Ni-Al/SiO2 Hydrogenation Catalyst Precursor for Resin Stability

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Solution Overview

Problem

Current hydrogenation catalysts for petrochemical resins exhibit limited catalytic activity, particularly in thermal and oxidative stability, necessitating the development of a more effective catalyst system for improved performance.

Innovation Solution

A hydrogenation catalyst precursor comprising Ni, Al, and a SiO2 support material, where Ni is supported on the SiO2, exhibiting a specific peak maximum in temperature programmed reduction, achieving high Ni dispersion and enhanced catalytic activity.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If conventional hydrogenation catalysts are used, then the basic hydrogenation function is provided, but the catalytic activity is limited and thermal/oxidative stability is insufficient

Engineering Contradiction:
Improvethermal and oxidative stabilityVSAvoidcatalytic activity
Core Design Contradiction:
ReliabilityVSProductivity

Solution Approach 1:

The patent employs a composite catalyst system combining nickel particles supported on silica-alumina with specific pore structures. The composite nature of the catalyst (Ni/SiO2-Al2O3) provides both high catalytic activity from the nickel component and enhanced thermal/oxidative stability from the stable oxide support structure, resolving the contradiction between activity and stability

Inventive Principle:
Principle #40Composite materials

Solution Approach 2:

The patent utilizes porous silica-alumina support materials with specifically controlled pore volumes (≥0.4 ml/g) and pore size distributions. The porous structure provides high surface area for nickel dispersion (enhancing activity) while the stable oxide framework maintains structural integrity under thermal and oxidative conditions (enhancing stability)

Inventive Principle:
Principle #31Porous materials

2Productivity

If nickel loading is increased to improve catalytic activity, then hydrogenation performance improves, but Ni aggregation occurs reducing effectiveness

Engineering Contradiction:
Improvehydrogenation activityVSAvoidNi dispersion
Core Design Contradiction:
ProductivityVSStability of the object's composition

Solution Approach 1:

The patent creates localized high-surface-area regions on the porous silica-alumina support where nickel particles are dispersed. The specific pore structure creates favorable local environments that prevent nickel aggregation even at high loadings, maintaining both high activity and stable composition through optimized local nickel distribution

Inventive Principle:
Principle #3Local quality

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The catalyst precursor demonstrates improved activity in hydrogenation reactions, with a lower peak maximum in temperature programmed reduction, leading to enhanced stability and performance in petrochemical resin hydrogenation.

Implementation Method 1

the precursor exhibits a specific peak maximum in the temperature programmed reduction

Methodology Applied
Scientific EffectTemperature programmed reduction: Reduction

Implementation Method 2

a hydrogenation is normally performed. As such, the double bonds, the reason for the thermal and oxidative instability, are removed

Methodology Applied
Scientific EffectHydrogenation: Hydrogenation

Implementation Method 3

these usually comprise nickel as the catalytically active component

Methodology Applied
Scientific EffectCatalysis: Catalysis

Implementation Method 4

the Ni is supported on the support material comprising SiO2

Methodology Applied
Scientific EffectAdsorption: Adsorption

Data Source

PatentUS20240238773A1A hydrogenation catalyst and its precursor comprising ni, al, and a support material comprising sio2
Publication Date: 2024.07.18 IQATALYST BV

AI summary

The present invention relates to a specific hydrogenation catalyst and to its precursor. Further, the present invention relates to methods for preparation of the hydrogenation catalyst and its precursor and use thereof. In particular, the specific hydrogenation catalyst and its precursor comprise Ni, Al, and a support material comprising SiO2, wherein the Ni is supported on the support material, and wherein the precursor exhibits a specific peak maximum in the temperature programmed reduction.