Polycrystalline Diamond Compacts With Interstitial Grains

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Solution Overview

Problem

Conventional polycrystalline diamond (PCD) compacts face challenges with thermal stability due to the presence of catalyst materials, which can cause back-conversion of diamond to softer carbon allotropes and induce stress, leading to decreased toughness and abrasion resistance, especially at elevated temperatures.

Innovation Solution

Incorporating interstitial diamond grains and metal carbides within the interstitial pockets of the PCD compacts, formed during the HPHT sintering process, reduces the contact area between diamond grains and catalyst material, thereby minimizing back-conversion and stress, and enhancing thermal stability.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Strength

If catalyst material is present in the PCD compact to promote inter-diamond bonding during HPHT process, then bonding strength is improved, but thermal stability deteriorates due to back-conversion and stress induction

Engineering Contradiction:
Improveinter-diamond bonding strengthVSAvoidthermal stability
Core Design Contradiction:
StrengthVSStability of the object's composition

Solution Approach 1:

The patent removes catalyst material from interstitial pockets between diamond grains after the HPHT bonding process is complete. This extraction eliminates the source of thermal instability (back-conversion and stress) while preserving the bonding strength already achieved during the HPHT process. The catalyst is taken out selectively from regions where it causes harm rather than removing it entirely from the system.

Inventive Principle:
Principle #2Taking out (Extraction)

Solution Approach 2:

The patent segments the catalyst removal process into specific regions - targeting only the interstitial pockets between diamond grains for catalyst removal while leaving catalyst in other regions. This selective segmentation allows removal of harmful catalyst portions while maintaining the bonding function where catalyst is still present.

Inventive Principle:
Principle #1Segmentation

2Stability of the object's composition

If catalyst material is removed from interstitial pockets to reduce stress and back-conversion, then thermal stability is improved, but complete removal becomes difficult

Engineering Contradiction:
Improvethermal stabilityVSAvoidcatalyst removal difficulty
Core Design Contradiction:
Stability of the object's compositionVSEase of manufacture

Solution Approach 1:

The patent performs catalyst removal as a preliminary or subsequent step after HPHT bonding but before final product completion. By timing the removal operation at this specific stage, the process takes advantage of the already-formed diamond grain structure to selectively access and remove catalyst from interstitial pockets more effectively than if attempted at other stages.

Inventive Principle:
Principle #10Preliminary action

Solution Approach 2:

The patent employs an intermediary substance or method to facilitate catalyst removal from interstitial pockets. This intermediary enables selective extraction of catalyst without requiring complete disassembly or destruction of the diamond grain structure, making the removal process practically feasible.

Inventive Principle:
Principle #24Intermediary (Mediator)

3Ease of manufacture

If catalyst material remains in interstitial pockets, then manufacturing simplicity is maintained, but diamond grains undergo back-conversion to softer carbon allotropes at elevated temperatures

Engineering Contradiction:
Improvemanufacturing simplicityVSAvoidabrasion resistance
Core Design Contradiction:
Ease of manufactureVSReliability

Solution Approach 1:

The patent extracts catalyst material specifically from interstitial pockets where it contacts diamond grains and promotes back-conversion. This selective extraction maintains manufacturing feasibility while eliminating the specific harmful effect of catalyst-induced back-conversion that degrades abrasion resistance.

Inventive Principle:
Principle #2Taking out (Extraction)

Solution Approach 2:

The patent applies different catalyst presence conditions to different regions: catalyst is removed from interstitial pockets surrounding diamond grains (where it causes harm) but may remain in other regions where it serves useful functions. This local differentiation of catalyst presence optimizes both reliability and manufacturability.

Inventive Principle:
Principle #3Local quality

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The introduction of interstitial diamond grains and metal carbides increases the thermal stability and wear performance of PCD compacts by reducing the volume of catalyst material and minimizing the surface area contact with the catalyst, resulting in improved performance at elevated temperatures.

Implementation Method 1

The polycrystalline diamond body may be formed in a high pressure high temperature (HPHT) process, in which diamond grains are held at pressures and temperatures at which the diamond particles bond to one another.

Methodology Applied
Scientific EffectHigh pressure high temperature sintering: Sintering

Implementation Method 2

the diamond particles are introduced to the HPHT process in the presence of a catalyst material that, when subjected to the conditions of the HPHT process, promotes formation of inter-diamond bonds

Methodology Applied
Scientific EffectCatalysis: Catalysis

Implementation Method 3

Some of the diamond grains may undergo a back-conversion to a softer non-diamond allotrope of carbon (for example, graphite or amorphous carbon) at elevated temperatures

Methodology Applied
Scientific EffectBack-conversion to graphite: Phase Change

Implementation Method 4

mismatch of the coefficients of thermal expansion between diamond and the catalyst may induce stress into the diamond lattice causing microcracks in the diamond body

Methodology Applied
Scientific EffectThermal expansion mismatch: Thermal Expansion

Data Source

PatentEP3416927B1Methods of making of polycrystalline diamond compacts having interstitial diamond grains
Publication Date: 2024.01.03 DIAMOND INNOVATIONS INC
  • EP3416927B1 patent drawingFigure 1~2
  • EP3416927B1 patent drawingFigure 3
  • EP3416927B1 patent drawingFigure 4

AI summary

Polycrystalline diamond compacts having interstitial diamonds and methods of forming polycrystalline diamond compact shaving interstitial diamonds with a quench cycle are described herein. In one embodiment, a polycrystalline diamond compact includes a substrate and a polycrystalline diamond body attached to the substrate. The polycrystalline diamond body includes a plurality of inter-bonded diamond grains that are attached to one another in an interconnected network of diamond grains and interstitial pockets between the inter-bonded diamond grains, and a plurality of interstitial diamond grains that are positioned in the interstitial pockets. Each of the plurality of interstitial diamond grains are attached to a single diamond grain of the interconnected network of diamond grains or other interstitial diamond grains.