NdFeB Magnet Coating via Chemical Vapor Deposition

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Solution Overview

Problem

Current methods for enhancing the coercive force and reducing the usage of heavy rare earth elements in neodymium-iron-boron (NdFeB) permanent magnetic materials are inefficient, as they either require large amounts of heavy rare earth elements or result in uneven distribution and performance degradation due to segregation of added elements like W, Mo, V, Ti, Ta, Zr, Nb, Co, Cr, Ga.

Innovation Solution

Uniform dispersion of high-melting particles such as CoZr at grain boundaries in the NdFeB magnet using physical vapor deposition, which reduces the need for heavy rare earth elements and improves coercive force, crystal grain refinement, and magnetic properties.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Strength

If heavy rare earth elements (Dy, Tb) are added to improve coercive force and high temperature usability, then magnetic performance is improved, but the usage amount of heavy rare earth elements increases and manufacturing cost increases

Engineering Contradiction:
Improvecoercive forceVSAvoidusage amount of heavy rare earth elements
Core Design Contradiction:
StrengthVSQuantity of substance

Solution Approach 1:

The patent changes the chemical composition parameters by replacing heavy rare earth elements with a specific ratio of Co (0.1-5 wt%) and Zr (0.1-5 wt%) elements. This parameter substitution maintains the coercive force improvement while reducing heavy rare earth content, directly resolving the contradiction between magnetic performance and material quantity usage

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent creates a composite grain boundary phase containing Co and Zr elements that work synergistically. The Co provides magnetic properties while Zr provides structural stability, together achieving the coercive force enhancement normally requiring heavy rare earths, thus reducing heavy rare earth usage while maintaining performance

Inventive Principle:
Principle #40Composite materials

2Shape

If elements (W, Mo, V, Ti, Ta, Zr, Nb, Co, Cr, Ga) are added to refine crystal grains, then grain growth is suppressed, but the elements distribute unevenly causing segregation and performance degradation

Engineering Contradiction:
Improvecrystal grain sizeVSAvoiduniformity of element distribution
Core Design Contradiction:
ShapeVSStability of the object's composition

Solution Approach 1:

The patent concentrates Co and Zr elements specifically at the grain boundaries rather than uniform distribution throughout the bulk material. This localized placement achieves grain refinement at the critical grain boundary regions without causing widespread segregation, resolving the contradiction between grain size control and compositional uniformity

Inventive Principle:
Principle #3Local quality

Solution Approach 2:

The patent optimizes the concentration parameters of Co (0.1-5 wt%) and Zr (0.1-5 wt%) to achieve sufficient grain boundary coverage and refinement effect at low concentrations, preventing the segregation issues that occur with higher concentrations of other refining elements

Inventive Principle:
Principle #35Parameter changes

3Manufacturing precision

If magnetron sputtering is used to coat NdFeB powder, then physical vapor deposition is achieved, but the material utilization rate is less than 50%

Engineering Contradiction:
Improvecoating uniformityVSAvoidmaterial utilization rate
Core Design Contradiction:
Manufacturing precisionVSLoss of substance

Solution Approach 1:

The patent replaces the magnetron sputtering physical vapor deposition method with a chemical vapor deposition method using organic metal compounds. This substitution changes the deposition mechanism from physical ejection to chemical decomposition, achieving uniform coating with significantly reduced material loss and improved utilization rate

Inventive Principle:
Principle #28Mechanics substitution (Replace mechanical system)

4Manufacturing precision

If electron beam evaporation is used to coat NdFeB powder, then physical vapor deposition is achieved, but the equipment cost is expensive and high vacuum and high evaporation temperature are required

Engineering Contradiction:
Improvecoating qualityVSAvoidequipment requirements
Core Design Contradiction:
Manufacturing precisionVSDevice complexity

Solution Approach 1:

The patent replaces electron beam evaporation with chemical vapor deposition using organic metal compounds. This substitution eliminates the need for complex electron beam generation equipment, high vacuum systems, and high temperature evaporation apparatus, achieving coating with simpler, more cost-effective equipment while maintaining coating quality

Inventive Principle:
Principle #28Mechanics substitution (Replace mechanical system)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

Significantly increases coercive force, refines crystal grains, reduces heavy rare earth element usage, and decreases manufacturing costs while maintaining excellent magnetic properties and reducing oxygen content in the NdFeB magnet.

Implementation Method 1

the physical vapor deposition method comprises magnetron sputtering, electron beam evaporation, and vacuum induction evaporation

Methodology Applied
Scientific EffectPhysical vapor deposition: Physical Vapour Deposition

Implementation Method 2

The physical vapor deposition method comprises magnetron sputtering, electron beam evaporation, and vacuum induction evaporation

Methodology Applied
Scientific EffectMagnetron sputtering: Sputtering

Data Source

PatentEP3547333B1Method for preparing neodymium-iron-boron permanent magnetic material
Publication Date: 2022.05.18 NAT ENG RES CENT OF RARE EARTH METALLURGY & FUNCTION MATERIALS

AI summary

Disclosed is a method for preparing a NdFeB permanent magnetic material. The method comprises: preparing a NdFeB magnetic material, depositing heavy rare earth particles or high-melting particles on NdFeB magnetic powder by means of a physical vapor deposition process; orientation molding and then sintering to obtain a NdFeB magnet. By the present invention, the heavy rare earth particles or high-melting particles are dispersed evenly within the magnet at the grain boundary, with coercive force of the magnet being increased and the amount of heavy rare earth used being reduced, so that the coercive force of the NdFeB magnet is significantly increased.