Organic Semiconductor Ink-Jet Printing with Crystallization Agents

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Solution Overview

Problem

Current methods for producing organic semiconductor thin films often result in disordered molecular arrangements due to drying processes, leading to undesirable morphologies and performance issues in electronic and optoelectronic devices, which are not compatible with industrial scales or complex applications.

Innovation Solution

A process involving an ink composition with organic semiconductor material, crystallization agents, and solvents is used for ink-jet printing, where the crystallization agent has a melting temperature higher than the substrate temperature and boiling/sublimation temperature higher than the solvent, allowing for controlled molecular orientation and deposition of highly ordered structures.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Productivity

If solution processing methods (coating and printing) are used to deposit organic semiconductor materials, then low-cost high-throughput manufacturing is enabled, but a high degree of molecular disorder is introduced resulting in undesired morphologies

Engineering Contradiction:
Improvemanufacturing throughputVSAvoidmolecular arrangement order
Core Design Contradiction:
ProductivityVSManufacturing precision

Solution Approach 1:

The patent changes the temperature parameter during the deposition process. The substrate is heated to a temperature above the melting point of the organic semiconductor material, enabling the material to crystallize in a highly ordered manner directly from the solution during deposition, thereby achieving both high throughput and molecular order

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent utilizes phase transition of the organic semiconductor material from solid to liquid and back to solid crystalline structure. By controlling the substrate temperature above the melting point during deposition, the material undergoes phase transition to form highly ordered crystalline structures directly during the coating process, resolving the contradiction between solution processing and molecular order

Inventive Principle:
Principle #36Phase transitions

2Ease of manufacture

If conventional coating methods are used, then industrial scale production is enabled, but grain boundaries and amorphous regions are formed reducing device performance

Engineering Contradiction:
Improveindustrial scalabilityVSAvoiddevice performance
Core Design Contradiction:
Ease of manufactureVSReliability

Solution Approach 1:

The patent changes the temperature parameter by heating the substrate above the melting point of the organic semiconductor material during deposition. This parameter change enables the formation of highly ordered crystalline structures without grain boundaries or amorphous regions, thereby maintaining both industrial scalability and high device performance

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent applies preliminary heating to the substrate before and during the deposition process. This preliminary action of heating the substrate to appropriate temperature ensures that the organic semiconductor material crystallizes in a highly ordered manner as it is deposited, preventing the formation of defects before they can occur

Inventive Principle:
Principle #10Preliminary action

3Manufacturing precision

If mechanical rubbing and shearing methods are used to control molecular orientation, then anisotropic properties are achieved, but the process complexity increases and lateral resolution is insufficient for complex applications

Engineering Contradiction:
Improvemolecular orientation controlVSAvoidprocess complexity
Core Design Contradiction:
Manufacturing precisionVSDevice complexity

Solution Approach 1:

The patent replaces mechanical rubbing and shearing methods with a thermal field approach. By controlling the substrate temperature above the melting point of the material, the patent achieves molecular orientation and anisotropic properties through thermal effects during deposition, eliminating the need for complex mechanical processing steps

Inventive Principle:
Principle #28Mechanics substitution (Replace mechanical system)

Solution Approach 2:

The patent changes the temperature parameter to achieve molecular orientation. By heating the substrate to a temperature above the melting point of the organic semiconductor material during deposition, the material self-organizes into highly ordered anisotropic structures without requiring mechanical rubbing or shearing, thereby simplifying the process while maintaining precision

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

This method enables the production of electronic and optoelectronic devices with highly ordered fibers, exhibiting anisotropic properties, such as enhanced charge carrier mobilities, and simplifies the production of devices with complex geometries, improving their performance and adaptability.

Implementation Method 1

the crystallization agent has a melting temperature equal to or higher than the substrate temperature

Methodology Applied
Scientific EffectMelting: Melting

Implementation Method 2

the crystallization agent has a boiling temperature or sublimation temperature equal to or higher than the boiling temperature of the solvent

Methodology Applied
Scientific EffectCrystallization: Crystallisation

Implementation Method 3

the crystallization agent has a boiling temperature or sublimation temperature equal to or higher than the boiling temperature of the solvent

Methodology Applied
Scientific EffectSublimation: Sublimation

Implementation Method 4

one or more solvent; and applying the ink composition to the substrate

Methodology Applied
Scientific EffectEvaporation: Evaporation

Data Source

PatentEP3630896B1Electronic and optoelectronic devices having anisotropic properties and method for their production
Publication Date: 2023.11.29 INNOVATIONLAB GMBH
  • EP3630896B1 patent drawingFigure 1~2
  • EP3630896B1 patent drawingFigure 3~4
  • EP3630896B1 patent drawingFigure 5

AI summary

The present invention relates to a method for the production of electronic or optoelectronic devices with an anisotropic molecular structure of the organic semiconductor material as well as to such electronic or optoelectronic devices comprising an organic semiconductor material with anisotropic molecular structure.The present application further relates to fibers comprising a hollow core and a shell comprising an organic semiconductor material.