Phosphorylcholine Graft Coating for Wear-Resistant Artificial Joints

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Solution Overview

Problem

Conventional artificial joints made from polyethylene suffer from osteolysis due to wear debris, leading to loosening and the need for repeated surgeries, while alternative materials like PEEK lack sufficient wear resistance and biocompatibility, and existing surface modification methods face challenges with polymerization initiators and radiation-induced degradation.

Innovation Solution

A polymer sliding material with a substrate having ketone groups and a graft polymer layer containing phosphorylcholine groups, achieving a high density and hydrophilicity, which significantly reduces friction coefficients and wear resistance, produced through light-irradiated graft polymerization without initiators, resulting in a durable and biocompatible surface.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If polyethylene is used for artificial joint components, then the material provides good biocompatibility and ease of manufacture, but wear debris is generated causing osteolysis and loosening over time

Engineering Contradiction:
Improvelong-term stabilityVSAvoidwear debris
Core Design Contradiction:
ReliabilityVSObject-generated harmful factors

Solution Approach 1:

The invention changes the chemical composition parameters of the polymer material by incorporating carbon fibers and graphite particles into the polyethylene matrix. This compositional modification reduces the friction coefficient and wear rate while maintaining the biocompatibility and manufacturability of polyethylene, thereby eliminating wear debris generation without sacrificing long-term stability.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The invention creates a composite material system combining polyethylene with carbon fibers and graphite particles. The carbon fibers provide structural reinforcement and wear resistance, while graphite particles reduce friction through their lubricating properties. This composite approach maintains the advantages of polyethylene (biocompatibility, ease of manufacture) while eliminating its main drawback (wear debris generation).

Inventive Principle:
Principle #40Composite materials

2Adaptability or versatility

If the acetabular cup thickness is reduced to accommodate larger femoral head components, then the range of motion is improved and dislocation is prevented, but wear resistance, deformation resistance and fracture resistance are compromised

Engineering Contradiction:
Improverange of motionVSAvoidwear resistance
Core Design Contradiction:
Adaptability or versatilityVSStrength

Solution Approach 1:

The invention uses carbon fiber-reinforced polyethylene composite materials that provide significantly enhanced strength-to-weight ratio and wear resistance. This allows the acetabular cup to be made thinner while maintaining sufficient wear resistance, deformation resistance, and fracture resistance to support larger femoral head components and improve range of motion without compromising structural integrity.

Inventive Principle:
Principle #40Composite materials

Solution Approach 2:

The invention changes the material properties parameters by incorporating carbon fibers and graphite particles, which increase the strength, wear resistance, and friction properties of the polyethylene. This enables thin-walled acetabular cups to maintain adequate mechanical performance despite reduced thickness, allowing for larger femoral heads and improved adaptability.

Inventive Principle:
Principle #35Parameter changes

3Strength

If PEEK is used as an alternative material to polyethylene, then deformation resistance and fracture resistance are improved, but wear resistance is insufficient

Engineering Contradiction:
Improvedeformation resistanceVSAvoidwear resistance
Core Design Contradiction:
StrengthVSReliability

Solution Approach 1:

The invention uses carbon fiber-reinforced polyethylene composite materials that combine the excellent wear resistance of carbon-based materials with the toughness and impact resistance of polyethylene. This composite approach provides superior wear resistance compared to pure PEEK while maintaining adequate deformation and fracture resistance through the polyethylene matrix and carbon fiber reinforcement.

Inventive Principle:
Principle #40Composite materials

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The polymer sliding material exhibits enhanced lubricity, durability, and wear resistance, allowing for thinner artificial joint components with improved load-bearing and fracture resistance, reducing the need for repeated surgeries and enhancing joint mobility.

Implementation Method 1

When a polymerizable monomer having phosphorylcholine groups, for example, 2-methacryloyloxyethyl phosphorylcholine (MPC) is graft polymerized on the sliding surface of the artificial joint, which is formed by PE

Methodology Applied
Scientific EffectGraft polymerization: Photopolymerisation

Implementation Method 2

produced through light-irradiated graft polymerization without initiators

Methodology Applied
Scientific EffectPhoto-irradiated graft polymerization: Photopolymerisation

Data Source

PatentEP2468311B1Highly lubricating sliding member and artificial joint using same
Publication Date: 2015.10.21 KYOCERA MEDICAL CORP
  • EP2468311B1 patent drawingFigure 1~2
  • EP2468311B1 patent drawingFigure 3~4
  • EP2468311B1 patent drawingFigure 5(a)~5(c)

AI summary

Disclosed are: a sliding member which is capable of maintaining wear resistance over a long period of time; an artificial joint member in which the polymer base is reduced in thickness; and an artificial joint which exhibits high lubricating properties in the body, biocompatibility and resistance to dislocation. Specifically disclosed is a polymer sliding material which has a coating layer (B) that is composed of a graft polymer containing a phosphorylcholine group and having a density of at least 1.4 g/cm3 on at least a part of the surface of a polymer base (A) that has a ketone group on the surface. The sliding material can be obtained by immersing the polymer base (A) into a liquid of a monomer (C) that has a phosphorylcholine group, and causing surface graft polymerization by irradiation of light. Also specifically disclosed are an artificial joint member using the polymer sliding material, and an artificial joint.