Super Absorbent Polymer Surface Cross-Linking Without Epoxy

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Solution Overview

Problem

Existing super absorbent polymers face challenges in achieving high absorption performance under pressure while maintaining anti-caking properties, particularly when using silica or clay as cross-linking agents, which can lead to reduced water retention capacity and separation issues, especially in hygiene products like diapers, and there is a need for a method that excludes hazardous chemical substances.

Innovation Solution

A preparation method involving the formation of hydrogel polymers through cross-linking with a non-epoxy surface cross-linking agent, followed by surface cross-linking at controlled temperatures, including a first raising and then lowering of temperature stages, to create super absorbent polymer particles with improved anti-caking and absorption properties.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Quantity of substance

If silica or clay is added as cross-linking agent to improve permeability, then permeability is improved, but water retention capacity and absorbency under pressure are reduced

Engineering Contradiction:
ImprovepermeabilityVSAvoidwater retention capacity
Core Design Contradiction:
Quantity of substanceVSReliability

Solution Approach 1:

The patent changes the chemical composition parameters by replacing traditional silica/clay cross-linking agents with a two-stage cross-linking system using glycerol monomethacrylate (internal) and ethylene glycol dimethacrylate (surface), optimizing the molecular structure and cross-linking density to achieve both high permeability and water retention capacity

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent creates a composite polymer structure combining polyacrylic acid chains with specific cross-linking agents, forming a network that integrates porous structure for permeability with cross-linked bonds for water retention, achieving synergistic performance

Inventive Principle:
Principle #40Composite materials

2Quantity of substance

If silica or clay is added to improve permeability, then permeability is improved, but separation occurs during transport due to external physical impact

Engineering Contradiction:
ImprovepermeabilityVSAvoidanti-caking property
Core Design Contradiction:
Quantity of substanceVSStability of the object's composition

Solution Approach 1:

The patent merges the permeability-enhancing function and the anti-caking function into a single integrated polymer network structure, where the cross-linked gel particles maintain both porous channels for fluid flow and structural integrity for transport stability, eliminating the need for separate silica/clay additives

Inventive Principle:
Principle #5Merging (Combining)

3Stability of the object's composition

If epoxy-based surface cross-linking agent is used to achieve anti-caking, then anti-caking performance is improved, but chemical hazards are introduced

Engineering Contradiction:
Improveanti-caking propertyVSAvoidchemical hazards
Core Design Contradiction:
Stability of the object's compositionVSObject-affected harmful factors

Solution Approach 1:

The patent replaces hazardous epoxy-based cross-linking agents with biocompatible, non-toxic alternatives (glycerol monomethacrylate and ethylene glycol dimethacrylate) that provide equivalent anti-caking performance without chemical hazards, making the product safe for hygiene applications

Inventive Principle:
Principle #27Cheap short-living objects (Disposable)

Solution Approach 2:

The patent changes the chemical safety parameters by selecting cross-linking agents with favorable toxicological profiles, specifically using glycerol-derived and ethylene glycol-derived monomers that are recognized as safe for contact with skin and mucous membranes

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The method maintains excellent absorption-related physical properties and anti-caking performance of super absorbent polymers, even under high temperature and humidity conditions, without using epoxy-based agents that pose chemical hazards.

Implementation Method 1

forming a hydrogel polymer by cross-linking polymerizing a water-soluble ethylene-based unsaturated monomer

Methodology Applied
Scientific EffectCross-linking: Chemical Bonding

Implementation Method 2

polymerizing a water-soluble ethylene-based unsaturated monomer having at least partially neutralized acidic groups in the presence of a polymerization initiator

Methodology Applied
Scientific EffectPolymerization: Chemical Bonding

Data Source

PatentUS12453957B2Preparation method of super absorbent polymer
Publication Date: 2025.10.28 LG CHEM LTD

AI summary

The present disclosure relates to a preparation method of a super absorbent polymer, and there is provided a preparation method of a super absorbent polymer capable of achieving anti-caking while maintaining excellent absorption-related physical properties of super absorbent polymer particles by performing surface cross-linking at a relatively lower temperature than before using a non-epoxy cross-linking agent without an epoxy-based surface cross-linking agent, which is a controversial source of chemical hazards.