Oxide Phosphor Surface Coating for Broad Near-Infrared Emission

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Solution Overview

Problem

Existing light emitting devices lack a near-infrared phosphor with a wide full width at half maximum and a light emission peak wavelength in a longer range, suitable for applications such as non-destructive measurement of food and agricultural products, plant growth, and safe visualization inside living bodies.

Innovation Solution

An oxide phosphor is produced by heat-treating a raw material mixture containing Ga and Cr with a flux containing Group 4, 5, or 14 elements, resulting in phosphor particles with adhered first compound particles, enhancing light emission intensity and particle size.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Illumination intensity

If a conventional phosphor is used, then the light emitting device can be manufactured with standard materials, but the light emission intensity in the near-infrared range is insufficient

Engineering Contradiction:
Improvelight emission intensityVSAvoidphosphor composition complexity
Core Design Contradiction:
Illumination intensityVSEase of manufacture

Solution Approach 1:

The patent employs a composite phosphor system consisting of a host crystal (β-Ga2O3) doped with activating elements (Cr, Mn, Fe, Co, or Ni) and surface-coated oxide particles (TiO2, ZrO2, HfO2, Nb2O5, Ta2O5, SiO2, GeO2, SnO2, PbO2, P2O5, As2O3, Sb2O3, or Bi2O3). This composite structure enables enhanced near-infrared light emission intensity while maintaining manufacturability through established ceramic processing techniques.

Inventive Principle:
Principle #40Composite materials

2Adaptability or versatility

If a phosphor with longer peak wavelength is used, then the suitability for non-destructive measurement and visualization applications is improved, but the full width at half maximum becomes narrower

Engineering Contradiction:
Improveapplication suitabilityVSAvoidfull width at half maximum
Core Design Contradiction:
Adaptability or versatilityVSIllumination intensity

Solution Approach 1:

The patent achieves a broad emission spectrum with extended near-infrared coverage by carefully controlling the composition ratios of multiple activating elements (Cr: 0.01-5 wt%, Mn: 0.01-5 wt%, Fe: 0.01-5 wt%, Co: 0.01-5 wt%, Ni: 0.01-5 wt%) in the β-Ga2O3 host crystal. This compositional parameter optimization results in a phosphor with both long peak wavelength and wide full width at half maximum, satisfying both application suitability and spectral breadth requirements.

Inventive Principle:
Principle #35Parameter changes

3Illumination intensity

If the phosphor particle size is increased, then the light emission intensity is enhanced, but the particle aggregation and handling difficulty increase

Engineering Contradiction:
Improvelight emission intensityVSAvoidparticle handling
Core Design Contradiction:
Illumination intensityVSEase of operation

Solution Approach 1:

The patent applies oxide particle coatings (TiO2, ZrO2, HfO2, Nb2O5, Ta2O5, SiO2, GeO2, SnO2, PbO2, P2O5, As2O3, Sb2O3, or Bi2O3) on the surface of the phosphor particles. This surface modification enhances the mechanical strength and dispersibility of large particles (10-50 μm diameter), preventing aggregation while maintaining high light emission intensity. The coated surface provides better handling characteristics despite the increased particle size.

Inventive Principle:
Principle #3Local quality

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The oxide phosphor achieves high light emission intensity and a wide full width at half maximum, enabling effective non-destructive measurement and safe visualization in the near-infrared range.

Implementation Method 1

a light emitting element configured to emit light having a light emission peak wavelength of 365 nm or more and 650 nm or less

Methodology Applied
Scientific EffectLight emission from light emitting element: Light Emitting Diode

Implementation Method 2

an oxide phosphor... containing a host crystal containing Ga and oxygen and an activating element

Methodology Applied
Scientific EffectPhotoluminescence: Photoluminescence

Data Source

PatentEP4610329A1Oxide phosphor, light emitting device, and method for producing oxide phosphor
Publication Date: 2025.09.03 NICHIA CORP
  • EP4610329A1 patent drawingFigure 1
  • EP4610329A1 patent drawingFigure 2
  • EP4610329A1 patent drawingFigure 3

AI summary

An oxide phosphor includes phosphor particles containing a host crystal containing Ga and oxygen and an activating element, and a first compound particle disposed on at a surface(s) of the phosphor particles, the at least one first compound particle containing an oxide particle containing a first element selected from the group consisting of Group 4 elements, Group 5 elements, Group 14 elements, and Group 15 elements.