Photoresist Stripping Solution for Selective Dissolution

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Solution Overview

Problem

Current resin stripping solutions for microelectronic component integration processes are ineffective in completely dissolving semi-novolac resins at temperatures below 100°C, leading to residual debris and potential defects, and often compromise the integrity of exposed metals like copper and aluminum.

Innovation Solution

A formulation using two ether or polyether solvents as the principal solvent, combined with an acid and minimal water content, which enables complete dissolution of photoresists at temperatures between 40 and 100°C while ensuring compatibility with metal interconnections and dielectrics, allowing for efficient recirculation and minimal substrate damage.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Manufacturing precision

If conventional resin stripping solutions are used, then resin can be removed at high temperatures, but the solutions fail to completely dissolve semi-novolac resins at temperatures below 100°C, leaving residual debris

Engineering Contradiction:
Improvecomplete dissolution of photoresistVSAvoidprocess temperature
Core Design Contradiction:
Manufacturing precisionVSTemperature

Solution Approach 1:

The patent modifies the chemical composition parameters of the stripping solution by incorporating specific ether solvents (diethylene glycol monobutyl ether, dipropylene glycol monomethyl ether) in optimized concentrations (70-95% v/v), combined with controlled amounts of acid (0.1-5% v/v) and water (0.1-30% v/v). This parameter optimization enables complete photoresist dissolution at reduced temperatures (40-100°C) while maintaining solution stability and effectiveness.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent creates a composite chemical formulation combining multiple solvent types (ether solvents, acids, and water) with complementary functions. The ether solvents provide photoresist swelling and dissolution capability, the acid enhances polymer matrix breakdown, and minimal water content prevents metal corrosion while maintaining solution homogeneity. This composite approach achieves complete dissolution at lower temperatures than conventional single-solvent systems.

Inventive Principle:
Principle #40Composite materials

2Productivity

If strong chemical agents are used to strip resin, then resin removal effectiveness improves, but the integrity of exposed metals such as copper and aluminum is compromised

Engineering Contradiction:
Improveresin stripping effectivenessVSAvoidchemical attack on metals
Core Design Contradiction:
ProductivityVSObject-affected harmful factors

Solution Approach 1:

The patent uses ether solvents as intermediary substances that mediate between the photoresist polymer matrix and the metal substrates. These solvents swell and dissolve the photoresist through hydrogen bonding and dipole interactions without directly attacking metal surfaces. The minimal water content (0.1-30% v/v) further reduces chemical aggressiveness while maintaining dissolution effectiveness, creating a buffered chemical environment that protects metals from corrosion.

Inventive Principle:
Principle #24Intermediary (Mediator)

Solution Approach 2:

The patent optimizes the concentration parameters of corrosive components by limiting acid content to 0.1-5% v/v and water content to 0.1-30% v/v, while maintaining high ether solvent content (70-95% v/v). This parameter control reduces the chemical potential for metal attack while preserving photoresist dissolution capability through the dominant ether solvent system.

Inventive Principle:
Principle #35Parameter changes

3Manufacturing precision

If photoresist stripping is performed, then surface quality improves, but the stripping solution requires frequent replacement due to particulate accumulation

Engineering Contradiction:
Improvesurface qualityVSAvoidstripping solution degradation
Core Design Contradiction:
Manufacturing precisionVSLoss of substance

Solution Approach 1:

The patent formulates a stripping solution with enhanced stability and complete dissolution capability that prevents particulate precipitation during extended use. The optimized ether solvent composition (70-95% v/v of diethylene glycol monobutyl ether and/or dipropylene glycol monomethyl ether) maintains photoresist in complete solution form, preventing filter clogging and solution degradation. This enables continuous recirculation and extends solution lifespan, maintaining surface quality consistency over prolonged operation.

Inventive Principle:
Principle #20Continuity of useful action

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The solution achieves complete dissolution of photoresists without damaging exposed metals, facilitating optimal surface quality and enabling the recirculation of stripping solutions, thus improving the performance and reliability of microelectronic component fabrication.

Implementation Method 1

A formulation using two ether or polyether solvents as the principal solvent, combined with an acid and minimal water content, which enables complete dissolution of photoresists at temperatures between 40 and 100°C

Methodology Applied
Scientific EffectSolvation: Solvation

Implementation Method 2

A formulation using two ether or polyether solvents as the principal solvent, combined with an acid

Methodology Applied
Scientific EffectChemical Bonding: Chemical Bonding

Data Source

PatentEP2718767B1Composition of solutions and conditions for use enabling the stripping and complete dissolution of photoresists
Publication Date: 2019.08.07 TECH FRANCE SA
  • EP2718767B1 patent drawingFigure 1~2

AI summary

The present invention relates to the formulation of a chemical, comprised of an ether solvent as the principal solvent, an ether or non-ether cosolvent, an acid, optionally a surfactant and optionally a corrosion inhibitor, dedicated to the complete and selective stripping by pure dissolution of photoresists (novolac and semi-novolac) of all thicknesses used in microelectronic component integration processes. Said solution is optimized to dissolve the polymer matrix while ensuring and protecting the physicochemical integrity of exposed materials such as metal interconnections (copper, aluminum), dielectrics (SiO2, MSQ, etc.) and adhesion and diffusion barriers (TiN, Ti, Ta, TaN, etc.). Furthermore, the singular cleaning properties and performance characteristics of these solutions make it possible to envisage the use thereof in a variety of industrial applications such as single wafer, batch, immersion and/or spray by simple adjustment of process time and temperature.