Polyamide Solid Phase Post-Condensation Gas Treatment

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Solution Overview

Problem

Existing processes for producing polyamides lack sufficient processing stability, leading to issues such as thermal degradation and increased viscosity during melt extrusion, which results in reduced throughput and increased contamination in film production.

Innovation Solution

A process involving solid phase post-condensation of polyamides with a gas mixture containing inert gases, water, acid, anhydride, lactone, ammonia, or amine at controlled temperatures and pressures, which reduces residual moisture and end-group imbalances, enhancing processing stability.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Productivity

If polyamide is processed during melt extrusion, then production throughput is increased, but thermal degradation and viscosity increase occur leading to processing instability

Engineering Contradiction:
Improveproduction throughputVSAvoidprocessing stability
Core Design Contradiction:
ProductivityVSReliability

Solution Approach 1:

The patent applies preliminary action by conducting solid phase post-condensation treatment before melt extrusion processing. This pre-treatment adjusts the end group ratio and reduces residual moisture in the polyamide granules, thereby preventing thermal degradation and viscosity increase during subsequent melt extrusion, ensuring processing stability while maintaining high throughput

Inventive Principle:
Principle #10Preliminary action

2Loss of substance

If polyamide undergoes solid phase post-condensation with inert gas only, then residual moisture is reduced, but end group imbalance persists causing processing issues

Engineering Contradiction:
Improveresidual moisture contentVSAvoidend group ratio stability
Core Design Contradiction:
Loss of substanceVSStability of the object's composition

Solution Approach 1:

The patent applies parameter changes by modifying the gas composition parameters during solid phase post-condensation. Instead of using only inert gas, the patent introduces reactive gases (oxygen at 0.1-10% or carbon dioxide at 1-50%) to change the chemical reaction parameters, enabling end group adjustment through controlled oxidation or carboxylation while simultaneously reducing residual moisture

Inventive Principle:
Principle #35Parameter changes

3Stability of the object's composition

If reactive gases are added to solid phase post-condensation, then end group balance is improved, but process complexity increases

Engineering Contradiction:
Improveend group ratioVSAvoidgas mixture control system
Core Design Contradiction:
Stability of the object's compositionVSDevice complexity

Solution Approach 1:

The patent applies local quality by making the gas composition adaptable to specific needs. The gas mixture can be customized based on the desired end group adjustment: oxygen-rich mixtures for amino end group reduction, or carbon dioxide-rich mixtures for carboxyl end group increase. This localized optimization simplifies the overall system by allowing selective gas composition rather than requiring complex continuous control

Inventive Principle:
Principle #3Local quality

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The process results in polyamides with improved stability during melt extrusion, reducing thermal degradation, viscosity, and monomer recovery, leading to increased production efficiency and reduced contamination in final products like films and fibers.

Implementation Method 1

the polyamide is treated during the solid phase post-condensation with a gas, the inert gas, water and acid or anhydride or lactone or their mixtures or ammonia or Contains amine or mixtures thereof

Methodology Applied
Scientific EffectAbsorption: Absorption (physical)

Implementation Method 2

solid phase post-condensation of polyamides with a gas mixture containing inert gases, water, acid, anhydride, lactone, ammonia, or amine at controlled temperatures and pressures

Methodology Applied
Scientific EffectCondensation: Condensation

Implementation Method 3

reduces residual moisture and end-group imbalances

Methodology Applied
Scientific EffectEvaporation: Evaporation

Data Source

PatentEP2614105B2Method for producing processing-stable polyamide
Publication Date: 2022.05.18 BASF SE

AI summary

The invention relates to a method for producing processing-stable polyamides, wherein the polyamide is treated with a gas that contains carrier gas (inert gas), water and acid or anhydride or lactone or mixtures thereof, or ammonia or amine or mixtures thereof, at a temperature of 130 to 200 °C and at a pressure of 0.01 to 10 bar during the solid phase post-condensation.