Photocurable Composition for Nanoimprint Alignment Accuracy

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Solution Overview

Problem

In photonanoimprint technology, the alignment accuracy of patterns on semiconductor devices and MEMS is compromised due to thermal strain caused by exposure heat during photoirradiation, leading to pattern collapse defects when attempting to reduce exposure dose for lower heat generation.

Innovation Solution

A photocurable composition with a polymerizable compound and photopolymerization initiator is used, where the polymerizable compound has a polymerization conversion ratio of 50% or more under specific light exposure conditions, ensuring sufficient curing while minimizing thermal strain and pattern collapse.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Temperature

If exposure dose is reduced to minimize exposure heat, then thermal strain is reduced, but photocurable composition is not cured sufficiently leading to pattern collapse

Engineering Contradiction:
Improveexposure heatVSAvoidcuring completeness
Core Design Contradiction:
TemperatureVSReliability

Solution Approach 1:

The patent changes the chemical parameters of the photocurable composition by selecting specific polymerizable compounds with appropriate polymerization rates and photopolymerization initiators with suitable absorption characteristics. This allows the system to achieve sufficient curing at lower exposure doses, thereby reducing thermal strain while maintaining pattern integrity.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent uses composite photocurable compositions containing specific combinations of polymerizable compounds (acrylate, vinyl ether, vinyl silane) and photopolymerization initiators. This composite approach enables optimized curing characteristics that achieve complete polymerization at reduced exposure doses, resolving the contradiction between sufficient curing and heat generation.

Inventive Principle:
Principle #40Composite materials

2Reliability

If exposure dose is increased to ensure sufficient curing, then pattern collapse is prevented, but thermal strain increases reducing alignment accuracy

Engineering Contradiction:
Improvecuring completenessVSAvoidalignment accuracy
Core Design Contradiction:
ReliabilityVSManufacturing precision

Solution Approach 1:

The patent modifies the photoirradiation parameters by using photopolymerization initiators with specific absorption characteristics that allow efficient curing at lower exposure doses. This parameter optimization ensures complete curing while minimizing exposure heat generation, thereby maintaining alignment accuracy in adjacent regions.

Inventive Principle:
Principle #35Parameter changes

3Productivity

If high exposure dose is used for rapid curing, then productivity is improved, but thermal strain increases causing alignment errors in adjacent regions

Engineering Contradiction:
Improvecuring speedVSAvoidalignment accuracy
Core Design Contradiction:
ProductivityVSManufacturing precision

Solution Approach 1:

The patent changes the chemical composition parameters to include polymerizable compounds with high polymerization conversion ratios and photopolymerization initiators with appropriate absorption coefficients. This enables rapid curing at optimized exposure doses that balance productivity with minimal thermal strain, preventing alignment errors in adjacent regions.

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The method achieves high alignment accuracy and reduces pattern collapse defects by optimizing the photocurable composition's properties to balance curing efficiency and thermal strain, allowing for precise pattern formation on semiconductor devices and MEMS.

Implementation Method 1

a step of irradiating the photocurable composition with light to form a cured product

Methodology Applied
Scientific EffectPhotopolymerization: Photopolymerisation

Implementation Method 2

part of irradiation light is absorbed by the substrate, and hence heat (exposure heat) is generated in the substrate

Methodology Applied
Scientific EffectAbsorption (EM radiation): Absorption (EM radiation)

Data Source

PatentEP3017460B1Method of producing film, method of producing optical component, method of producing circuit board, method of producing electronic component, and photocurable composition
Publication Date: 2021.11.10 CANON KK
  • EP3017460B1 patent drawingFigure 1
  • EP3017460B1 patent drawingFigure 2A~2G
  • EP3017460B1 patent drawingFigure 3

AI summary

A method of producing a film includes: a disposing step of disposing a photocurable composition on a substrate; a mold contact step of bringing the photocurable composition and a mold into contact with each other; a photoirradiation step of irradiating the photocurable composition with light to form a cured product; and a mold release step of releasing the cured product and the mold from each other, in which the method further includes an alignment step of aligning the mold and the substrate with each other before the photoirradiation step, in which the photocurable composition contains at least a polymerizable compound serving as a component (A) and a photopolymerization initiator serving as a component (B), and in which the polymerizable compound has a polymerization conversion ratio of 50% or more when exposed to light under conditions of an illuminance of 0.12 mW/cm2 and an exposure time of 11.0 seconds.