Nb-Silicide Composite Microstructure for High-Temperature Strength

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Solution Overview

Problem

Current high-temperature heat-resistant materials, such as nickel-based superalloys, have limitations in achieving higher heatproof temperatures, and niobium-based composites face challenges in balancing high-temperature strength and room temperature toughness, making them unsuitable for next-generation applications.

Innovation Solution

A Nb-silicide based composite with specific atomic percentages of Si, Cr, Ti, Zr, Hf, W, Sn, Mo, and B is developed, combined with a heat treatment process to form a microstructure with niobium crystal grains and niobium silicide phases, enhancing both high-temperature strength and room temperature toughness.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Temperature

If Nb 3 Al intermetallic compound is used to achieve high melting point, then high-temperature strength is improved, but room temperature toughness deteriorates due to brittleness

Engineering Contradiction:
Improveheatproof temperatureVSAvoidroom temperature toughness
Core Design Contradiction:
TemperatureVSStrength

Solution Approach 1:

The patent employs a composite material system consisting of Nb 3 Si intermetallic compound matrix with dispersed precipitates of γ-Nb 5 Si 3 and NbB 2. This composite structure combines the high melting point advantage of intermetallic compounds with improved toughness through the synergistic effect of multiple phases, resolving the contradiction between high-temperature strength and room temperature toughness.

Inventive Principle:
Principle #40Composite materials

Solution Approach 2:

The patent optimizes the composition parameters by controlling Si content at 13-23 at%, B content at 0.20-5.0 at%, and adding ternary elements (Cr: 2.0-10 at%, Ti: 5.0-23 at%, Mo: 3.1-8.0 at%, W: 0.0-2.0 at%, Hf: 1.0-8.0 at%, Sn: 0.10-6.0 at%). These parameter changes transform the material from a brittle intermetallic compound to a composite with balanced mechanical properties at both room and high temperatures.

Inventive Principle:
Principle #35Parameter changes

2Strength

If niobium silicide network structure is formed to improve high-temperature strength, then high-temperature strength is improved, but crack propagation resistance deteriorates due to brittleness

Engineering Contradiction:
Improvehigh-temperature strengthVSAvoidcrack propagation resistance
Core Design Contradiction:
StrengthVSReliability

Solution Approach 1:

The patent creates local quality differentiation by forming discrete precipitates of γ-Nb 5 Si 3 and NbB 2 phases distributed within the Nb 3 Si matrix. Instead of a continuous network structure that facilitates crack propagation, the local precipitate structure provides crack deflection and termination sites, improving reliability while maintaining high-temperature strength through the reinforcing precipitates.

Inventive Principle:
Principle #3Local quality

3Strength

If Ni based superalloy is used to achieve good room temperature toughness, then room temperature toughness is improved, but heatproof temperature increases are limited

Engineering Contradiction:
Improveroom temperature toughnessVSAvoidheatproof temperature
Core Design Contradiction:
StrengthVSTemperature

Solution Approach 1:

The patent fundamentally changes the base material composition from Ni-based superalloy to Nb-based intermetallic compound system. By selecting Nb as the base element and optimizing the alloying composition (Si: 13-23 at%, Cr: 2.0-10 at%, Ti: 5.0-23 at%, Mo: 3.1-8.0 at%, W: 0.0-2.0 at%, Hf: 1.0-8.0 at%, Sn: 0.10-6.0 at%, B: 0.20-5.0 at%), the material achieves both improved room temperature toughness and significantly higher heatproof temperature capability.

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The composite achieves improved mechanical characteristics and toughness at ultrahigh temperatures, making it suitable for high-temperature components and heat engines, particularly in gas turbines and other high-temperature environments.

Implementation Method 1

a heat treatment process to form a microstructure with niobium crystal grains and niobium silicide phases

Methodology Applied
Scientific EffectPhase transformation: Phase Change

Implementation Method 2

niobium silicide precipitation

Methodology Applied
Scientific EffectPrecipitation: Precipitation

Data Source

PatentEP3339458B1Niobium silicide-based composite material, high-temperature component using same, and high-temperature heat engine
Publication Date: 2020.07.08 MITSUBISHI HITACHIPOWER SYST LTD
  • EP3339458B1 patent drawingFigure 1

AI summary

To provide a Nb-silicide based composite achieving both mechanical characteristics and toughness at high levels in an ultrahigh temperature region (1200°C or more) as well as a high-temperature component and a high-temperature heat engine which employ the same. The Nb-silicide based composite according to the present invention includes 13 to 23 at% of Si, 2.0 to 10 at% of Cr, 5.0 to 23 at% of Ti, 0.0 to 6.0 at% of Al, 0.10 to 8.0 at% of Zr, 1.0 to 8.0 at% of Hf, 0.0 to 2.0 at% of W, 0.10 to 6.0 at% of Sn, 3.1 to 8.0 at% of Mo, 0.20 to 5.0 at% of B, and the balance being Nb and inevitable impurities.