Particulate Vanadium Oxide Desulfurization Catalyst

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Solution Overview

Problem

Existing desulfurization catalysts for catalytic cracked gasoline have low desulfurization activity and cracking efficiency, and they often lead to increased generation of hydrogen and coke due to the destruction of zeolite structures by vanadium, which reduces their effectiveness.

Innovation Solution

A desulfurization catalyst comprising porous spherical particles of inorganic oxide containing particulate vanadium oxide, with an average diameter of 0.1 to 10 μm and a vanadium oxide content of 0.3 to 3 weight %, along with antimony, which maintains high cracking activity and suppresses hydrogen and coke generation by distributing vanadium oxide in a particulate state and enhancing sulfur compound affinity.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If oxidized vanadium metal is used as desulfurization catalyst, then desulfurization capability is improved, but cracking activity decreases due to destruction of molecular sieve crystalline structure

Engineering Contradiction:
Improvedesulfurization capabilityVSAvoidcracking activity
Core Design Contradiction:
ReliabilityVSProductivity

Solution Approach 1:

The patent changes the physical state parameter of vanadium from oxidized/cationic form to particulate metallic form with specific size (0.1-10 μm). This parameter change allows vanadium to maintain desulfurization capability while avoiding destruction of the molecular sieve crystalline structure, thus preserving cracking activity.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent applies local quality by distributing vanadium oxide as discrete particulate matter (0.1-10 μm) throughout the catalyst rather than as a homogeneous oxidized phase. This localized particulate distribution enables desulfurization function while minimizing structural damage to the molecular sieve.

Inventive Principle:
Principle #3Local quality

2Adaptability or versatility

If vanadium is homogeneously carried on inorganic porous carrier, then desulfurization function is provided, but affinity with sulfur compounds is low resulting in low desulfurization activity

Engineering Contradiction:
Improvedesulfurization functionVSAvoiddesulfurization activity
Core Design Contradiction:
Adaptability or versatilityVSReliability

Solution Approach 1:

The patent changes the distribution parameter of vanadium from homogeneous to particulate (0.1-10 μm). This creates localized high-concentration zones of vanadium that significantly enhance affinity with sulfur compounds and desulfurization activity while maintaining the overall desulfurization function.

Inventive Principle:
Principle #35Parameter changes

3Productivity

If Y-zeolite is used as FCC catalyst, then cracking activity is maintained, but sulfur content removal effect is insufficient without additional vanadium

Engineering Contradiction:
Improvecracking activityVSAvoidsulfur content removal effect
Core Design Contradiction:
ProductivityVSReliability

Solution Approach 1:

The patent creates a composite catalyst system combining Y-zeolite (for cracking activity) with particulate vanadium oxide (for desulfurization). The composite structure allows both functions to coexist: Y-zeolite maintains cracking activity while particulate vanadium oxide provides effective sulfur removal through its high affinity and particulate distribution.

Inventive Principle:
Principle #40Composite materials

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The catalyst achieves high desulfurization activity and maintains cracking efficiency while minimizing hydrogen and coke production, as the particulate vanadium oxide and antimony effectively manage sulfur compound removal and zeolite stability during catalytic cracking.

Implementation Method 1

the catalyst has high affinity with sulfur compounds, so that the activity for desulfurization is high

Methodology Applied
Scientific EffectAdsorption: Adsorption

Implementation Method 2

desulfurization catalyst for catalytic cracked gasoline containing particulate vanadium oxide

Methodology Applied
Scientific EffectCatalysis: Catalysis

Implementation Method 3

porous spherical particles of inorganic oxide containing particulate vanadium oxide

Methodology Applied
Scientific EffectPorosity: Porosity

Implementation Method 4

the catalyst achieves high desulfurization activity and maintains cracking efficiency while minimizing hydrogen and coke production

Methodology Applied
Scientific EffectCatalysis: Catalysis

Data Source

PatentUS8048293B2Desulfurization catalyst for catalytic cracked gasoline and method for desulfurizing catalytic cracked gasoline using the same
Publication Date: 2011.11.01 JGC CATALYSTS & CHEMICALS LTD

AI summary

The desulfurization catalyst for catalytic cracked gasoline according to the present invention has high performance in removal of sulfur compounds in gasoline fractions. This catalyst contains particulate vanadium oxide having the average particle diameter in the range from 0.1 to 10 μm at the content in the range from 0.3 to 3 weight % calculated as that of V2O5. The porous spherical particles of inorganic oxide are made of crystalline aluminosilicate zeolite and a porous inorganic oxide matrix, and furthermore contain antimony.