Plastic Scintillator Doped with Metal 2-Methylbutyrate

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Solution Overview

Problem

Existing plastic scintillators face challenges in incorporating metals like lithium, which are poorly soluble in non-polar media, limiting their scintillation performance and solubility, particularly for applications in detecting fast neutrons, thermal neutrons, and gamma rays.

Innovation Solution

The development of a plastic scintillator with a polymer matrix containing metallic 2-methylbutyrate, such as lithium 2-methylbutyrate, which exhibits high solubility in non-polar media, allowing for increased metal ion content and enhanced scintillation properties, including the use of metals like lithium, gadolinium, bismuth, and lead for improved detection capabilities.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Quantity of substance

If conventional carboxylates (e.g., lithium pivalate, lithium salicylate) are used to incorporate metal ions in plastic scintillators, then some solubility is achieved, but the solubility remains insufficient to reach optimal doping levels for enhanced scintillation performance

Engineering Contradiction:
Improvemetal ion contentVSAvoidsolubility in non-polar media
Core Design Contradiction:
Quantity of substanceVSEase of manufacture

Solution Approach 1:

The patent applies parameter changes by modifying the chemical structure of the carboxylate ligand from conventional options (pivalate, salicylate) to 2-methylbutyrate. This structural parameter change increases the solubility product of the metal carboxylate in non-polar polymer matrices, enabling higher metal ion concentrations to be achieved without precipitation or phase separation.

Inventive Principle:
Principle #35Parameter changes

Solution Approach 2:

The patent creates a composite material system combining the polymer matrix, fluorophores, and metal carboxylate dopants. By selecting 2-methylbutyrate as the carboxylate ligand, the composite achieves optimal compatibility between the polar metal carboxylate and non-polar polymer matrix, resolving the solubility contradiction while maintaining scintillation performance.

Inventive Principle:
Principle #40Composite materials

2Reliability

If higher metal ion content is incorporated to enhance scintillation performance, then detection capability improves, but solubility limitations prevent achieving optimal doping levels

Engineering Contradiction:
Improvedetection capabilityVSAvoidmetal ion solubility
Core Design Contradiction:
ReliabilityVSQuantity of substance

Solution Approach 1:

By changing the carboxylate ligand to 2-methylbutyrate, the patent increases the solubility parameter of the metal complex in the non-polar matrix. This enables higher metal ion concentrations (optimal doping levels) to be achieved, directly improving neutron and gamma ray detection capability through enhanced scintillation signal.

Inventive Principle:
Principle #35Parameter changes

3Ease of manufacture

If conventional carboxylates are used, then the scintillator maintains basic functionality, but the metal ion incorporation efficiency is limited by poor solubility

Engineering Contradiction:
Improvemetal incorporation efficiencyVSAvoidsolubility
Core Design Contradiction:
Ease of manufactureVSQuantity of substance

Solution Approach 1:

The patent changes the chemical parameter of the carboxylate ligand from conventional options to 2-methylbutyrate, which has superior solubility characteristics in non-polar media. This parameter change directly improves metal incorporation efficiency during the manufacturing process, allowing metal ions to be uniformly distributed at optimal concentrations without solubility constraints.

Inventive Principle:
Principle #35Parameter changes

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The high solubility of metallic 2-methylbutyrates enables the scintillator to be doped with higher metal ion contents, resulting in remarkable scintillation performances, transparency, chemical and mechanical stability, and ease of industrial-scale production, effectively enhancing detection and identification of neutrons and gamma rays.

Implementation Method 1

A plastic scintillator (also called plastic scintillator) is a fluorescent polymer material which has the capacity to emit photons, called scintillation photons, when excited by a particle or ionizing radiation.

Methodology Applied
Scientific EffectScintillation: Scintillation

Implementation Method 2

a so-called primary fluorophore, which has the role of transform electronic energy into fluorescent light

Methodology Applied
Scientific EffectFluorescence: Fluorescence

Implementation Method 3

a so-called secondary fluorophore, which plays the role of wavelength shifter (or 'wavelength shifter' in English) by absorbing the light emitted by the primary fluorophore and re-emitting it at a higher wavelength

Methodology Applied
Scientific EffectWavelength shifting: Fluorescence

Data Source

PatentEP3591025B1Plastic scintillator doped with metal ions and uses thereof
Publication Date: 2021.04.14 COMMISSARIAT A LENERGIE ATOMIQUE ET AUX ENERGIES ALTERNATIVES
  • EP3591025B1 patent drawingFigure 1~2
  • EP3591025B1 patent drawingFigure 3~4
  • EP3591025B1 patent drawingFigure 5A~5B

AI summary

The invention relates to a plastic scintillator comprising a polymer matrix containing at least one fluorophore and at least one metal carboxylate, characterized in that the metal carboxylate is a metal 2-methylbutyrate of formula (I): where M represents a metal selected from lithium, gadolinium, bismuth, lead, cadmium, tin, tungsten, mercury, and osmium, and n represents the oxidation state of metal M. The invention also relates to the uses of this plastic scintillator. Applications: any field of application for a plastic scintillator.