Polyamide Stabilization via Covalent Polyhydric Alcohol Bonding

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Solution Overview

Problem

Polyamide compositions used in various applications, such as motor vehicle parts, face instability under heat, light, and inclement weather, leading to degradation and loss of mechanical properties, and existing stabilization methods are either ineffective or costly, especially when polyhydric alcohols are added post-polymerization, which can lead to additional processing issues and reduced performance over time.

Innovation Solution

Incorporating a polyhydric alcohol, particularly one with aliphatic carbons, during the polyamide polymerization process to form covalent bonds within the polyamide chains, enhancing stability and preventing the 'washing' or extraction of the alcohol, thus providing improved heat, light, and weather resistance without the need for additional stabilization steps.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If polyhydric alcohol is added to polyamide as a mixture during extrusion, then heat stabilization is improved, but additional processing steps are required and the alcohol is readily extractable over time

Engineering Contradiction:
Improveheat stabilizationVSAvoidprocessing steps
Core Design Contradiction:
ReliabilityVSDevice complexity

Solution Approach 1:

The patent combines the polyhydric alcohol with polyamide monomers before polymerization, merging the stabilizer incorporation step with the polymerization process itself. This eliminates the need for separate extrusion and stabilization steps, resolving the contradiction between heat stabilization and processing complexity

Inventive Principle:
Principle #5Merging (Combining)

Solution Approach 2:

The polyhydric alcohol is incorporated into the polyamide structure during polymerization rather than added afterward. This preliminary action ensures the alcohol is covalently bonded to the polymer chains before the product is formed, preventing extraction and eliminating subsequent processing steps

Inventive Principle:
Principle #10Preliminary action

2Ease of operation

If polyhydric alcohol is added during polyamide synthesis, then melt fluidity is improved, but heat stabilization performance decreases due to ester function formation

Engineering Contradiction:
Improvemelt fluidityVSAvoidheat stabilization
Core Design Contradiction:
Ease of operationVSReliability

Solution Approach 1:

The patent changes the timing parameter of alcohol incorporation from post-polymerization to during polymerization. This parameter change allows the alcohol to react with monomers rather than forming ester functions with end groups, simultaneously improving melt fluidity and maintaining heat stabilization performance

Inventive Principle:
Principle #35Parameter changes

3Reliability

If polyhydric alcohol is added as a mixture via extrusion, then heat stabilization is achieved, but the alcohol is readily extractable leading to performance decrease

Engineering Contradiction:
Improveheat stabilizationVSAvoidstabilization duration
Core Design Contradiction:
ReliabilityVSDuration of action of stationary object

Solution Approach 1:

The polyhydric alcohol is incorporated into the polyamide structure during polymerization rather than added afterward. This preliminary action ensures the alcohol is covalently bonded to the polymer chains before the product is formed, preventing extraction and eliminating subsequent processing steps

Inventive Principle:
Principle #10Preliminary action

Solution Approach 2:

The patent creates a permanent copy of the stabilizing function by incorporating the polyhydric alcohol into the polymer structure itself. The alcohol becomes an integral part of the polyamide chains, ensuring long-term stability without extraction or degradation of performance over time

Inventive Principle:
Principle #26Copying

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The modified polyamide exhibits superior stability and retention of mechanical properties over time, even at high temperatures, with improved distribution and retention of the polyhydric alcohol, reducing the need for excessive additive amounts and minimizing equipment fouling, while maintaining adequate rheological and mechanical properties.

Implementation Method 1

the polyhydric alcohol may be found covalently bonded to the polyamide chains either by reaction with the end groups of carboxylic acid type or by reaction with the intracatenary amides

Methodology Applied
Scientific EffectCovalent bonding: Chemical Bonding

Implementation Method 2

the polyhydric alcohol may be found covalently bonded to the polyamide chains either by reaction with the end groups of carboxylic acid type or by reaction with the intracatenary amides

Methodology Applied
Scientific EffectCovalent bonding: Chemical Bonding

Data Source

PatentUS10611882B2Stabilized polyamide
Publication Date: 2020.04.07 PERFORMANCE POLYAMIDES SAS

AI summary

The present invention relates to the use of a polyhydric alcohol in a polyamide polymerization process for giving the modified polyamide obtained increased stability toward heat, light and/or bad weather. The invention also relates to a polyamide modified in this way, and also to polyamide compositions that may be used for the preparation of specific articles liable to be subjected to high temperatures.