PET Container Creep Control and Gas Barrier via Silane Crosslinking

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Solution Overview

Problem

Polyethylene terephthalate (PET) containers have limitations due to high permeability to carbon dioxide, which affects the shelf life of carbonated beverages and restricts their use in smaller sizes and oxygen-sensitive products, while existing enhancements often compromise mechanical properties or clarity.

Innovation Solution

A polyester container composition incorporating a creep control agent and a gas barrier additive, specifically designed to enhance mechanical properties and reduce gas permeability without degrading stretch ratio or clarity, comprising compounds like cyclobutane-1,2,3,4-tetracarboxylic acid dianhydride and bisoxazoline, present in controlled amounts within the PET composition.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If PET containers are used for carbonated beverages, then mechanical properties and clarity are maintained, but gas barrier properties deteriorate due to high carbon dioxide permeability

Engineering Contradiction:
Improvegas barrier propertiesVSAvoidcarbon dioxide permeability
Core Design Contradiction:
ReliabilityVSObject-generated harmful factors

Solution Approach 1:

The patent introduces silane-crosslinked polyester as an intermediary material that modifies the PET structure to reduce gas permeability. The silane groups form a crosslinked network within the polyester matrix, creating a more tortuous path for carbon dioxide molecules to traverse, thereby improving the gas barrier properties while maintaining the inherent mechanical properties and clarity of PET containers.

Inventive Principle:
Principle #24Intermediary (Mediator)

2Volume of moving object

If smaller PET container sizes are used, then surface area to volume ratio increases, but carbon dioxide loss rate increases due to higher relative permeability

Engineering Contradiction:
Improvecontainer sizeVSAvoidcarbon dioxide loss
Core Design Contradiction:
Volume of moving objectVSLoss of substance

Solution Approach 1:

The patent changes the chemical and physical parameters of the PET material by incorporating silane groups that undergo crosslinking. This modification alters the polymer matrix density and free volume, reducing the permeability parameter to carbon dioxide. As a result, smaller containers experience reduced relative carbon dioxide loss rates, extending shelf life without requiring larger container sizes.

Inventive Principle:
Principle #35Parameter changes

3Strength

If chain extenders are added to improve creep resistance, then mechanical properties are enhanced, but gas barrier properties and clarity may deteriorate

Engineering Contradiction:
Improvecreep resistanceVSAvoidgas barrier properties
Core Design Contradiction:
StrengthVSReliability

Solution Approach 1:

The patent creates a composite polyester system combining conventional PET with silane-modified polyester components. The silane-crosslinked segments act as reinforcing elements within the polymer matrix, providing creep resistance through enhanced molecular network structure. Simultaneously, the crosslinked network reduces gas permeability by creating a more dense and tortuous path for carbon dioxide molecules, thus improving gas barrier properties without compromising clarity.

Inventive Principle:
Principle #40Composite materials

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The solution significantly improves the gas barrier properties and reduces creep in PET containers, extending the shelf life of carbonated beverages and enabling their use in smaller sizes without compromising mechanical properties or visual appearance.

Implementation Method 1

the PET bottle will slowly expand with time due to the creep of PET molecules under pressure

Methodology Applied
Scientific EffectCreep: Creep

Implementation Method 2

The permeability of PET to carbon dioxide and the degree of bottle expansion due to PET molecule creep therefore determines the shelf life of the packaged carbonated beverage

Methodology Applied
Scientific EffectPermeation: Permeation

Data Source

PatentEP2358804B1Pet container and compositions having enhanced mechanical properties and gas barrier properties
Publication Date: 2020.02.05 THE COCA COLA CO
  • EP2358804B1 patent drawingFigure 1
  • EP2358804B1 patent drawingFigure 2~4
  • EP2358804B1 patent drawingFigure 5

AI summary

A container comprising a polyester composition with enhanced mechanical properties is provided. The polyester composition comprises a polyester and a creep control agent. In particular embodiments, the polyester composition comprises a polyester, a creep control agent, and a gas barrier additive. In particular embodiments, the creep control agents are molecules or polymers comprising dianhydrides, bis-lactams, bis-oxazoles, and epoxides.