NEXAFS Polymer Surface Analysis via Thin Metal Coating

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Solution Overview

Problem

Conventional methods struggle to accurately analyze the surface deterioration of polymer materials, particularly those with low conductivity, such as tire rubber compositions with reduced carbon black content, using NEXAFS measurements.

Innovation Solution

A deterioration analysis method involving a metal coating with a thickness of 100 Å or less is applied to the polymer material, allowing irradiation with high intensity monochromatic X-rays and electron yield measurement to analyze X-ray absorption, ensuring conductivity and detailed surface analysis.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Loss of energy

If a polymer material with low carbon black content is measured by NEXAFS, then fuel efficiency is improved, but electrical conductivity deteriorates making measurement difficult

Engineering Contradiction:
Improvefuel efficiencyVSAvoidelectrical conductivity
Core Design Contradiction:
Loss of energyVSReliability

Solution Approach 1:

A metal coating layer is introduced as an intermediary between the polymer material and the measurement system. This coating layer serves as a mediator that provides the necessary electrical conductivity for NEXAFS measurement without altering the underlying polymer structure or requiring changes to the fuel-efficient low carbon black formulation.

Inventive Principle:
Principle #24Intermediary (Mediator)

Solution Approach 2:

The electrical conductivity parameter of the sample is changed by adding a metal coating layer. This allows the measurement process to be performed on samples that would otherwise be non-conductive, enabling analysis of fuel-efficient rubber formulations with reduced carbon black content.

Inventive Principle:
Principle #35Parameter changes

2Measurement precision

If the sample is cut with a microtome to achieve thin sections, then measurement precision is improved, but the outermost surface cannot be accessed and orientation becomes uncertain

Engineering Contradiction:
ImproveS/B and S/N ratiosVSAvoidsurface accessibility and orientation
Core Design Contradiction:
Measurement precisionVSEase of operation

Solution Approach 1:

The metal coating is applied preliminarily to the outermost surface of the polymer material before any cutting or sectioning operations. This preliminary action preserves the surface integrity and provides a permanent marker that identifies the original outer surface, enabling subsequent cutting to proceed while maintaining surface orientation information.

Inventive Principle:
Principle #10Preliminary action

Solution Approach 2:

The metal coating provides a visual distinction (color/reflectivity change) that marks the outermost surface. This visual marker allows operators to easily identify and preserve the surface orientation during sample preparation, solving the orientation uncertainty problem without affecting measurement precision.

Inventive Principle:
Principle #32Color changes

3Ease of manufacture

If a thick sample is measured, then sample preparation is simplified, but measurement accuracy deteriorates due to insufficient conductivity

Engineering Contradiction:
Improvesample preparationVSAvoidmeasurement accuracy
Core Design Contradiction:
Ease of manufactureVSMeasurement precision

Solution Approach 1:

The metal coating acts as an intermediary conductive layer that enables accurate NEXAFS measurement of thick samples. By providing a continuous conductive path across the sample surface, the coating allows measurement of thicker sections without requiring complex thin sectioning procedures.

Inventive Principle:
Principle #24Intermediary (Mediator)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This method enables detailed analysis of polymer material deterioration, including surface condition evaluation, deterioration degree, and contribution rates of oxygen and ozone deterioration, even in samples with low carbon black content, by ensuring conductivity and minimizing the metal coating's impact.

Implementation Method 1

irradiating a polymer material with high intensity X-rays, and measuring X-ray absorption while varying the energy of the X-rays

Methodology Applied
Scientific EffectX-ray absorption: Absorption (EM radiation)

Implementation Method 2

the sample generally needs to be an electrically conductive material... ensures that even a relatively thick sample, such as having a thickness of about 1 mm, has conductivity

Methodology Applied
Scientific EffectElectrical conduction: Conduction (electrical)

Data Source

PatentEP2966437B1Deterioration analysis method
Publication Date: 2017.12.13 SUMITOMO RUBBER INDUSTRIES LTD
  • EP2966437B1 patent drawingFigure 1-1~1-2
  • EP2966437B1 patent drawingFigure 1-3~1-4
  • EP2966437B1 patent drawingFigure 1-5~1-6

AI summary

The present invention provides a deterioration analysis method capable of analyzing in detail deterioration of a polymer material, and in particular deterioration in the surface condition of a polymer material with low conductivity. The present invention relates to a deterioration analysis method including irradiating a polymer material with a metal coating having a thickness of 100 Å or less formed thereon, with high intensity X-rays, and measuring X-ray absorption while varying the energy of the X-rays, to analyze deterioration of the polymer.