Nickel-Iron Battery with Carbon Negative Electrode for High Pulse Currents

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Solution Overview

Problem

Nickel-iron accumulators are not suitable for providing high pulse currents due to their limited ability to handle high currents, and they have stability issues during overcharging, especially at high temperatures.

Innovation Solution

A cell assembly composed of two or more secondary electrochemical cells connected in parallel or series, featuring a carbon-based negative electrode with a high proportion of activated carbon or graphene for pseudocapacitive properties and nickel hydroxide-based positive electrodes, allowing for efficient storage of electrical charge and high pulse current delivery, along with a gas-tight housing to manage overcharging stability.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If traditional nickel-iron accumulator design is used, then reliability and durability are improved, but the ability to deliver high pulse currents deteriorates

Engineering Contradiction:
Improvereliability and durabilityVSAvoidhigh pulse current delivery
Core Design Contradiction:
ReliabilityVSPower

Solution Approach 1:

The negative electrode uses a composite material consisting of iron powder and carbon-based storage material (activated carbon or graphene). This composite structure combines the high capacity and reliability of iron with the high power density and pseudocapacitive properties of carbon, enabling the electrode to deliver both high pulse currents and maintain long-term stability.

Inventive Principle:
Principle #40Composite materials

Solution Approach 2:

The invention changes the compositional parameters of the negative electrode by incorporating carbon-based materials in specific proportions (5-50% by weight of activated carbon or graphene). This parameter modification transforms the electrode's electrochemical behavior, enabling pseudocapacitive charge storage mechanisms that support high current delivery while maintaining the underlying iron-based reliability.

Inventive Principle:
Principle #35Parameter changes

2Device complexity

If traditional nickel-iron accumulator design is used, then simplicity of structure is improved, but stability during overcharging at high temperatures deteriorates

Engineering Contradiction:
Improvestructure simplicityVSAvoidovercharging stability at high temperatures
Core Design Contradiction:
Device complexityVSStability of the object's composition

Solution Approach 1:

The carbon-based storage material in the negative electrode converts the harmful effect of overcharging (oxygen evolution and potential damage) into a beneficial process by consuming the evolved oxygen through oxidation reactions. This transforms the overcharging hazard into a self-regulating mechanism that protects the electrode structure and maintains stability even at high temperatures.

Inventive Principle:
Principle #22Blessing in disguise (Convert harm into benefit)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The cell assembly can deliver high pulse currents quickly while maintaining higher capacity and stability during overcharging, especially at high temperatures, due to the carbon-based storage material's ability to consume oxygen and form an electrical double layer, enhancing the cell's durability and safety.

Implementation Method 1

a carbon-based storage material that enables the storage of electrical charge in the electrode by forming an electrical double layer (Helmholtz double layer)

Methodology Applied
Scientific EffectElectrical double layer formation (Helmholtz double layer): Capacitance

Implementation Method 2

the equilibrium between the oxidized and the metallic form shifts during charging and discharging

Methodology Applied
Scientific EffectRedox reaction: Redox Reactions

Implementation Method 3

the carbon-based storage material in the negative electrode, which can contribute to the consumption of oxygen produced as a result of overcharging

Methodology Applied
Scientific EffectOxidation: Oxidation

Data Source

PatentEP2983236B1Secondary electrochemical element based on nickel/iron
Publication Date: 2017.10.18 VARTA MICROBATTERY GMBH

AI summary

A secondary electrochemical element is described, comprising a negative electrode, a positive electrode, a porous separator that separates the negative and positive electrodes, and an aqueous, alkaline electrolyte with which the electrodes and the separator are impregnated. The negative electrode has a current collector, a carbon-based storage material that enables the storage of electrical charge in the electrode by forming an electrical double layer (Helmholtz double layer), and iron in metallic and/or oxidized form. The positive electrode contains a current collector as well as nickel hydroxide and/or nickel oxyhydroxide. The carbon-based storage material is present in the negative electrode in a proportion of at least 5% by weight.