Multilayer Hydrogen Tank Liner Using Polyamide and Composite Reinforcement

Resolve Bottlenecks,
Find Innovative Solutions
Generate Solutions

Solution Overview

Problem

Current hydrogen tanks face challenges such as low thermal resistance, high permeability to hydrogen, and limited operating temperature range, which hinder efficient hydrogen storage and distribution, especially in high-pressure applications.

Innovation Solution

A multilayer structure comprising a sealing layer with short-chain or long-chain semi-crystalline polyamide thermoplastic polymers and a composite reinforcement layer impregnated with epoxy resin, which enhances mechanical strength and reduces hydrogen permeability, allowing for increased operating temperatures and filling speeds.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Ease of manufacture

If HDPE is used as the liner material, then the manufacturing process is simple and cost-effective, but the thermal resistance is insufficient and hydrogen permeability is too high

Engineering Contradiction:
Improvemanufacturing simplicityVSAvoidthermal resistance
Core Design Contradiction:
Ease of manufactureVSTemperature

Solution Approach 1:

The patent employs a composite liner structure consisting of multiple layers with distinct functions: an inner polyamide layer for hydrogen barrier properties, an intermediate adhesive layer for bonding, and an outer polyethylene layer for impact resistance and chemical resistance. This composite approach allows each layer to contribute its specific advantages, achieving both thermal resistance and manufacturing feasibility that single-material solutions cannot provide.

Inventive Principle:
Principle #40Composite materials

2Ease of manufacture

If HDPE is used as the liner material, then the manufacturing process is simple and cost-effective, but the hydrogen permeability is too high

Engineering Contradiction:
Improvemanufacturing simplicityVSAvoidhydrogen permeability
Core Design Contradiction:
Ease of manufactureVSLoss of substance

Solution Approach 1:

The patent employs a composite liner structure consisting of multiple layers with distinct functions: an inner polyamide layer for hydrogen barrier properties, an intermediate adhesive layer for bonding, and an outer polyethylene layer for impact resistance and chemical resistance. This composite approach allows each layer to contribute its specific advantages, achieving both thermal resistance and manufacturing feasibility that single-material solutions cannot provide.

Inventive Principle:
Principle #40Composite materials

Solution Approach 2:

The patent applies different materials to different regions of the liner structure based on local requirements: the inner layer contacts hydrogen and requires low permeability (polyamide), the intermediate layer requires adhesion (adhesive), and the outer layer requires mechanical and chemical resistance (polyethylene). This localized material assignment optimizes performance for each specific function while maintaining overall manufacturing efficiency.

Inventive Principle:
Principle #3Local quality

3Temperature

If PA6 is used as the liner material, then the thermal resistance is improved, but the resistance to cold is insufficient

Engineering Contradiction:
Improvethermal resistanceVSAvoidcold resistance
Core Design Contradiction:
TemperatureVSReliability

Solution Approach 1:

The patent employs a composite liner structure consisting of multiple layers with distinct functions: an inner polyamide layer for hydrogen barrier properties, an intermediate adhesive layer for bonding, and an outer polyethylene layer for impact resistance and chemical resistance. This composite approach allows each layer to contribute its specific advantages, achieving both thermal resistance and manufacturing feasibility that single-material solutions cannot provide.

Inventive Principle:
Principle #40Composite materials

4Productivity

If the filling speed is increased to match fuel tank refilling times, then the operating efficiency is improved, but the thermal resistance is exceeded due to heating

Engineering Contradiction:
Improvefilling speedVSAvoidthermal resistance
Core Design Contradiction:
ProductivityVSTemperature

Solution Approach 1:

The patent employs a composite liner structure consisting of multiple layers with distinct functions: an inner polyamide layer for hydrogen barrier properties, an intermediate adhesive layer for bonding, and an outer polyethylene layer for impact resistance and chemical resistance. This composite approach allows each layer to contribute its specific advantages, achieving both thermal resistance and manufacturing feasibility that single-material solutions cannot provide.

Inventive Principle:
Principle #40Composite materials

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The multilayer structure effectively reduces hydrogen permeability and increases the maximum usable temperature to 120°C, improving the efficiency and safety of hydrogen storage and distribution systems.

Implementation Method 1

Low permeability to hydrogen, indeed, the permeability of the liner is a key factor in limiting hydrogen losses from the tank

Methodology Applied
Scientific EffectPermeation: Permeation

Implementation Method 2

a structural layer made of fiber impregnated with thermoset resin surrounding said liner

Methodology Applied
Scientific EffectComposite materials: Composite Materials

Data Source

PatentUS12072062B2Multilayer structure for transporting or storing hydrogen
Publication Date: 2024.08.27 ARKEMA FRANCE SA

AI summary

A multilayer structure for transporting, distributing and storing hydrogen including, from the inside to the outside, a sealing layer and at least one composite reinforcement layer, the sealing layer including from the inside to the outside: a layer of a composition including: a short-chain polyamide thermoplastic polymer, more than 15% and up to 50% by weight of impact modifier, or including: a semi-crystalline long-chain polyamide thermoplastic polymer, up to 50% by weight of impact modifier, up to 3% by weight of plasticizer; a hydrogen barrier layer; a layer of a composition including: a short-chain polyamide thermoplastic polymer, more than 15% and up to 50% by weight of impact modifier, or including: a semi-crystalline long-chain polyamide thermoplastic polymer, up to 50% by weight of impact modifier, up to 3% of weight of plasticizer, the innermost composite reinforcement layer being wound around the sealing layer.