Organometallic Compound for Deep Blue OLEDs

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Solution Overview

Problem

Existing organic light-emitting devices (OLEDs) face challenges in achieving low driving voltage, high efficiency, and long lifespan while maintaining deep blue emission and stability against hole injection.

Innovation Solution

The use of an organometallic compound represented by Formula 1, which includes a transition metal and specific carbocyclic or heterocyclic groups, is introduced in the organic layer of OLEDs. This compound facilitates hole injection with a deep highest occupied molecular orbital (HOMO) energy level and enhances stability and light-emitting ability.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Illumination intensity

If conventional organic light-emitting devices are used, then deep blue emission can be achieved, but driving voltage is high and lifespan is short

Engineering Contradiction:
Improvedeep blue emissionVSAvoiddriving voltage
Core Design Contradiction:
Illumination intensityVSPower

Solution Approach 1:

The patent modifies the molecular structure of the organometallic compound by changing parameters such as the metal center (Ir, Pt, Os), ligand types (carbazole, triazole, tetrazole), and substituent groups to optimize the HOMO energy level. This structural parameter optimization enables deep blue emission while reducing driving voltage through improved hole injection characteristics

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent employs composite organometallic compounds combining transition metals with specific organic ligands (carbazole derivatives, triazole/tetrazole rings). This composite structure synergistically combines the deep blue emission capability of iridium/platinum/osmium complexes with the high hole mobility and stability of carbazole-based ligands, achieving both low driving voltage and long lifespan

Inventive Principle:
Principle #40Composite materials

2Illumination intensity

If conventional organic light-emitting devices are used, then deep blue emission can be achieved, but stability against hole injection is poor

Engineering Contradiction:
Improvedeep blue emissionVSAvoidstability against hole injection
Core Design Contradiction:
Illumination intensityVSReliability

Solution Approach 1:

The patent optimizes the HOMO energy level parameter of the organometallic compound by adjusting ligand structures and substituents. The deep HOMO level (below -5.5 eV) is specifically engineered to improve stability against hole injection while maintaining deep blue emission, resolving the contradiction between emission quality and injection stability

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent uses robust organometallic compounds with high chemical stability and resistance to degradation from hole injection. The stable triazole and tetrazole ligand structures provide long-term operational stability, effectively replacing less stable conventional materials

Inventive Principle:
Principle #27Cheap short-living objects (Disposable)

3Reliability

If conventional organic light-emitting devices are used, then operation can be maintained, but efficiency is low

Engineering Contradiction:
Improveoperation continuityVSAvoidluminous efficiency
Core Design Contradiction:
ReliabilityVSProductivity

Solution Approach 1:

The patent optimizes the photophysical parameters of the organometallic compound including photoluminescence quantum yield, emission wavelength, and charge carrier mobility. These parameter optimizations enable high luminous efficiency while maintaining stable operation, achieving both reliability and productivity improvements

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent replaces conventional organic electroluminescent materials with organometallic compounds that utilize metal-to-ligand charge transfer (MLCT) mechanisms. This substitution provides more efficient radiative decay pathways and better charge carrier management, improving overall device efficiency

Inventive Principle:
Principle #28Mechanics substitution (Replace mechanical system)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The incorporation of the organometallic compound into the OLEDs results in a low driving voltage, high efficiency, and long lifespan, while maintaining deep blue emission and improved stability against hole injection.

Implementation Method 1

the organometallic compound has a deep highest occupied molecular orbital (HOMO) energy level and thus has stability against hole injection and hole injection is facilitated

Methodology Applied
Scientific EffectHole injection:

Implementation Method 2

The holes and the electrons recombine in the emission layer to produce excitons. These excitons may transition from an excited state to a ground state, thereby generating light

Methodology Applied
Scientific EffectElectroluminescence: Electroluminescence

Data Source

PatentEP4299692B1Organometallic compound, organic light-emitting device including the same, and electronic apparatus including the organic light-emitting device
Publication Date: 2025.05.14 SAMSUNG DISPLAY CO LTD
  • EP4299692B1 patent drawingFigure 1
  • EP4299692B1 patent drawingFigure 2
  • EP4299692B1 patent drawingFigure 3

AI summary

An organometallic compound represented by Formula 1: wherein, M is a transition metal, X11 is N or C(R11), X12 is N or C(R12), at least one of X11 and X12 is N, ring CY2, ring CY31, ring CY32, and ring CY4 are each independently a C3-C60 carbocyclic group or a C1-C60 heterocyclic group, Y2 to Y4 are each independently C or N, A2 to A4 are each independently a chemical bond, O, or S, a1 to a3 are each independently an integer from 0 to 3, and the remaining substitutions are as provided in the detailed description.