 1

polymerizing a first monomer and optionally a second monomer in a hydrocarbon solvent to form the liquid polymer

Methodology Applied
Scientific EffectPolymerization: Chemical Bonding

Implementation Method 2

The polymerization is partially quenched or terminated with a quenching agent

Methodology Applied
Scientific EffectChemical reaction: Chemical Bonding

Implementation Method 3

a core including the multiple-vinyl aromatic monomer, and a shell including the first monomer or the first monomer and the second monomer

Methodology Applied
Scientific EffectCross-linking: Chemical Bonding

Data Source

PatentEP2167557B1One-pot synthesis of nanoparticles and liquid polymer for rubber applications
Publication Date: 2015.01.07 BRIDGESTONE CORP
  • EP2167557B1 patent drawingFigure 1
  • EP2167557B1 patent drawingFigure 2
  • EP2167557B1 patent drawing

AI summary

A method for performing a one-pot synthesis of a blend of nanoparticles and liquid polymer includes polymerizing a first monomer and optionally a second monomer in a hydrocarbon solvent to form the liquid polymer. The polymerization is terminated before completion with a quenching agent. Then a charge of polymerization initiator, and a mixture of cross-linking agent and mono- vinyl aromatic monomer are added. This causes further polymerization whereby nanoparticles are formed having a core including the cross-linking agent, and a shell including the first monomer or the first monomer and the second monomer. Nanoparticle/liquid polymer blends resulting from the method and rubber compositions incorporating the blends are also disclosed.