OLED Emissive Layer Host-Dopant Composite for Efficiency and Lifespan

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Solution Overview

Problem

Current organic light emitting diodes (OLEDs) face challenges in achieving high luminous efficiency and long luminous lifespan, particularly due to the short lifespan of phosphorescent materials used in commercial applications and the low efficiency of fluorescent materials that only utilize singlet exciton energy.

Innovation Solution

An OLED structure incorporating an emissive layer with a host material represented by specific formulas and an organometallic compound as a dopant, which includes a metal atom linked to a fused hetero aromatic ring ligand, enhances luminous efficiency and lifespan by facilitating rapid charge and exciton energy transfer, thereby improving color purity and reducing driving voltages.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Use of energy by moving object

If phosphorescent material is used to achieve high luminous efficiency, then luminous efficiency is improved, but luminous lifespan deteriorates

Engineering Contradiction:
Improveluminous efficiencyVSAvoidluminous lifespan
Core Design Contradiction:
Use of energy by moving objectVSDuration of action of stationary object

Solution Approach 1:

The patent uses a composite emissive layer containing both phosphorescent dopant (Ir(III) complex) and fluorescent host materials (carbazole derivatives). This composite structure enables the system to benefit from both high efficiency (phosphorescent triplet excitons) and long lifespan (fluorescent host stability), resolving the contradiction between efficiency and lifespan by combining materials with complementary characteristics

Inventive Principle:
Principle #40Composite materials

Solution Approach 2:

The fluorescent host material acts as an intermediary that receives excitons from charge recombination and transfers energy to the phosphorescent dopant. This intermediary mechanism allows efficient energy utilization while the host material's stable structure protects the system, extending operational lifespan

Inventive Principle:
Principle #24Intermediary (Mediator)

2Duration of action of stationary object

If fluorescent material is used to achieve long luminous lifespan, then luminous lifespan is improved, but luminous efficiency deteriorates

Engineering Contradiction:
Improveluminous lifespanVSAvoidluminous efficiency
Core Design Contradiction:
Duration of action of stationary objectVSUse of energy by moving object

Solution Approach 1:

The patent creates a composite system where fluorescent host materials provide structural stability and long lifespan, while phosphorescent dopants provide high efficiency through triplet exciton utilization. The synergistic combination allows the system to achieve both extended operational life and high energy conversion efficiency

Inventive Principle:
Principle #40Composite materials

Solution Approach 2:

The fluorescent host serves as an intermediary that facilitates efficient energy transfer from charge recombination to the phosphorescent dopant. This intermediary role enables the system to overcome the inherent low efficiency of pure fluorescent materials while maintaining their stability advantages

Inventive Principle:
Principle #24Intermediary (Mediator)

3Use of energy by moving object

If organometallic compound with hetero aromatic ligand is used to enhance luminous efficiency, then luminous efficiency is improved, but device complexity increases

Engineering Contradiction:
Improveluminous efficiencyVSAvoidemissive layer composition
Core Design Contradiction:
Use of energy by moving objectVSDevice complexity

Solution Approach 1:

The patent optimizes parameters such as dopant concentration (0.1-10 wt%), host-to-dopant energy level matching, and molecular structure parameters of the organometallic compound. By carefully controlling these parameters, the system achieves high luminous efficiency while managing the complexity of the emissive layer composition

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent applies local quality by using specific carbazole-based host materials with particular molecular structures ( Formulae 7 and 9) that are optimized for their local environment in the emissive layer. This targeted molecular design improves efficiency at the molecular level while keeping the overall device structure manageable

Inventive Principle:
Principle #3Local quality

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The proposed OLED structure significantly enhances luminous efficiency and lifespan by utilizing an organometallic compound with a hetero aromatic ligand for efficient charge and exciton energy transfer, leading to improved color purity and reduced driving voltages in organic light emitting diodes.

Implementation Method 1

an emissive layer disposed between the first and second electrodes and including at least one emitting material layer

Methodology Applied
Scientific EffectElectroluminescence: Electroluminescence

Implementation Method 2

facilitating rapid charge and exciton energy transfer

Methodology Applied
Scientific EffectEnergy transfer:

Implementation Method 3

phosphorescent material can show high luminous efficiency since it uses triplet exciton energy as well as singlet exciton energy in the luminous process

Methodology Applied
Scientific EffectPhosphorescence: Phosphorescence

Implementation Method 4

Since fluorescent material uses only singlet exciton energy in the luminous process

Methodology Applied
Scientific EffectFluorescence: Fluorescence

Data Source

PatentEP4188058B1Organic light emitting diode and organic light emitting device having thereof
Publication Date: 2024.12.11 LG DISPLAY CO LTD
  • EP4188058B1 patent drawingFigure 1
  • EP4188058B1 patent drawingFigure 2
  • EP4188058B1 patent drawingFigure 3

AI summary

An organic light emitting diode (OLED) in which at least one emitting material layer includes a dopant having a structure represented by Formula 1 and a biscarbazole-base host and an azine-based host, and an organic light emitting device including the OLED. The OLED and the organic light emitting device including the hosts and the dopant can improve their luminous efficiency and luminous lifespan.         [Formula 1]     Ir(LA)m(LB)n