Optical Brightener Formulation for Papermaking Brightness and Retention

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Solution Overview

Problem

Conventional optical brighteners (OBAs) face limitations in achieving higher brightness in papermaking due to cost constraints and inefficiencies in retention and stability, with tetra-sulfonated stilbene OBA causing sheet yellowing and hexa-sulfonated OBA being expensive, and current carriers like polyvinyl alcohol requiring costly cooking processes.

Innovation Solution

A formulation combining polyvinyl alcohol, glucomannan, carboxymethyl cellulose, and sorbitol as carriers to optimize OBA retention, reducing dosage rates and enhancing brightness and whiteness while minimizing the need for external heating and water addition, using low viscosity polyvinyl alcohol and konjac glucomannan for improved dispersion and cohesion.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Illumination intensity

If tetra-sulfonated stilbene OBA is used to improve brightness, then brightness is improved, but sheet yellowing and over-greening occur due to overdosing

Engineering Contradiction:
ImprovebrightnessVSAvoidsheet yellowing
Core Design Contradiction:
Illumination intensityVSObject-affected harmful factors

Solution Approach 1:

The patent uses a carrier system comprising polyvinyl alcohol and glucomannan as intermediary substances to deliver the OBA to the paper. This mediator approach allows controlled release and distribution of the OBA, preventing localized overdosing that causes yellowing while maintaining overall brightness enhancement.

Inventive Principle:
Principle #24Intermediary (Mediator)

Solution Approach 2:

The patent changes the physical and chemical parameters of the OBA delivery system by using a carrier formulation with specific molecular weights and ratios of polyvinyl alcohol to glucomannan. This parameter optimization enables better retention and uniform distribution of OBA, avoiding the yellowing effect associated with conventional direct addition methods.

Inventive Principle:
Principle #35Parameter changes

2Illumination intensity

If hexa-sulfonated stilbene OBA is used to achieve higher brightness, then brightness is improved, but cost increases significantly

Engineering Contradiction:
ImprovebrightnessVSAvoidcost
Core Design Contradiction:
Illumination intensityVSQuantity of substance

Solution Approach 1:

The carrier system acts as an efficient delivery mechanism that maximizes the utilization of tetra-sulfonated stilbene OBA, extracting maximum brightness performance from this more cost-effective compound and reducing the need to use expensive hexa-sulfonated alternatives.

Inventive Principle:
Principle #24Intermediary (Mediator)

Solution Approach 2:

The patent employs a cost-effective carrier formulation using readily available polyvinyl alcohol and glucomannan materials, creating an economical system that achieves high brightness without requiring expensive specialty chemicals.

Inventive Principle:
Principle #27Cheap short-living objects (Disposable)

3Reliability

If polyvinyl alcohol carrier is used to improve OBA retention, then OBA retention is improved, but costly cooking processes are required

Engineering Contradiction:
ImproveOBA retentionVSAvoidcooking cost
Core Design Contradiction:
ReliabilityVSEase of manufacture

Solution Approach 1:

The patent merges polyvinyl alcohol with glucomannan in a carrier formulation, creating a synergistic system where glucomannan enhances the OBA retention capability while the combination allows for simplified processing that reduces or eliminates the need for expensive cooking operations.

Inventive Principle:
Principle #5Merging (Combining)

Solution Approach 2:

The carrier is formulated as a composite material combining polyvinyl alcohol and glucomannan, leveraging the properties of both components to achieve superior OBA retention without requiring the high-energy cooking process traditionally needed for polyvinyl alcohol alone.

Inventive Principle:
Principle #40Composite materials

4Illumination intensity

If OBA addition dosage is increased to satisfy higher brightness demand, then brightness is improved, but water retention capability deteriorates

Engineering Contradiction:
ImprovebrightnessVSAvoidwater retention
Core Design Contradiction:
Illumination intensityVSLoss of substance

Solution Approach 1:

The carrier system serves as an intermediary that binds OBA molecules, preventing them from interfering with the water retention mechanisms in the paper. This mediated approach allows high OBA concentrations for brightness enhancement without the negative impact on water retention that would occur with direct high-dosage OBA addition.

Inventive Principle:
Principle #24Intermediary (Mediator)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The formulation achieves significant brightness gains with reduced OBA addition rates, improved whiteness, and enhanced water retention, while minimizing cost and environmental impact, and provides resistance to light-induced aging and color aberrations.

Implementation Method 1

The formulation includes the optical brightener, polyvinyl alcohol, glucomannan, carboxymethyl cellulose, and sorbitol. These complementary elements gives noticeable retention power to OBA

Methodology Applied
Scientific EffectAdsorption: Adsorption

Implementation Method 2

using low viscosity polyvinyl alcohol and konjac glucomannan for improved dispersion and cohesion

Methodology Applied
Scientific EffectCohesion: Cohesion

Implementation Method 3

When observed under light, OBAs can absorb invisible ultraviolet light and re-emit visible blue light back, giving viewers the visual perception of a brighter sheet

Methodology Applied
Scientific EffectFluorescence: Fluorescence

Implementation Method 4

using low viscosity polyvinyl alcohol and konjac glucomannan for improved dispersion and cohesion

Methodology Applied
Scientific EffectViscosity reduction:

Implementation Method 5

The formulation includes the optical brightener, polyvinyl alcohol, glucomannan, carboxymethyl cellulose, and sorbitol. These complementary elements gives noticeable retention power to OBA, yielding significant OBA dosage reduction along with other benefits such as lower additive viscosity and reinforced bonding to the sizing/coating medium

Methodology Applied
Scientific EffectHydration: Mineral Hydration

Data Source

PatentUS9512569B1Formulation of optical brighteners for papermaking
Publication Date: 2016.12.06 MENG JUN LI

AI summary

This invention relates to a formulation of optical brightener, polyvinyl alcohol, glucomannan, carboxymethyl cellulose, and sorbitol which can be used on the sizing or coating application of papermaking. This composition yields high whiteness and brightness on the product paper.