NiFe Nanosheet Anode for Stable Alkaline Water Electrolysis

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Solution Overview

Problem

Alkaline water electrolysis anodes experience performance deterioration when used with renewable energy sources that have large output fluctuations, leading to instability and reduced catalytic activity over time.

Innovation Solution

The use of a hybrid nickel-iron hydroxide nanosheet (NiFe-ns) as a catalyst component in the anode, dispersed in a common electrolyte supplied to both the anode and cathode chambers, enhances durability and maintains catalytic activity even under fluctuating power conditions.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Stability of the object's composition

If a nickel-based anode is used in alkaline water electrolysis with high-concentration alkali aqueous solution, then the anode stability in the electrolyte is improved, but the catalytic activity deteriorates when electric power with large output fluctuation (such as renewable energy) is used as power source

Engineering Contradiction:
Improveanode stability in electrolyteVSAvoidcatalytic activity under fluctuating power
Core Design Contradiction:
Stability of the object's compositionVSReliability

Solution Approach 1:

The patent uses a composite catalyst layer comprising nickel oxide and iron oxide (or iron hydroxide) on the nickel-based anode. This composite structure combines the electrochemical activity of iron compounds with the stability of nickel, creating a material that maintains catalytic activity under fluctuating power conditions while remaining stable in high-concentration alkali electrolyte.

Inventive Principle:
Principle #40Composite materials

Solution Approach 2:

The patent modifies the chemical composition parameters of the catalyst layer by incorporating iron oxide/ hydroxide in specific ratios (Fe/Ni ratio controlled). This parameter change transforms the surface properties of the nickel-based anode, enabling it to withstand potential fluctuations without significant performance degradation.

Inventive Principle:
Principle #35Parameter changes

2Use of energy by moving object

If the operation temperature is increased to improve electric conductivity of the alkali aqueous solution, then the electric conductivity is improved, but the corrosiveness of the electrolyte increases

Engineering Contradiction:
Improveelectric conductivity of electrolyteVSAvoidcorrosiveness of electrolyte
Core Design Contradiction:
Use of energy by moving objectVSObject-affected harmful factors

Solution Approach 1:

The composite catalyst layer of nickel oxide and iron oxide/hydroxide forms a protective surface structure on the nickel-based anode. This composite material resists corrosion from the high-concentration alkali electrolyte even at elevated temperatures, allowing the system to operate at higher temperatures for improved conductivity without excessive material degradation.

Inventive Principle:
Principle #40Composite materials

3Reliability

If renewable energy is used as power source for alkaline water electrolysis, then the environmental sustainability is improved, but the severe conditions (sudden start/stop and abrupt load fluctuation) cause performance deterioration of the nickel-based anode

Engineering Contradiction:
Improveenvironmental sustainabilityVSAvoidanode service life under fluctuating load
Core Design Contradiction:
ReliabilityVSDuration of action of stationary object

Solution Approach 1:

The nickel-iron composite catalyst layer provides enhanced tolerance to the severe operating conditions caused by renewable energy integration. The iron oxide/hydroxide component stabilizes the nickel surface during frequent start-stop cycles and load fluctuations, extending the anode's service life while maintaining compatibility with sustainable energy sources.

Inventive Principle:
Principle #40Composite materials

Solution Approach 2:

The iron oxide/hydroxide in the composite catalyst layer acts as a protective buffer that anticipates and mitigates the harmful effects of potential fluctuations before they can damage the nickel-based anode structure. This beforehand cushioning effect prevents performance deterioration during abrupt load changes.

Inventive Principle:
Principle #11Beforehand cushioning (Prior cushioning)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This approach stabilizes the catalytic activity of the anode over a long period, ensuring consistent electrolysis performance even with renewable energy sources, and allows for the use of versatile materials in the catalyst layer formation.

Implementation Method 1

alkaline water electrolysis in which the electrolysis performance is unlikely to be deteriorated and which is stable for a long period of time can be performed

Methodology Applied
Scientific EffectElectrolysis: Electrolysis

Implementation Method 2

supplying a common electrolyte having particular constitution to an anode chamber and a cathode chamber that form an electrolytic cell

Methodology Applied
Scientific EffectIon conduction: Conduction (electrical)

Implementation Method 3

A nickel-based material which is stable in a high-concentration alkali aqueous solution is used as an alkaline water electrolysis anode

Methodology Applied
Scientific EffectCatalysis: Catalysis

Data Source

PatentEP4119700B1Alkaline water electrolysis method, and anode for alkaline water electrolysis
Publication Date: 2025.05.21 DE NORA PERMELEC LTD
  • EP4119700B1 patent drawingFigure 1~3
  • EP4119700B1 patent drawingFigure 4(a)~4(c)
  • EP4119700B1 patent drawingFigure 5

AI summary

The present invention realizes industrially excellent effects such that when electric power having a large output fluctuation, such as renewable energy, is used as a power source, electrolysis performance is unlikely to be deteriorated and excellent catalytic activity is retained stably over a longer period of time, and in addition, the present invention provides a technique that enables forming a catalyst layer of an oxygen generation anode, which gives such excellent effects, with a more versatile materials and by a simple electrolysis method. Provided are an alkaline water electrolysis method including supplying an electrolyte obtained by dispersing a catalyst containing a hybrid nickel-iron hydroxide nanosheet (NiFe-ns) being a composite of a metal hydroxide and an organic substance to an anode chamber and a cathode chamber, and using the electrolyte for electrolysis in each chamber in common, an alkaline water electrolysis method including supplying an electrolyte obtained by dispersing a catalyst containing the NiFe-ns to an anode chamber and a cathode chamber, and performing electrolytic deposition of the NiFe-ns in the electrolytic cell during operation to electrolytically deposit the NiFe-ns on a surface of an electrically conductive substrate having a catalyst layer formed on a surface of an oxygen generation anode, thereby recovering and improving electrolysis performance, and an alkaline water electrolysis anode.