Nanoparticulate Compressed Tablets for Microanalysis

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Solution Overview

Problem

Existing methods lack homogeneous standard reference materials (SRM) with properties similar to unknown samples for microanalysis, particularly for trace and ultra-trace elements, and existing press tablets are too coarse-grained and often contain binders, making them unsuitable for high-resolution microanalysis.

Innovation Solution

A process involving wet grinding and high-pressure pressing of analysis-ground powders with grain sizes <75 µm, forming nanoparticles without binders, and using a 'top-down' approach to create stable tablets with sizes between 30-150 nm, ensuring homogeneity and smooth surfaces.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Manufacturing precision

If conventional powder pressing methods are used, then tablets can be produced with sufficient mechanical stability, but the particle size remains too coarse (10-100 μm) for high-resolution microanalysis

Engineering Contradiction:
Improveparticle sizeVSAvoidmicroanalysis resolution
Core Design Contradiction:
Manufacturing precisionVSMeasurement precision

Solution Approach 1:

The patent applies parameter changes by reducing the particle size parameter from conventional 10-100 μm to nanoscale 30-150 nm through intensive ball milling processes. This dramatic parameter change enables the tablets to be suitable for high-resolution microanalysis while maintaining mechanical stability through the novel pressing methodology.

Inventive Principle:
Principle #35Parameter changes

2Strength

If binders are added to ensure tablet stability, then mechanical strength is improved, but material homogeneity and purity are compromised

Engineering Contradiction:
Improvetablet stabilityVSAvoidmaterial homogeneity
Core Design Contradiction:
StrengthVSStability of the object's composition

Solution Approach 1:

The patent applies the taking out principle by completely eliminating binders from the tablet formulation. Instead of adding external binding agents, the method achieves tablet stability through the inherent properties of nanoscale particles and optimized pressing parameters, thereby maintaining complete material homogeneity and purity without contamination.

Inventive Principle:
Principle #2Taking out (Extraction)

Solution Approach 2:

The nanoscale powder particles serve their own binding function through enhanced cohesive forces at the nanoscale. The intensive ball milling process creates particles with high surface energy that naturally adhere to each other during pressing, eliminating the need for external binders while maintaining tablet integrity.

Inventive Principle:
Principle #25Self-service

3Adaptability or versatility

If natural materials are used as reference materials, then material diversity is improved, but homogeneity at the micrometer scale is extremely rare or difficult to achieve

Engineering Contradiction:
Improvematerial diversityVSAvoidhomogeneity
Core Design Contradiction:
Adaptability or versatilityVSStability of the object's composition

Solution Approach 1:

The patent applies parameter changes by transforming the particle size parameter from micrometer to nanoscale dimensions through intensive ball milling. This parameter transformation creates homogeneous nanoscale structures from diverse natural materials, enabling micrometer-scale homogeneity that is extremely rare in natural materials while preserving material diversity for various analytical applications.

Inventive Principle:
Principle #35Parameter changes

4Stability of the object's composition

If synthetic glasses are produced, then material homogeneity is improved, but production difficulty and material limitations increase

Engineering Contradiction:
ImprovehomogeneityVSAvoidproduction difficulty
Core Design Contradiction:
Stability of the object's compositionVSEase of manufacture

Solution Approach 1:

The patent applies mechanics substitution by replacing the complex thermal melting and glass-forming processes with a purely mechanical ball milling approach followed by low-temperature pressing. This substitution eliminates the need for high-temperature melting, volatile loss, and strict material compatibility constraints, significantly easing production while achieving comparable or superior homogeneity.

Inventive Principle:
Principle #28Mechanics substitution (Replace mechanical system)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The process produces ultra-homogeneous tablets suitable for high-resolution microanalysis, suitable as certified SRM, enabling accurate element and isotope composition measurements without binder dilution or material change, and suitable for various microanalysis methods.

Implementation Method 1

a) grinding in a ball mill

Methodology Applied
Scientific EffectMechanical impact and friction: Abrasion

Implementation Method 2

b) freeze-drying

Methodology Applied
Scientific EffectFreeze drying: Freeze Drying

Implementation Method 3

c) pressing of the nanopowder, particularly with sapphire discs, in a preferably programmable high-pressure press

Methodology Applied
Scientific EffectHigh-pressure compression: Compression

Data Source

PatentEP3635362B1Production of nanoparticulate compressed tablets/pellets, compressed tablets/pellets produced by the process and use thereof
Publication Date: 2025.04.30 UNIVERSITY OF KIEL
  • EP3635362B1 patent drawingFigure 1~2

AI summary

The invention relates to a method for producing nanoparticulate compressed tablets/pellets from synthetic and/or natural materials. The invention also relates to compressed tablets/pellets produced using a method for producing nanoparticulate compressed tablets/pellets from synthetic and/or natural materials and to uses thereof.