Nitrogen Analysis Using Hydrogen Carrier Gas and Catalyst

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Solution Overview

Problem

Existing methods for determining nitrogen content, such as the Dumas method, face challenges with high maintenance and costs due to rapid consumption of reducing agents, requiring frequent replacement and manual intervention, which complicates the analysis process.

Innovation Solution

The method involves adding hydrogen to the measurement gas to reduce oxygen and nitrogen oxide components using a catalyst, with controlled parameters to convert these components into nitrogen and water, avoiding further reduction to ammonia, and using hydrogen as a carrier gas to simplify and cost-effectively maintain the process.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If copper or tungsten is used as reducing agent to convert nitrogen oxides to nitrogen, then nitrogen compounds are converted into nitrogen, but the reducing agent is consumed very quickly and requires frequent replacement, leading to large maintenance effort and high costs

Engineering Contradiction:
Improvecontinuous process operationVSAvoidmaintenance effort
Core Design Contradiction:
ReliabilityVSEase of repair

Solution Approach 1:

The catalyst enables the reducing agent (hydrogen or carbon monoxide) to be continuously regenerated from the reaction products (water or carbon dioxide), creating a self-sustaining system that eliminates the need for frequent manual replacement of consumables and allows continuous operation without interruption

Inventive Principle:
Principle #25Self-service

2Productivity

If copper or tungsten is used as reducing agent, then nitrogen oxides are reduced to nitrogen, but the process requires manual intervention and interruption for agent replacement, increasing complexity and cost

Engineering Contradiction:
Improveanalysis continuityVSAvoidprocess complexity
Core Design Contradiction:
ProductivityVSDevice complexity

Solution Approach 1:

The catalyst automatically regenerates the reducing agent from reaction products, creating a closed-loop system that eliminates manual intervention and maintains continuous operation, thereby simplifying the overall process while improving productivity

Inventive Principle:
Principle #25Self-service

Solution Approach 2:

The catalyst acts as an intermediary substance that facilitates the conversion of nitrogen oxides to nitrogen while simultaneously regenerating the reducing agent from oxidation products, enabling continuous operation without direct human intervention

Inventive Principle:
Principle #24Intermediary (Mediator)

3Productivity

If hydrogen is added to reduce oxygen and nitrogen oxide components, then continuous process flow is enabled, but excess hydrogen must be carefully managed to avoid further reduction to ammonia

Engineering Contradiction:
Improveprocess continuityVSAvoidnitrogen determination accuracy
Core Design Contradiction:
ProductivityVSMeasurement precision

Solution Approach 1:

The catalyst modifies the reaction parameters (temperature, activation energy) to selectively promote nitrogen oxide reduction to nitrogen while suppressing further reduction to ammonia, even in the presence of excess hydrogen, thereby maintaining measurement precision through controlled chemical transformation

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This approach enables a continuous, cost-effective, and reproducible nitrogen determination process with reduced maintenance, allowing for reliable control of gas components and precise nitrogen content measurement, while avoiding unnecessary complexity and expense.

Implementation Method 1

the reduction of the measurement gas takes place on a catalyst

Methodology Applied
Scientific EffectCatalysis: Catalysis

Implementation Method 2

hydrogen is added to the measurement gas to reduce the oxygen and nitrogen oxide components

Methodology Applied
Scientific EffectChemical reduction: Reduction

Implementation Method 3

the oxygen and nitrogen oxide components in the sample gas are converted to water and nitrogen

Methodology Applied
Scientific EffectRedox reactions: Redox Reactions

Implementation Method 4

hydrogen is added to the measurement gas to reduce the oxygen and nitrogen oxide components

Methodology Applied
Scientific EffectChemical reduction: Reduction

Data Source

PatentEP3615929B1Method for determining the nitrogen content in solid or liquid samples
Publication Date: 2023.01.25 TAUNUS INSTR GMBH
  • EP3615929B1 patent drawingFigure 1
  • EP3615929B1 patent drawingFigure 2

AI summary

In a method for determining a nitrogen concentration in solid or liquid samples, hydrogen (5) is used as a carrier gas and for reducing the oxygen and nitrogen oxide components in a combustion gas of the samples (1). After eliminating water (6) and other unwanted gas components (10), the nitrogen concentration in the carrier gas is determined using a thermal conductivity detector (9).