ODDA Process Lime Removal via Polyacrylamide Flocculation

Resolve Bottlenecks,
Find Innovative Solutions
Generate Solutions

Solution Overview

Problem

The ODDA process for fertilizer production faces challenges in removing residual calcium carbonate (CaCO3) from the ammonium-nitrate containing liquid, which interferes with pH levels, heat exchange in evaporators, and granulation processes, and traditional methods like pressure filtration are costly and labor-intensive.

Innovation Solution

The use of an ultrahigh molecular weight anionic polyacrylamide flocculant, such as Magnafloc 919, is added in low concentrations to the sedimentation vessel to facilitate the complete precipitation of calcium carbonate, eliminating the need for pressure filtration and reducing maintenance costs.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Manufacturing precision

If pressure filtration is used to remove calcium carbonate, then CaCO3 removal efficiency is improved, but maintenance costs and process downtime increase

Engineering Contradiction:
ImproveCaCO3 removal efficiencyVSAvoidprocess downtime
Core Design Contradiction:
Manufacturing precisionVSProductivity

Solution Approach 1:

The harmful component (CaCO3) is extracted from the solution through enhanced sedimentation using flocculant, separating it from the ammonium nitrate solution without requiring complex filtration equipment that needs frequent maintenance

Inventive Principle:
Principle #2Taking out (Extraction)

Solution Approach 2:

A flocculant is introduced as an intermediary substance to facilitate the aggregation and sedimentation of CaCO3 particles, enabling effective removal through simple sedimentation rather than complex pressure filtration

Inventive Principle:
Principle #24Intermediary (Mediator)

2Manufacturing precision

If pressure filtration is used to remove calcium carbonate, then CaCO3 removal efficiency is improved, but maintenance costs increase

Engineering Contradiction:
ImproveCaCO3 removal efficiencyVSAvoidmaintenance costs
Core Design Contradiction:
Manufacturing precisionVSEase of manufacture

Solution Approach 1:

The process replaces expensive, maintenance-intensive pressure filtration equipment with simple sedimentation vessels and inexpensive flocculant chemicals, accepting that the flocculant is consumed but eliminating equipment maintenance costs

Inventive Principle:
Principle #27Cheap short-living objects (Disposable)

Solution Approach 2:

The mechanical pressure filtration system is replaced with a chemical-facilitated sedimentation system, where chemical flocculation replaces mechanical filtration to achieve the same separation goal with lower maintenance requirements

Inventive Principle:
Principle #28Mechanics substitution (Replace mechanical system)

3Reliability

If lime is present in the AN solution, then pH control is maintained, but heat exchange capability in evaporators deteriorates

Engineering Contradiction:
ImprovepH controlVSAvoidheat exchange capability
Core Design Contradiction:
ReliabilityVSUse of energy by moving object

Solution Approach 1:

The harmful effect of lime accumulation in evaporators is prevented by converting the lime into easily removable sediment through flocculation, allowing the lime to be beneficially separated before the evaporation stage rather than causing heat exchange problems

Inventive Principle:
Principle #22Blessing in disguise (Convert harm into benefit)

4Quantity of substance

If lime is present in the overflow liquid, then ammonium carbonate is available for conversion, but granulation process is negatively interfered with

Engineering Contradiction:
Improveammonium carbonate availabilityVSAvoidgranulation process
Core Design Contradiction:
Quantity of substanceVSEase of operation

Solution Approach 1:

The solution applies different treatment to different components: ammonium carbonate is preserved in solution for conversion reactions, while calcium carbonate is selectively flocculated and removed to protect the granulation process, achieving local quality differentiation in the treatment approach

Inventive Principle:
Principle #3Local quality

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This approach achieves nearly complete removal of CaCO3 (up to 99.99%) without the need for pressure filtration, improving process efficiency and reducing downtime and costs by ensuring effective sedimentation and preventing blockages in evaporators.

Implementation Method 1

the addition of less than 5 ppm of an ultrahigh molecular weight anionic polyacrylamide as flocculant leads to an effective and complete removal of CaCO3

Methodology Applied
Scientific EffectFlocculation: Flocculation

Implementation Method 2

The mixture is then cooled, in general to below 0 °C. The calcium nitrate crystallizes

Methodology Applied
Scientific EffectCrystallization: Crystallisation

Implementation Method 3

CaCO3 precipitates from the reaction mixture obtained by chemical equation 4 in the thickener

Methodology Applied
Scientific EffectSedimentation: Sedimentation

Data Source

PatentEP4056542A1ODDA process for the production of nitrogen-based fertilizers with reduced sand formation
Publication Date: 2022.09.14 EUROCHEM ANTWERPEN
  • EP4056542A1 patent drawingFigure 1
  • EP4056542A1 patent drawingFigure 2
  • EP4056542A1 patent drawingFigure 3

AI summary

The present invention is directed at an ODDA process with an improved lime removal for fertilizer production. In a preferred embodiment, the improved lime removal is obtained by the addition of an ultra-high molecular weight anionic polyacrylamide as flocculant.