Nd-S-CoSb3 Skutterudite Thermoelectric Material

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Solution Overview

Problem

Existing compound semiconductors fail to simultaneously achieve high thermoelectric conversion efficiency, long-term electrical and optical stability, and cost-effectiveness for use in thermoelectric conversion elements and solar batteries.

Innovation Solution

A novel compound semiconductor represented by Chemical Formula NdxSyCo4Sb12-zQz, where Q is O, Se, or Te, is synthesized, optimizing carrier concentration and lattice thermal conductivity through controlled mole ratios of neodymium, sulfur, and selenium/tellurium, enhancing Seebeck coefficient and electrical conductivity while reducing thermal conductivity.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Loss of energy

If existing compound semiconductors are used for thermoelectric conversion elements, then manufacturing cost is reduced, but thermoelectric conversion efficiency is insufficient

Engineering Contradiction:
Improvethermoelectric conversion efficiencyVSAvoidmanufacturing cost
Core Design Contradiction:
Loss of energyVSEase of manufacture

Solution Approach 1:

The patent changes the chemical composition parameters by incorporating rare earth elements (Nd, Sm, Gd, Dy, Er) and adjusting the stoichiometric ratios of Co, Sb, and Q elements to optimize thermoelectric performance while maintaining cost-effectiveness

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent creates a composite compound semiconductor structure with formula NdxSyCo4-zSb12-yQz where multiple elements are combined to achieve synergistic effects that improve thermoelectric conversion efficiency

Inventive Principle:
Principle #40Composite materials

2Reliability

If existing compound semiconductors are used for solar batteries, then manufacturing cost is reduced, but long-term electrical and optical stability is insufficient

Engineering Contradiction:
Improvelong-term electrical and optical stabilityVSAvoidmanufacturing cost
Core Design Contradiction:
ReliabilityVSEase of manufacture

Solution Approach 1:

The patent optimizes the compositional parameters including the ratios of Nd to CoSb3 base structure and the amount of Q elements to enhance electrical and optical stability for solar battery applications

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent develops a composite material system combining rare earth elements with CoSb3 skutterudite structure to achieve both stability and cost-effectiveness for commercial solar battery use

Inventive Principle:
Principle #40Composite materials

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The compound semiconductor exhibits improved thermoelectric performance with high ZT figure of merit, durability at high temperatures, and reduced manufacturing costs, making it suitable for thermoelectric conversion elements and solar batteries.

Implementation Method 1

the thermoelectric generation is the form of power generation that converts heat energy into electrical energy using thermoelectromotive force generated by causing a temperature difference in a thermoelectric conversion element

Methodology Applied
Scientific EffectSeebeck effect: Seebeck Effect

Implementation Method 2

the compound semiconductor solar battery uses a compound semiconductor in a photo-absorbing layer that absorbs sunlight to form an electron-hole pair

Methodology Applied
Scientific EffectPhotoelectric effect: Photoelectric Effect

Data Source

PatentUS11127891B2Compound semiconductor and use thereof
Publication Date: 2021.09.21 LG CHEM LTD

AI summary

A novel compound semiconductor that can be used for a solar battery, a thermoelectric material, and the like, and use thereof. The novel compound semiconductor may be represented by the following Chemical Formula: NdxSyCo4Sb12-zQz, wherein Q is one or more selected from the O, Se, or Te, 0<x<0.2, 0<y≤1, and 0<z<12.