Multi-layer Polycarbonate Containers with Barrier Inner Layer

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Solution Overview

Problem

Current polycarbonate containers face challenges with gas permeation and substance migration, losing transparency and dimensional stability during sterilization processes, and lack effective barrier properties compared to glass containers.

Innovation Solution

A multi-layer article comprising a bisphenol A polycarbonate layer and an inner layer of poly(2,2,4,4-tetramethyl-1,3-cyclobutylene terephthalate)-co-poly(cyclohexanedimethylene terephthalate) is developed, which maintains transparency and dimensional stability during sterilization and provides improved barrier properties through specific layer configurations and manufacturing processes.

Engineering Contradictions & Design Principles

VSEngineering Contradiction Analysis

1Reliability

If glass containers are used to provide transparency, barrier properties, and sterilization resistance, then these properties are improved, but weight increases and fragility causes production interruptions

Engineering Contradiction:
Improvesterilization resistanceVSAvoidcontainer weight
Core Design Contradiction:
ReliabilityVSWeight of stationary object

Solution Approach 1:

The patent employs a multi-layer composite structure combining polycarbonate (PC) and polyethylene naphthalate (PEN) materials. The PC layer provides impact resistance and toughness, while the PEN layer contributes barrier properties against gas and moisture permeation. This composite approach achieves the reliability and performance characteristics of glass containers while maintaining the weight and durability advantages of plastic materials.

Inventive Principle:
Principle #40Composite materials

2Strength

If polycarbonate containers are used to provide transparency and strength, then these properties are improved, but gas barrier properties deteriorate compared to glass

Engineering Contradiction:
Improvecontainer strengthVSAvoidgas barrier properties
Core Design Contradiction:
StrengthVSReliability

Solution Approach 1:

The patent utilizes a multi-layer composite structure where the polycarbonate layer provides mechanical strength and impact resistance, while the polyethylene naphthalate layer provides superior gas and moisture barrier properties. This composite design allows the container to achieve both high strength and effective gas barrier performance, overcoming the limitations of single-material polycarbonate containers.

Inventive Principle:
Principle #40Composite materials

3Reliability

If heat treatment is applied to polycarbonate containers above glass transition temperature, then sterilization is achieved, but transparency is lost due to haze formation

Engineering Contradiction:
Improvesterilization capabilityVSAvoidtransparency
Core Design Contradiction:
ReliabilityVSIllumination intensity

Solution Approach 1:

The patent employs a multi-layer composite structure where the polycarbonate layer can withstand high-temperature sterilization processes, while the polyethylene naphthalate layer maintains optical clarity and resistance to haze formation. This composite design allows the container to achieve effective sterilization while preserving transparency, overcoming the limitation of single-material polycarbonate containers that develop haze after heat treatment.

Inventive Principle:
Principle #40Composite materials

Applied Scientific Principles

This section explains which scientific principles are used to turn an abstract innovation direction into a practical engineering solution.

Function Achieved in This Case

The multi-layer structure maintains greater than 90% transmission and less than 2.5% haze after sterilization, offering enhanced mechanical strength, thermal stability, and improved gas barrier properties, making it suitable for food and healthcare packaging applications.

Implementation Method 1

the inner layer forms a barrier between the polycarbonate layer and the interior; wherein the multi-layer article is a bi-layer

Methodology Applied
Scientific EffectBarrier properties: Permeation

Implementation Method 2

the article has a decrease in transparency of less than or equal to 5% after sterilization in an autoclave for 30 minutes at 120°C

Methodology Applied
Scientific EffectThermal stability: Thermal Expansion

Data Source

PatentEP3164266B1Multi-layer materials and articles made therefrom and methods of making
Publication Date: 2019.05.29 SABIC GLOBAL TECHNOLOGIES BV
  • EP3164266B1 patent drawingFigure 1A~3
  • EP3164266B1 patent drawingFigure 4~5
  • EP3164266B1 patent drawingFigure 6

AI summary

In an embodiment, a multi-layer article having an interior, the article comprises a second layer comprising a bisphenol A polycarbonate; and an inner layer comprising a terephthalic copolyester; polyethylene furanoate; or a combination comprising at least one of the foregoing; wherein the inner layer forms a barrier between the second layer and the interior. The article has at least one of: a decrease in transparency of less than or equal to 5% after sterilization in an autoclave for 30 minutes at 120°C, and a decrease in transparency of less than or equal to 5% after 50 cycles of hot filling with water for 30 minutes at 90°C.