NMR Sample Holder Cooling and Rotation via Segmented Gas Flows

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Solution Overview

Problem

Current NMR technologies face challenges in achieving high sensitivity and cost-effectiveness for solid sample analysis, while ensuring operator safety and environmental friendliness, particularly in reaching high rotation speeds and low temperatures efficiently.

Innovation Solution

The method involves generating high-pressure gaseous flows from a primary source, cooling them in a heat exchanger with a coolant, and using these flows to rotate and cool the sample-holder, allowing for adjustable rotation speeds up to 30 kHz and temperatures between 4.2 K and 300 K, with a separate flow supporting the sample-holder, and incorporating a computer program and device for precise control.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Measurement precision

If high rotation speeds are achieved using conventional gas flows, then NMR sensitivity is improved, but the temperature control becomes inadequate and safety risks increase

Engineering Contradiction:
ImproveNMR sensitivityVSAvoidtemperature control
Core Design Contradiction:
Measurement precisionVSTemperature

Solution Approach 1:

The gas flow system is segmented into separate functional flows: a first high-pressure cooled gas flow dedicated to rotation and a second gas flow dedicated to temperature control. This segmentation allows each flow to be independently optimized for its specific function, enabling high rotation speeds while maintaining precise temperature control and safety.

Inventive Principle:
Principle #1Segmentation

2Adaptability or versatility

If multiple gas flows are used for rotation and temperature control, then functionality is improved, but device complexity increases

Engineering Contradiction:
ImprovefunctionalityVSAvoiddevice complexity
Core Design Contradiction:
Adaptability or versatilityVSDevice complexity

Solution Approach 1:

A single high-pressure gas source serves multiple functions by generating different cooled gas flows that are directed to different components. The first flow rotates the sample holder while the second flow controls temperature, allowing one gas source to fulfill multiple roles and reducing overall system complexity.

Inventive Principle:
Principle #6Universality (Multi-functionality)

Solution Approach 2:

A cooling device acts as an intermediary between the high-pressure gas source and the gas flows. This intermediary cools the gas before it is distributed to different functions, enabling temperature control to be integrated into the rotation system without requiring separate heating/cooling infrastructure.

Inventive Principle:
Principle #24Intermediary (Mediator)

3Speed

If high-pressure gas is used for rotation, then rotation speed is improved, but safety and environmental concerns worsen

Engineering Contradiction:
Improverotation speedVSAvoidsafety and environmental risks
Core Design Contradiction:
SpeedVSObject-affected harmful factors

Solution Approach 1:

The high-pressure gas, which could be considered a hazard, is converted into a beneficial cooling medium. By cooling the high-pressure gas flows before they contact the sample holder and surrounding components, the system transforms a potential safety risk into an active temperature control mechanism that enhances both safety and performance.

Inventive Principle:
Principle #22Blessing in disguise (Convert harm into benefit)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This approach enhances NMR sensitivity, achieves high rotation speeds, and maintains safety and environmental sustainability by allowing precise control over temperature and rotation speed, dissociating cooling and rotation functions, and enabling efficient gas recovery and reheating.

Implementation Method 1

The first high-pressure gaseous flow can drive the rotation of the sample-holder by its action on fins or blades of a device linked to the sample-holder to drive its rotation.

Methodology Applied
Scientific EffectGas flow action on fins/blades: Turbine

Implementation Method 2

cooling of the gaseous flows in at least one heat exchanger from the circulation of a coolant originating from at least one second source

Methodology Applied
Scientific EffectHeat exchanger cooling: Heat Exchanger

Implementation Method 3

cooling of the gaseous flows in at least one heat exchanger from the circulation of a coolant

Methodology Applied
Scientific EffectCoolant circulation: Convection

Data Source

PatentUS9995802B2Very low temperature NMR method and device
Publication Date: 2018.06.12 COMMISSARIAT A LENERGIE ATOMIQUE ET AUX ENERGIES ALTERNATIVES

AI summary

The NMR analysis method for analyzing a solid sample positioned in a sample-holder (21) includes generation of a plurality of high-pressure gaseous flows (2, 3, 4) from at least one first source (1) of a high-pressure gas; cooling of the gaseous flows (2, 3, 4) in at least one heat exchanger (12) from a coolant gas (15) originating from at least one second source (11) of gas; and rotation of the sample-holder (21) by a first cooled high-pressure gaseous flow (2) and cooling of the sample-holder by a second cooled high-pressure gaseous flow (3).