Nitroxide Fluorescent Powder Core-Shell Gradient Oxygen Distribution

Resolve Bottlenecks,
Find Innovative Solutions
Generate Solutions

Solution Overview

Problem

Current nitride red fluorescent powders for LEDs face a trade-off between aging and light decay resistance and luminescent efficiency, with existing solutions either improving one at the expense of the other, lacking a comprehensive solution that enhances both without reducing efficiency.

Innovation Solution

A nitroxide fluorescent powder with a specific inorganic compound structure featuring an increasing oxygen atom content distribution from core to surface, forming distinct zones that enhance chemical and thermal stability, and luminescent efficiency, comprising elements like Ca, Sr, and Eu, with a manufacturing method involving high-temperature calcination and post-treatment to create a stable and efficient luminescent device.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If oxygen content is increased to improve chemical stability and aging resistance, then durability is improved, but luminescent efficiency decreases

Engineering Contradiction:
Improveaging resistanceVSAvoidluminescent efficiency
Core Design Contradiction:
ReliabilityVSUse of energy by moving object

Solution Approach 1:

The patent applies local quality by creating a gradient oxygen distribution where the surface layer has higher oxygen content (improving stability) while the core maintains lower oxygen content (preserving luminescent efficiency). This is achieved through controlled low-temperature calcination that limits oxygen diffusion to primarily the surface regions, thereby resolving the contradiction between durability and efficiency.

Inventive Principle:
Principle #3Local quality

Solution Approach 2:

The fluorescent powder particle is segmented into distinct zones: a core region with low oxygen content for high luminescent efficiency and a surface layer with high oxygen content for improved chemical stability and aging resistance. This spatial segmentation allows each region to optimize its function without compromising the other.

Inventive Principle:
Principle #1Segmentation

2Use of energy by moving object

If oxygen content is limited to maintain luminescent brightness, then luminescent efficiency is maintained, but durability and aging resistance are reduced

Engineering Contradiction:
Improveluminescent efficiencyVSAvoiddurability
Core Design Contradiction:
Use of energy by moving objectVSReliability

Solution Approach 1:

The invention resolves this contradiction by applying local quality differently - the core maintains low oxygen content to preserve luminescent brightness while the surface layer is enriched with oxygen to provide durability and aging resistance. This localized differentiation allows simultaneous optimization of both parameters.

Inventive Principle:
Principle #3Local quality

3Manufacturing precision

If alloy process is used to achieve low oxygen content and high phase purity, then manufacturing precision is improved, but durability is significantly reduced

Engineering Contradiction:
Improvephase purityVSAvoiddurability
Core Design Contradiction:
Manufacturing precisionVSReliability

Solution Approach 1:

The patent changes the processing parameters by introducing a low-temperature calcination step (400-800°C) after the alloy process. This parameter change enables oxygen to be selectively introduced into the surface layer without disrupting the core's low-oxygen, high-purity phase structure, thereby improving durability while maintaining manufacturing precision.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The low-temperature calcination is performed as a preliminary surface treatment before final product completion. This preliminary action of oxygen enrichment at the surface prepares the material for improved durability without affecting the core properties that provide high phase purity.

Inventive Principle:
Principle #10Preliminary action

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The nitroxide fluorescent powder achieves good chemical stability, excellent aging and light decay resistance, high luminescent efficiency, and wide applicability, making it suitable for various luminescent devices, while the manufacturing method is simple and suitable for industrial mass production.

Implementation Method 1

a nitroxide fluorescent powder capable of being effectively excited with UV light, violet light, or blue light

Methodology Applied
Scientific EffectPhotoluminescence: Photoluminescence

Data Source

PatentEP3225677B1Nitrogen oxide fluorescent powder and preparation method therefor, nitrogen oxide light emitting body, and light-emitting device
Publication Date: 2020.05.13 JIANGSU BREE OPTRONICS CO LTD
  • EP3225677B1 patent drawingFigure 1~2
  • EP3225677B1 patent drawingFigure 3~4
  • EP3225677B1 patent drawingFigure 5~6

AI summary

The present invention discloses a nitroxide fluorescent powder comprising an inorganic compound containing M, A, B, O, N, and R elements; in which the M element is at least one of Ca, Sr, Ba, Mg, Li, Na, and K, the A element is at least one of B, Al, Ga, and In, the B element is at least one of C, Si, Ge, and Sn, the R element is at least one of Ce, Eu, Lu, Dy, Gd, and Ho, characterized in that the inorganic compound forms a crystal in a crystalline phase, and the oxygen atom content in the crystal in a crystalline phase is in an increasing structural distribution from a core to surface of the crystal. The nitroxide fluorescent powder and the nitroxide illuminant of the present invention have the advantages of good chemical stability, good aging and light decay resistance, and high luminescent efficiency, and are useful for various luminescent devices. The preparation method of the present invention is easy and reliable and useful for industrial mass production.