Supercritical CO2 Extraction of PFPE Oil from Grease Matrices

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Solution Overview

Problem

There is a need for a cost-effective and environmentally friendly process to separate and recover perfluoropolyether (PFPE) oil from lubricating greases, as existing methods are inefficient and generate waste, particularly in aerospace applications where high-temperature performance and chemical stability are critical.

Innovation Solution

A process involving the use of liquid or supercritical carbon dioxide as a solvent, combined with an extraction aid material, to extract PFPE oil from lubricating greases, ensuring minimal contamination from thickeners and other additives, with a yield of at least 75 wt% and minimal thickener content in the recovered oil.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Manufacturing precision

If traditional multi-stage extraction processes are used to extract PFPE from lubricating grease, then extraction completeness may be improved, but process complexity and cost increase significantly

Engineering Contradiction:
Improveextraction completenessVSAvoidprocess complexity
Core Design Contradiction:
Manufacturing precisionVSDevice complexity

Solution Approach 1:

The patent extracts the valuable PFPE oil from the grease matrix using a simple single-stage extraction process with supercritical CO2, removing only the necessary component without requiring complex multi-stage processes. The supercritical fluid selectively dissolves the PFPE oil while leaving the thickener and additives behind, achieving effective separation in one step.

Inventive Principle:
Principle #2Taking out (Extraction)

Solution Approach 2:

The patent utilizes parameter changes by transitioning CO2 from gaseous to supercritical state through controlled pressure and temperature adjustments. This single parameter change enables the solvent to penetrate the grease matrix effectively and selectively extract PFPE oil, simplifying the overall extraction process while maintaining high completeness.

Inventive Principle:
Principle #35Parameter changes

2Quantity of substance

If conventional extraction methods are used, then PFPE oil can be recovered, but environmental pollution and waste generation occur

Engineering Contradiction:
ImprovePFPE oil recoveryVSAvoidenvironmental pollution
Core Design Contradiction:
Quantity of substanceVSObject-generated harmful factors

Solution Approach 1:

The patent converts the typically harmful or wasteful extraction process into an environmentally beneficial operation. By using supercritical CO2, a non-toxic and recyclable solvent, the process eliminates the need for harmful organic solvents. The CO2 can be recovered and reused, transforming what would be waste into a beneficial循环 resource, thus recovering PFPE oil without environmental pollution.

Inventive Principle:
Principle #22Blessing in disguise (Convert harm into benefit)

Solution Approach 2:

The patent replaces conventional mechanical or chemical extraction methods that generate waste with a supercritical fluid extraction system. The supercritical CO2 acts as a clean alternative to traditional solvents, providing effective PFPE oil recovery without the harmful byproducts or waste streams associated with conventional methods.

Inventive Principle:
Principle #28Mechanics substitution (Replace mechanical system)

3Productivity

If simple extraction processes are used, then cost and time are reduced, but extraction yield and purity decrease

Engineering Contradiction:
Improveextraction efficiencyVSAvoidextraction purity
Core Design Contradiction:
ProductivityVSManufacturing precision

Solution Approach 1:

The patent exploits phase transitions of CO2 between gaseous and supercritical states to achieve both high extraction yield and purity in a single stage. By controlling pressure and temperature, the CO2 transitions to a supercritical state for effective extraction, then returns to gaseous state for easy separation and solvent recovery. This phase transition mechanism ensures complete PFPE oil extraction while maintaining high purity and enabling rapid process completion.

Inventive Principle:
Principle #36Phase transitions

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The process effectively separates and recovers PFPE oil with high yield and purity, maintaining its valuable properties, while being economically and environmentally sustainable, suitable for reuse in high-performance applications.

Implementation Method 1

contacting a solvent comprising a liquid or supercritical carbon dioxide with the lubricating grease comprising a thickener, an extraction aid material, and the perfluoropolyether in an extraction zone to form an extraction solution comprising an extracted perfluoropolyether

Methodology Applied
Scientific EffectSupercritical fluid extraction: Supercritical Fluid Extraction

Data Source

PatentEP3092044B1Recovery of perfluorinated polyether oils from grease matrices incorporating extraction aids by carbon dioxide extraction
Publication Date: 2021.03.03 THE CHEMOURS CO FC LLC
  • EP3092044B1 patent drawingFigure 1
  • EP3092044B1 patent drawingFigure 2~3

AI summary

This disclosure relates to a process for extracting a perfluoropolyether. The process involves: (a) contacting a solvent comprising a liquid or supercritical carbon dioxide with a lubricating grease comprising a thickener, an extraction aid material, and the perfluoropolyether in an extraction zone to form an extraction solution comprising an extracted perfluoropolyether; and (b) recovering the extracted perfluoropolyether from the extraction solution; wherein the recovered extracted perfluoropolyether comprises no more than about 2 wt % of the thickener.