Pd-Co Nitride Electrocatalyst for Fuel Cell Oxygen Reduction

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Solution Overview

Problem

Conventional fuel cells rely on expensive noble metals like platinum for high performance, limiting cost-effective alternatives with non-platinum metals exhibiting lower catalytic activities and onset potentials for oxygen reduction reactions.

Innovation Solution

Development of Pd-containing metal nitride electrocatalysts with specific molar ratios of Co, Fe, Y, Lu, Sc, Ti, V, Cu, or Ni, which offer higher onset potentials and catalytic activities, reducing energy consumption and improving fuel cell efficiency.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If noble metals like platinum are used as electrocatalysts, then catalytic activity and anti-corrosive properties are improved, but cost increases significantly

Engineering Contradiction:
Improveanti-corrosive propertiesVSAvoidcost
Core Design Contradiction:
ReliabilityVSQuantity of substance

Solution Approach 1:

The patent changes the chemical composition parameters by replacing platinum with palladium-based metal nitride compounds, adjusting the metal-to-Pd molar ratio to optimize both catalytic activity and cost-effectiveness while maintaining anti-corrosive properties in fuel cell environments

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent employs composite material strategy by creating Pd-containing metal nitride compounds that combine palladium with other metals (Co, Fe, Y, Lu, Sc, Ti, V, Cu, or Ni) to achieve synergistic effects that mimic or exceed platinum's performance at lower cost

Inventive Principle:
Principle #40Composite materials

2Quantity of substance

If non-platinum metals are used as electrode materials, then cost is reduced, but catalytic activity and onset potential of oxygen reduction reaction deteriorate

Engineering Contradiction:
ImprovecostVSAvoidcatalytic activity
Core Design Contradiction:
Quantity of substanceVSProductivity

Solution Approach 1:

The patent optimizes the metal-to-Pd molar ratio parameter (greater than 0 and less than or equal to 0.8) to enhance catalytic activity and onset potential of the oxygen reduction reaction, achieving performance comparable to or exceeding conventional catalysts while using cost-effective non-platinum metal compositions

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent applies local quality principle by selectively incorporating specific metals (Co, Fe, Y, Lu, Sc, Ti, V, Cu, or Ni) into the Pd-containing nitride structure to create localized active sites with enhanced catalytic properties for the oxygen reduction reaction

Inventive Principle:
Principle #3Local quality

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The Pd-containing metal nitride electrocatalysts demonstrate enhanced oxygen reduction reaction performance, comparable to platinum, while being more cost-effective, thus improving fuel cell operation efficiency and expanding suitable electrode material options.

Implementation Method 1

the performance of fuel cells depends on their electrocatalysts... development of a non-platinum electrocatalyst with a higher onset potential of the oxygen reduction reaction and a higher catalytic activity

Methodology Applied
Scientific EffectCatalysis: Catalysis

Data Source

PatentUS10566631B2Electrocatalyst and fuel cell employing the same
Publication Date: 2020.02.18 IND TECH RES INST

AI summary

An electrocatalyst is provided. The electrocatalyst includes Pd-containing metal nitride, wherein the metal is Co, Fe, Y, Lu, Sc, Ti, V, Cu, Ni, or a combination thereof. The molar ratio between the metal and Pd is greater than 0 and less than or equal to 0.8. A fuel cell utilizing the above electrocatalyst is further provided.