Triple-mode Neutron Detector Using Organic-Inorganic Scintillator Composite

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Solution Overview

Problem

Current neutron detection technologies fail to simultaneously detect thermal and fast neutrons and perform gamma spectroscopy effectively, with existing materials either lacking in sensitivity, stability, or being too expensive, and none efficiently combine neutron detection with gamma discrimination and spectroscopy capabilities.

Innovation Solution

A detector comprising an organic scintillator in combination with an inorganic scintillator containing neutron capture isotopes like 6Li or 10B, where the scintillators are read out separately by photodetectors to achieve simultaneous thermal/fast neutron detection and gamma ray discrimination with gamma spectroscopy, leveraging the high concentration of hydrogen in organic scintillators for fast neutron detection and the high cross-section of inorganic scintillators for neutron capture and gamma absorption.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If Li-containing plastic scintillators are used for slow neutron detection, then slow neutron detection capability is improved, but light yield is degraded and stability over time is poor

Engineering Contradiction:
Improveslow neutron detection capabilityVSAvoidstability of Li inside polymer
Core Design Contradiction:
ReliabilityVSStability of the object's composition

Solution Approach 1:

The patent uses a composite material consisting of lithium fluoride (LiF) crystals embedded in an organic scintillator matrix. This composite structure combines the high neutron capture cross-section of 6Li from LiF with the excellent scintillation properties and stability of the organic matrix, resolving the contradiction between slow neutron detection capability and long-term stability.

Inventive Principle:
Principle #40Composite materials

Solution Approach 2:

The patent employs commercially available LiF crystals rather than experimentally developed Li-doped plastics with uncertain longevity. This approach trades the potential for optimized scintillation properties against proven stability and availability, ensuring reliable long-term operation.

Inventive Principle:
Principle #27Cheap short-living objects (Disposable)

2Reliability

If B-doped plastic scintillators are used for thermal neutron detection, then neutron capture cross-section is improved, but cost increases significantly and gamma ray interference worsens

Engineering Contradiction:
Improvethermal neutron detection capabilityVSAvoidcost of detector material
Core Design Contradiction:
ReliabilityVSEase of manufacture

Solution Approach 1:

The patent replaces expensive boron-doped plastics with commercially available lithium fluoride crystals, dramatically reducing material cost while maintaining thermal neutron detection capability through the high cross-section of 6Li.

Inventive Principle:
Principle #27Cheap short-living objects (Disposable)

Solution Approach 2:

The patent extracts the neutron capture function into a separate component (LiF crystal) with optimized properties, leaving the organic scintillator matrix to handle gamma ray discrimination and fast neutron detection, thereby avoiding the gamma interference problem of boron-doped plastics.

Inventive Principle:
Principle #2Taking out (Extraction)

3Measurement precision

If fast plastic scintillators are used for fast neutron/gamma discrimination, then discrimination capability is improved, but gamma spectroscopy capability is lost

Engineering Contradiction:
Improvefast neutron/gamma discriminationVSAvoidgamma spectroscopy capability
Core Design Contradiction:
Measurement precisionVSAdaptability or versatility

Solution Approach 1:

The patent creates a multi-functional detector where the organic scintillator performs both fast neutron/gamma discrimination through pulse shape discrimination and gamma spectroscopy through Compton scattering, while the LiF crystal adds thermal neutron detection capability. This universal design resolves the contradiction by making the system adaptable to multiple detection modes.

Inventive Principle:
Principle #6Universality (Multi-functionality)

4Reliability

If ZnS phosphor detectors are used for fast neutron detection, then neutron detection efficiency is improved, but gamma rejection capability worsens

Engineering Contradiction:
Improvefast neutron detection efficiencyVSAvoidgamma rejection capability
Core Design Contradiction:
ReliabilityVSMeasurement precision

Solution Approach 1:

The patent extracts the gamma rejection function from the neutron detection process by using pulse shape discrimination in the organic scintillator, allowing the LiF crystal to focus solely on enhancing neutron detection efficiency without compromising gamma rejection capability.

Inventive Principle:
Principle #2Taking out (Extraction)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The solution enables efficient detection of fast and slow neutrons while performing gamma ray spectroscopy, offering improved sensitivity and stability, and cost-effectiveness by combining the strengths of organic and inorganic scintillators, effectively addressing the limitations of existing technologies.

Implementation Method 1

The high concentration of hydrogen renders neutron scattering on protons highly probable

Methodology Applied
Scientific EffectProton recoil scattering: Scattering

Implementation Method 2

Some organic scintillators also exhibit different scintillation pulse behavior for different types of incident radiation

Methodology Applied
Scientific EffectScintillation: Scintillation

Implementation Method 3

Detection of these low-energy neutrons is achieved by materials containing isotopes (notably 3He, 6Li and 10B) having high cross-sections for neutron capture

Methodology Applied
Scientific EffectNeutron capture: Nuclear Fission

Implementation Method 4

The addition of Bi increases remarkably the probability of photoelectric effect in the plastic scintillator

Methodology Applied
Scientific EffectPhotoelectric effect: Photoelectric Effect

Implementation Method 5

due to their very low effective atomic number (Zeff) these materials cannot be used for gamma spectroscopy, because the vast majority of the interactions of high-energy photons occurs by Compton scattering

Methodology Applied
Scientific EffectCompton scattering: Compton Scattering

Data Source

PatentUS11841471B2Triple-mode detector for fast neutrons, slow neutrons, and gamma ray spectroscopy
Publication Date: 2023.12.12 RGT UNIV OF CALIFORNIA
  • US11841471B2 patent drawing
  • US11841471B2 patent drawing
  • US11841471B2 patent drawing

AI summary

This disclosure provides systems, methods, and apparatus related to neutron detection and gamma ray detection. In one aspect, a detector comprises a scintillator structure that comprises an organic scintillator and an inorganic scintillator. The organic scintillator is in the form of one or more elements of a specified length. The inorganic scintillator is in the form of one or more elements of the specified length. First ends of the one or more organic scintillator elements and first ends of the one or more inorganic scintillator elements define a first surface. Second ends of the one or more organic scintillator elements and second ends of the one or more inorganic scintillator elements define a second surface.