Peroxidic Fluoropolyether Carboxylate Microemulsion for Stable Polymerization

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Solution Overview

Problem

Conventional surfactants like perfluorooctane sulfonate (PFOS) and perfluorooctanoic acid (PFOA) in microemulsions result in large particle sizes and instability during polymerization reactions, leading to unsafe explosive polymerization, especially in tetrafluoroethylene polymerization processes.

Innovation Solution

A microemulsion using peroxidic fluoropolyether carboxylate as an emulsifier, with a specific molecular structure and weight ratio of water to oil, is developed, allowing for the formation of stable microemulsions with smaller particle sizes and improved stability, suitable for polymerization reactions such as dispersion and emulsion polymerization of fluoropolymers.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Stability of the object's composition

If conventional surfactants (PFOS, PFOA, fluoropolyether) are used in microemulsion, then the microemulsion can be formed, but the particle size becomes large (150-300 nm) and the microemulsion becomes unstable during polymerization

Engineering Contradiction:
Improvemicroemulsion stabilityVSAvoidparticle size control
Core Design Contradiction:
Stability of the object's compositionVSManufacturing precision

Solution Approach 1:

The patent changes the chemical structure parameters of the surfactant by introducing peroxidic groups and specific fluoropolyether chains with controlled molecular weight (300-5000), which fundamentally alters the micelle formation and stabilizes the microemulsion at smaller particle sizes (30-150 nm) during polymerization

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent uses a composite surfactant system combining peroxidic groups with fluoropolyether chains, creating a synergistic effect that provides both steric stabilization and controlled micelle formation, resulting in stable microemulsions with uniform small particles suitable for polymerization

Inventive Principle:
Principle #40Composite materials

2Ease of manufacture

If conventional surfactants are used, then microemulsion can be formed, but violent stirring destroys the micelles and causes unsafe explosive polymerization

Engineering Contradiction:
Improvemicroemulsion formationVSAvoidpolymerization safety
Core Design Contradiction:
Ease of manufactureVSReliability

Solution Approach 1:

The peroxidic fluoropolyether carboxylate surfactant provides beforehand cushioning by forming a protective interface that prevents violent stirring from destroying micelles, thereby preventing unsafe explosive polymerization before it can occur

Inventive Principle:
Principle #11Beforehand cushioning (Prior cushioning)

Solution Approach 2:

The patent employs a surfactant with specific peroxidic and ether linkages that can be easily decomposed or replaced, providing a safe alternative that prevents explosive polymerization without requiring complex stabilization mechanisms

Inventive Principle:
Principle #27Cheap short-living objects (Disposable)

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The microemulsion achieves particle sizes of 30-150 nm, enhancing the stability and purity of polytetrafluoroethylene and fluoro-rubber products, reducing viscosity, and improving processing properties like film-forming and moulding operations.

Implementation Method 1

a microemulsion using peroxidic fluoropolyether carboxylate as emulsifier... the formation of a microemulsion mainly depends on the matching of each component in the system. The factors determining the stability of a microemulsion mainly are the kinds of the surfactants

Methodology Applied
Scientific EffectSurfactant: Surfactant

Data Source

PatentUS9101892B2Preparation method and use for fluorine-containing microemulsion
Publication Date: 2015.08.11 ZHONGHAO CHENGUANG RES INST OF CHEMICALINDUSTRY CO LTD

AI summary

A microemulsion consisting of water, peroxidic fluoropolyether carboxylate and oil is provided. When the microemulsion is used in homopolymerization, binary copolymerization or multi-component copolymerization of fluorine-containing olefin monomers, an emulsion with a low viscosity and a particle diameter of 30-200 nm can be obtained.