Oxygen Scavenging Polyester Containers

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Solution Overview

Problem

Existing oxygen scavenging compositions for PET containers suffer from intrinsic viscosity (IV) loss during processing, leading to reduced durability and effectiveness in blocking oxygen ingress, which affects the packaging of sensitive materials like food and beverages.

Innovation Solution

A composition comprising a polyester base polymer, a polyether polyol at 0.3-0.7 wt.%, a chain extending agent, and a transition metal in a positive oxidation state, which maintains IV and enhances oxygen scavenging properties without inducing an oxygen scavenging delay in blow molded containers.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If poly(alkylene glycol) and transition metal catalyst are blended into PET for oxygen scavenging, then oxygen scavenging effectiveness is improved, but intrinsic viscosity is degraded leading to poor melt extruding and blow molding performance

Engineering Contradiction:
Improveoxygen scavenging effectivenessVSAvoidintrinsic viscosity
Core Design Contradiction:
ReliabilityVSManufacturing precision

Solution Approach 1:

The patent changes the concentration parameter of poly(alkylene glycol) from typical higher levels to a specific range of 0.05-2 wt.%, which fundamentally alters the chemical reaction dynamics. This parameter change prevents excessive chain cleavage while maintaining sufficient oxygen scavenging capacity, thereby preserving intrinsic viscosity and manufacturing performance

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent introduces a spatial distribution strategy by incorporating the poly(alkylene glycol) and transition metal catalyst throughout the PET matrix at controlled concentrations. This creates localized oxygen scavenging zones that are sufficient for protection without causing widespread degradation of the polymer chains, thus maintaining overall material quality and processability

Inventive Principle:
Principle #3Local quality

2Object-affected harmful factors

If poly(alkylene glycol) is blended into PET for oxygen scavenging, then oxygen permeation is reduced, but container durability and impact resistance are reduced

Engineering Contradiction:
Improveoxygen permeationVSAvoidcontainer durability
Core Design Contradiction:
Object-affected harmful factorsVSStrength

Solution Approach 1:

By precisely controlling the poly(alkylene glycol) concentration at 0.05-2 wt.%, the patent achieves optimal balance between oxygen barrier properties and mechanical strength. This parameter optimization ensures that enough scavenger is present to block oxygen permeation while preventing excessive chain scission that would compromise container durability and impact resistance

Inventive Principle:
Principle #35Parameter changes

3Reliability

If modified copolymer with polypropylene oxide oligomers is used for oxygen scavenging, then oxygen scavenging is achieved, but processing complexity and material cost increase

Engineering Contradiction:
Improveoxygen scavengingVSAvoidmaterial composition complexity
Core Design Contradiction:
ReliabilityVSDevice complexity

Solution Approach 1:

The patent extracts the essential oxygen scavenging function from complex modified copolymer systems and implements it through a simpler formulation: pure PET base polymer combined with poly(alkylene glycol) and transition metal catalyst. This extraction maintains oxygen scavenging effectiveness while significantly reducing material composition complexity and processing difficulty

Inventive Principle:
Principle #2Taking out (Extraction)

Solution Approach 2:

The patent creates a functional composite material system combining PET, poly(alkylene glycol), and transition metal catalyst. This composite approach achieves oxygen scavenging through synergistic interaction of components rather than relying on complex copolymer structures, thereby simplifying the overall material system while maintaining effectiveness

Inventive Principle:
Principle #40Composite materials

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The solution effectively scavenges oxygen, maintaining container durability and preventing oxygen ingress, thereby extending the shelf life of sensitive products without compromising processing integrity.

Implementation Method 1

polymers capable of undergoing metal catalyzed oxidation such as m-xylylene diamine adipate or polybutadiene, oxidizable metals such as iron, or reduced anthraquinones

Methodology Applied
Scientific EffectOxidation: Oxidation

Implementation Method 2

at least one transition metal in a positive oxidation state

Methodology Applied
Scientific EffectCatalysis: Catalysis

Data Source

PatentEP3250640B1Durable oxygen scavenging plastic containers
Publication Date: 2019.03.13 GRAHAM PACKAGING CO LP
  • EP3250640B1 patent drawingFigure 1~2
  • EP3250640B1 patent drawingFigure 3~4
  • EP3250640B1 patent drawingFigure 5~6

AI summary

The present invention provides a wall for a package comprising at least one layer, the layer comprising a composition, the composition comprising: a polyester base polymer; at least one polyether polyol at a concentration of from 0.3 to 0.7 wt. %; and at least one transition metal in a positive oxidation state, the metal being present in the composition in an amount of from 10 to 400 ppm.