Optical Thermoplastic Resin with Low Birefringence

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Solution Overview

Problem

Existing optical thermoplastic resins face challenges in achieving low orientation birefringence, photoelastic birefringence, and maintaining heat stability while ensuring excellent transparency and color tone, especially in thick formed bodies like injection-formed bodies, due to issues with polymer decomposition and defects during high-temperature forming processes.

Innovation Solution

A novel optical thermoplastic resin with a specific composition of methacrylic and acrylic esters, along with a small amount of another monofunctional monomer, is developed, which has a melt viscosity reduction rate of less than 20%, orientation birefringence between -1.7 × 10^-4 and 1.7 × 10^-4, and a photoelastic constant between -3.7 × 10^-12 and 3.7 × 10^-12 Pa^-1, ensuring low birefringence and high heat stability, and is formed into a 2mm-thick body with haze of 1% or less.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Manufacturing precision

If conventional optical resins are used to form thick optical members, then the optical members can be produced with various shapes, but the resins exhibit high birefringence and poor transparency due to orientation and photoelastic birefringence

Engineering Contradiction:
Improveoptical isotropyVSAvoidtransparency
Core Design Contradiction:
Manufacturing precisionVSReliability

Solution Approach 1:

The patent changes the chemical composition parameters of the optical resin by incorporating fluorinated monomers (containing CF3 groups) and specific methacrylic/acrylic ester ratios to achieve low birefringence and high transparency in thick formed bodies

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent creates a composite resin system combining fluorinated monomers with methacrylic and acrylic esters to achieve synergistic effects that reduce both orientation and photoelastic birefringence while maintaining excellent optical properties

Inventive Principle:
Principle #40Composite materials

2Ease of manufacture

If high-temperature forming processes are used to produce thick optical members, then various complex shapes can be achieved, but polymer decomposition occurs causing defects and poor optical properties

Engineering Contradiction:
ImproveformabilityVSAvoidheat stability
Core Design Contradiction:
Ease of manufactureVSReliability

Solution Approach 1:

The patent modifies the thermal stability parameters of the resin by incorporating fluorinated monomers that raise the decomposition temperature, enabling high-temperature forming processes without polymer degradation while maintaining formability

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent uses a carefully controlled combination of monomers with specific functional groups that provide temporary thermal stability during the forming process, preventing decomposition defects without requiring expensive additional stabilizers

Inventive Principle:
Principle #27Cheap short-living objects (Disposable)

3Manufacturing precision

If polymer resins with low orientation birefringence are developed, then optical isotropy is improved, but photoelastic birefringence and heat stability remain problematic

Engineering Contradiction:
Improveorientation birefringenceVSAvoidphotoelastic birefringence
Core Design Contradiction:
Manufacturing precisionVSReliability

Solution Approach 1:

The patent simultaneously optimizes multiple chemical parameters including the incorporation of fluorinated monomers and specific ratios of methacrylic to acrylic esters to achieve low values for both orientation and photoelastic birefringence while maintaining heat stability

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent develops a multi-component resin system where fluorinated monomers, methacrylic esters, and acrylic esters work synergistically to reduce both types of birefringence and improve overall optical performance

Inventive Principle:
Principle #40Composite materials

4Reliability

If conventional resin compositions are used to ensure heat stability, then polymer decomposition is reduced, but birefringence increases and optical properties deteriorate

Engineering Contradiction:
Improveheat stabilityVSAvoidbirefringence
Core Design Contradiction:
ReliabilityVSManufacturing precision

Solution Approach 1:

The patent changes the chemical structure parameters by introducing fluorinated monomers and optimizing the ratio of methacrylic to acrylic esters to achieve both high heat stability and low birefringence simultaneously

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The resin achieves excellent optical isotropy, transparency, and color tone with reduced thermal decomposition defects, making it suitable for optical applications with improved heat stability and minimal birefringence-related issues.

Implementation Method 1

orientation birefringence mainly caused by the orientation of main chains of the polymer

Methodology Applied
Scientific EffectOrientation birefringence: Birefringence

Implementation Method 2

photoelastic birefringence caused by stress

Methodology Applied
Scientific EffectPhotoelastic birefringence: Photoelasticity

Data Source

PatentEP3088920B1Optical thermoplastic resin and formed body
Publication Date: 2020.02.26 KANEKA CORP
  • EP3088920B1 patent drawingFigure 1
  • EP3088920B1 patent drawingFigure 2
  • EP3088920B1 patent drawing

AI summary

An object of the present invention is to provide an optical thermoplastic resin having excellent transparency and color tone, and also excellent heat stability, as well as being extremely low in both orientation birefringence and photoelastic birefringence; and a formed body made of said resin. This optical thermoplastic resin has a rate of reduction in melt viscosity of less than 20%, an orientation birefringence of -1.7 × 10-4 to 1.7 × 10-4, a photoelastic constant of -3.7 × 10-12 to 3.7 × 10-12 Pa-1, and, when formed into a 2mm-thick formed body, has a haze of 1% or less.