Biosensor Reagent Composition Using Naphthol Green B

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Solution Overview

Problem

Existing biosensors face challenges in achieving high sensitivity and minimizing blood sample volume for glucose measurement, particularly in miniaturized formats, which affects user convenience and accuracy.

Innovation Solution

A reagent composition for biosensors incorporating Naphthol Green B and a ruthenium complex, along with an enzyme, is used to enhance electron transfer efficiency, including surfactants and water-soluble polymers to stabilize the enzyme and improve reaction efficiency on the electrode surface.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Quantity of substance

If the biosensor is miniaturized to reduce blood sample volume, then the amount of blood needed for measurement is reduced, but the detection sensitivity and analysis linearity deteriorate

Engineering Contradiction:
Improveblood sample volumeVSAvoiddetection sensitivity
Core Design Contradiction:
Quantity of substanceVSMeasurement precision

Solution Approach 1:

The patent uses a composite reagent system combining Naphthol Green B (a redox mediator) with ruthenium complexes and enzymes. This composite material approach enhances electron transfer efficiency and catalytic activity, enabling high sensitivity detection even in miniaturized biosensors with limited sample volumes. The synergistic interaction between multiple components compensates for the reduced reaction volume.

Inventive Principle:
Principle #40Composite materials

Solution Approach 2:

The patent optimizes the concentration ratios and physical-chemical parameters of the reagent components. By adjusting the concentration of Naphthol Green B relative to the enzyme and ruthenium complex, the system achieves maximum electron transfer efficiency. This parameter optimization enables the biosensor to maintain high detection sensitivity with minimal blood sample volume (0.3-2 μL).

Inventive Principle:
Principle #35Parameter changes

2Measurement precision

If the concentration of electron transfer mediator is increased to improve electron transfer efficiency, then the detection sensitivity improves, but the cost and complexity of the reagent composition increases

Engineering Contradiction:
Improvedetection sensitivityVSAvoidreagent composition complexity
Core Design Contradiction:
Measurement precisionVSDevice complexity

Solution Approach 1:

The patent employs Naphthol Green B as an intermediary redox mediator that facilitates electron transfer between the enzyme's active site and the electrode. This mediator acts as a bridge, enabling efficient electron transfer at low concentrations. The intermediary approach avoids the need for high concentrations of direct electron acceptors, simplifying the reagent composition while maintaining high detection sensitivity.

Inventive Principle:
Principle #24Intermediary (Mediator)

Solution Approach 2:

The patent replaces complex multi-component enzyme systems with a streamlined reagent composition centered on Naphthol Green B as the primary electron transfer mediator. This substitution simplifies the reagent formulation while achieving comparable or superior electron transfer efficiency through the unique redox properties of Naphthol Green B in combination with ruthenium complexes.

Inventive Principle:
Principle #28Mechanics substitution (Replace mechanical system)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The composition significantly increases glucose detection performance, improves analysis linearity, and reduces the amount of blood needed for measurement, making it suitable for frequent and accurate glucose monitoring.

Implementation Method 1

the reduced FADH 2 is oxidized to FAD through an oxidation-reduction reaction with the electron transfer mediator, and the electron transfer mediator is reduced. Electrons generated from the electron transfer mediator in a reduction state formed in this manner disperse to an electrode surface

Methodology Applied
Scientific EffectOxidation-reduction reaction: Redox Reactions

Implementation Method 2

the blood glucose is oxidized to gluconate due to a catalytic action of a glucose oxidase. At this time, FAD, which is an active site of the glucose oxidase, is reduced and became FADH 2

Methodology Applied
Scientific EffectCatalysis: Catalysis

Data Source

PatentEP3272874B1Reagent composition for biosensor and biosensor having the same
Publication Date: 2019.11.27 OSANG HEALTHCARE CO LTD
  • EP3272874B1 patent drawingFigure 1
  • EP3272874B1 patent drawingFigure 2
  • EP3272874B1 patent drawingFigure 3

AI summary

This invention discloses a reagent composition for a biosensor having high sensitivity which is capable of improving analysis linearity of an analyte such as glucose by reacting an oxidoreductase, a metal-containing complex, and Naphthol Green B, and minimizing blood necessary for measuring blood glucose since it is possible to detect a concentration of a small amount of the analyte, and a biosensor having the same. The reagent composition for a biosensor includes at least two kinds of electron transfer mediators including Naphthol Green B, and an enzyme.